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In monolayer transition metal dichalcogenides, quantum emitters are associated with localized strain that can be deterministically applied to create designer nano-arrays of single photon sources. Despite an overwhelming empirical…

Controlling excitons at the nanoscale in semiconductor materials represents a formidable challenge in the fields of quantum photonics and optoelectronics. Achieving this control holds great potential for unlocking strong exciton-exciton…

2D materials support unique excitations of quasi-particles that consist of a material excitation and photons called polaritons. Especially interesting are in-plane propagating polaritons which can be confined to a single monolayer and carry…

Excitons and their complexes govern optical-related behaviors in semiconductors. Here, using angle-resolved photoemission spectroscopy (ARPES), we have elucidated the light-matter interaction mediated by quasi-steady excitonic complexes…

Strongly Correlated Electrons · Physics 2025-12-03 Shangkun Mo , Hao Zhong , Keming Zhao , Yunfei Bai , Dingkun Qin , Chunlong Wu , Qiang Wan , Renzhe Li , Cao Peng , Xingzhe Wang , Enting Li , Sheng Meng , Nan Xu

Using first-principles simulations combined with many-body calculations, we show that two-dimensional free-standing quintuple-layer Bi2Se2Te is an inversion symmetric monolayer expected to achieve spatially indirect exciton with large…

Materials Science · Physics 2024-07-18 Yuanyuan Wang , Ying Dai , Baibiao Huang , Yee Sin Ang , Wei Wei

Two-dimensional semiconductors such as MoS2 are an emerging material family with wide-ranging potential applications in electronics, optoelectronics and energy harvesting. Large-area growth methods are needed to open the way to the…

Two-dimensional (2D) transition metal dichalcogenides (TMDs) are prospective materials for quantum devices owing to their inherent 2D confinements. They also provide a platform to realize even lower-dimensional in-plane electron…

Mesoscale and Nanoscale Physics · Physics 2019-12-19 Ziqian Wang , Ruichun Luo , Isaac Johnson , Hamzeh Kashani , Mingwei Chen

Neutral and charged excitons (trions) in atomically-thin materials offer important capabilities for photonics, from ultrafast photodetectors to highly-efficient light-emitting diodes and lasers. Recent studies of van der Waals (vdW)…

Mesoscale and Nanoscale Physics · Physics 2020-08-04 Jaydeep Joshi , Tong Zhou , Sergiy Krylyuk , Albert V. Davydov , Igor Zutic , Patrick M. Vora

We study experimentally and theoretically the exciton-phonon interaction in MoSe2 monolayers encapsulated in hexagonal BN, which has an important impact on both optical absorption and emission processes. The exciton transition linewidth…

TMDCs have attracted a lot of attention in recent years due to their unique indirect to direct band gap transition from bulk to monolayer thickness. Strong confinement in the out-of-plane direction enhances the Coulomb potential between the…

Exciton transport in 2D semiconductors holds promise for room-temperature, ultra-compact optoelectronic devices, but it is limited by short propagation distances. Hybridization of excitons with cavity photons to form exciton-polaritons can…

Mesoscale and Nanoscale Physics · Physics 2025-07-08 Jamie M. Fitzgerald , Roberto Rosati , Ermin Malic

Two-dimensional (2D) monolayer phosphorene, a 2D system with quasi-one-dimensional (quasi-1D) excitons, provides a unique 2D platform for investigating the dynamics of excitons in reduced dimensions and fundamental many-body interactions.…

Materials Science · Physics 2016-02-03 Renjing Xu , Jiong Yang , Ye Win Myint , Jiajie Pei , Han Yan , Fan Wang , Yuerui Lu

We perform coherent nonlinear spectroscopy of excitons in single-layers of MoSe$_2$ and WSe$_2$ encapsulated between thin films of hexagonal boron nitride. Employing four-wave mixing microscopy we identify virtually disorder free areas,…

We investigate the confinement of neutral excitons in a one-dimensional (1D) potential, engineered by proximizing hBN-encapsulated monolayer MoSe$_2$ to ferroelectric domain walls (DW) in periodically poled LiNbO$_3$. Our device exploits…

Mesoscale and Nanoscale Physics · Physics 2025-03-21 Pedro Soubelet , Yao Tong , Asier Astaburuaga Hernandez , Peirui Ji , Katia Gallo , Andreas V. Stier , Jonathan J. Finley

Two-dimensional (2D) heterostructures (HS) formed by transition-metal dichalcogenide (TMDC) monolayers offer a unique platform for the study of intralayer and interlayer excitons as well as moir\'e-pattern-induced features. Particularly,…

Mesoscale and Nanoscale Physics · Physics 2021-11-15 Mohammed Adel Aly , Manan Shah , Lorenz Maximilian Schneider , Kyungnam Kang , Martin Koch , Eui-Hyeok Yang , Arash Rahimi-Iman

The optical properties of atomically thin semiconductors are dominated by excitons, tightly bound electron-hole pairs, which give rise to particularly rich and remarkable physics. Despite their importance, the microscopic formation…

Atomically flat semiconducting materials such as monolayer WSe$_2$ hold great promise for novel optoelectronic devices. Recently, quantum light emission has been observed from bound excitons in exfoliated WSe$_2$. As part of developing…

Mesoscale and Nanoscale Physics · Physics 2018-07-10 L. C. Flatten , L. Weng , A. Branny , S. Johnson , P. R. Dolan , A. A. P. Trichet , B. D. Gerardot , J. M. Smith

We present the micro-photoluminescence ($\mu$PL) and micro-reflectance contrast spectroscopy studies on thin films of MoSe2 with layer thicknesses ranging from a monolayer (1L) up to 5L. The thickness dependent evolution of the ground and…

Mesoscale and Nanoscale Physics · Physics 2016-01-20 Ashish Arora , Karol Nogajewski , Maciej R. Molas , Maciej Koperski , Marek Potemski

Exciton binding energy and excited states in monolayers of tungsten diselenide (WSe2) are investigated using the combined linear absorption and two-photon photoluminescence excitation spectroscopy. The exciton binding energy is determined…

Materials Science · Physics 2015-06-19 Keliang He , Nardeep Kumar , Liang Zhao , Zefang Wang , Kin Fai Mak , Hui Zhao , Jie Shan

Monolayers of transition metal dichalcogenides (TMDs) have recently emerged as a promising optoelectronic platform. To leverage their full potential, however, it is important to understand and engineer the properties of the different…