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Direct laser cooling of molecules has reached a phase space density exceeding 10$^{-6}$ in optical traps, but with rather small molecular numbers. To progress towards quantum degeneracy, a mechanism is needed that combines sub-Doppler…

Atomic Physics · Physics 2023-05-24 Justin J. Burau , Parul Aggarwal , Kameron Mehling , Jun Ye

Calcium monofluoride (CaF) molecules are loaded into an optical dipole trap (ODT) and subsequently laser cooled within the trap. Starting with magneto-optical trapping, we sub-Doppler cool CaF and then load $150(30)$ CaF molecules into an…

We demonstrate loading of SrF molecules into an optical dipole trap (ODT) via in-trap $\Lambda$-cooling. We find that this cooling can be optimized by a proper choice of relative ODT and $\Lambda$ beam polarizations. In this optimized…

Atomic Physics · Physics 2021-10-27 Thomas K. Langin , Varun Jorapur , Yuqi Zhu , Qian Wang , David DeMille

Direct laser cooling and trapping of molecules to temperature below Doppler limit and density exceeding $10^8$ are challenging due to the sub-Doppler heating effects of molecular magneto-optical trap (MOT). In our previous paper [1], we…

Atomic Physics · Physics 2023-05-29 S. Xu , R. Li , Y. Zhai , Y. Xia , M. Siercke , S. Ospelkaus

We present the properties of a magneto-optical trap (MOT) of CaF molecules. We study the process of loading the MOT from a decelerated buffer-gas-cooled beam, and how best to slow this molecular beam in order to capture the most molecules.…

Atomic Physics · Physics 2017-12-06 H. J. Williams , S. Truppe , M. Hambach , L. Caldwell , N. J. Fitch , E. A. Hinds , B. E. Sauer , M. R. Tarbutt

Recent experiments have demonstrated direct cooling and trapping of diatomic and triatomic molecules in magneto-optical traps (MOTs). However, even the best molecular MOTs to date still have density $10^{-5}$ times smaller than in typical…

Atomic Physics · Physics 2023-04-19 Thomas K. Langin , David DeMille

Laser cooling and trapping are central to modern atomic physics. The workhorse technique in cold-atom physics is the magneto-optical trap (MOT), which combines laser cooling with a restoring force from radiation pressure. For a variety of…

Atomic Physics · Physics 2014-10-20 J. F. Barry , D. J. McCarron , E. B. Norrgard , M. H. Steinecker , D. DeMille

We describe experiments demonstrating efficient transfer of molecules from a magneto-optical trap (MOT) into a conservative magnetic quadrupole trap. Our scheme begins with a blue-detuned optical molasses to cool SrF molecules to $\sim\!50$…

Atomic Physics · Physics 2018-07-11 D. J. McCarron , M. H. Steinecker , Y. Zhu , D. DeMille

We demonstrate significantly improved magneto-optical trapping of molecules using a very slow cryogenic beam source and RF modulated and DC magnetic fields. The RF MOT confines $1.1(3) \times 10^5$ CaF molecules at a density of $4(1) \times…

A key method to produce trapped and laser-cooled molecules is the magneto-optical trap (MOT), which is conventionally created using light red-detuned from an optical transition. In this work, we report a MOT for CaF molecules created using…

Atomic Physics · Physics 2024-06-18 Samuel J. Li , Connor M. Holland , Yukai Lu , Lawrence W. Cheuk

We realize laser cooling and trapping of titanium (Ti) atoms in a mangeto-optical trap (MOT). While Ti does not possess a transition suitable for laser cooling out of its $\mathrm{3d^24s^2}$ $\mathrm{a^3F}$ ground term, there is such a…

In red-detuned magneto-optical traps (MOTs) of molecules, sub-Doppler heating competes with Doppler cooling, resulting in high temperature and low density. A solution is offered by the blue-detuned MOT where sub-Doppler cooling dominates…

Atomic Physics · Physics 2026-01-30 Qinshu Lyu , M. R. Tarbutt

We demonstrate a three-dimensional magneto-optical trap (MOT) of a metal hydride molecule, CaH. We are able to scatter $\sim$$10^{4}$ photons with vibrational loss covered up to vibrational quantum number $\nu=2$. This allows us to laser…

Atomic Physics · Physics 2025-12-30 Jinyu Dai , Benjamin Riley , Qi Sun , Debayan Mitra , Tanya Zelevinsky

We describe an approach to optically trapping small, chemically stable molecules at cryogenic temperatures by buffer-gas loading a deep optical dipole trap. The ~10 K trap depth will be produced by a tightly-focused, 1064-nm cavity capable…

We report magneto-optical trapping (MOT) of a polyatomic molecule, calcium monohydroxide (CaOH). The MOT contains $2.0(5)\times 10^4$ CaOH molecules at a peak density of $3.0(8)\times10^{6}$ cm$^{-3}$. CaOH molecules are further sub-Doppler…

We trap and cool a gas composed of 40K and 87Rb, using a two-species magneto-optical trap (MOT). This trap represents the first step towards cooling the Bose-Fermi mixture to quantum degeneracy. Laser light for the MOT is derived from laser…

Statistical Mechanics · Physics 2009-11-07 J. Goldwin , S. B. Papp , B. DeMarco , D. S. Jin

Optically trapped laser-cooled polar molecules hold promise for new science and technology in quantum information and quantum simulation. Large numerical aperture optical access and long trap lifetimes are needed for many studies, but these…

We demonstrate a scheme for magneto-optically trapping strontium monofluoride (SrF) molecules at temperatures one order of magnitude lower and phase space densities three orders of magnitude higher than obtained previously with laser-cooled…

Atomic Physics · Physics 2016-02-17 E. B. Norrgard , D. J. McCarron , M. H. Steinecker , M. R. Tarbutt , D. DeMille

We report an experimental study of peak and phase-space density of a two-stage magneto-optical trap (MOT) of 6-Li atoms, which exploits the narrower $2S_{1/2}\rightarrow 3P_{3/2}$ ultra-violet (UV) transition at 323 nm following trapping…

Atomic Physics · Physics 2015-06-22 Jimmy Sebastian , Christian Gross , Ke Li , Huat Chai Jaren Gan , Wenhui Li , Kai Dieckmann

We present the properties and advantages of a new magneto-optical trap (MOT) where blue-detuned light drives `type-II' transitions that have dark ground states. Using $^{87}$Rb, we reach a radiation-pressure-limited density exceeding…

Atomic Physics · Physics 2018-02-28 K. N. Jarvis , J. A. Devlin , T. E. Wall , B. E. Sauer , M. R. Tarbutt
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