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An adaptive algorithm for spectral proper orthogonal decomposition (SPOD) of mixed broadband-tonal turbulent flows is developed. Sharp peak resolution at tonal frequencies is achieved by locally minimizing the bias of the spectrum. Smooth…

Fluid Dynamics · Physics 2024-06-25 Brandon C. Y. Yeung , Oliver T. Schmidt

We investigate cooperative phenomena and superradiance for vibrational transitions in polar molecule spectroscopy when a high optical-depth (OD) sample is studied. Such cooperativity comes from the build-up of inter-particle coherence…

Atomic Physics · Physics 2015-06-15 Guin-Dar Lin , Susanne F. Yelin

Typical astronomical spectrographs have a resolution ranging between a few hundred to 200.000. Deconvolution and correlation techniques are being employed with a significance down to 1/1000 th of a pixel. HeAr and ThAr lamps are usually…

Astrophysics · Physics 2015-05-13 Piet O. Schmidt , Stefan Kimeswenger , Hans Ulrich Kaeufl

We demonstrated the observation of Rb two-photon absorption directly excided by an optical frequency comb at fiber communication bands. A chain of comb spectral control is elaborately implemented to increase the power of the second harmonic…

Optics · Physics 2015-06-16 Jiutao Wu , Dong Hou , Xiaoliang Dai , Zhengyu Qin , Zhigang Zhang , Jianye Zhao

We propose and demonstrate pump-probe spectroscopy of rubidium absorption which reveals the sub-Doppler hyperfine structure of the $^{5}$S$_{1/2} \leftrightarrow$ $^{5}$P$_{3/2}$ (D2) transitions. The counter propagating pump and probe…

High resolution and fast detection of molecular vibrational absorption is important for organic synthesis, pharmaceutical process and environmental monitoring, and is enabled by mid-infrared (mid-IR) laser frequency combs via dual-comb…

Broadband, high resolution and rapid measurement of dual-comb spectroscopy (DCS) generates a large amount of data stream. We numerically demonstrate significant data compression of DCS spectra by using a compressive sensing technique. Our…

Signal Processing · Electrical Eng. & Systems 2025-05-06 Akira Kawai , Takahiro Kageyama , Ryoichi Horisaki , Takuro Ideguchi

We demonstrate the first cavity-enhanced optical frequency comb spectroscopy in the mid-infrared wavelength region and report the sensitive real-time trace detection of hydrogen peroxide in the presence of a large amount of water. The…

We demonstrate a dual optical frequency comb concept that down-converts arbitrary narrowband D-band (110-170 GHz) signals to baseband without any filter or optical/RF frequency tuning, using low frequency RF components.

Optics · Physics 2025-12-24 Callum Deakin , Zichuan Zhou , Ronit Sohanpal , Zhixin Liu

We demonstrate a miniaturised and highly robust system for performing Doppler-free spectroscopy on thermal atomic vapour for three frequencies as required for cold atom-based quantum technologies. The application of additive manufacturing…

Atomic Physics · Physics 2022-10-04 Somya H Madkhaly , Nathan Cooper , Laurence Coles , Lucia Hackermüller

We present an experiment demonstrating high-resolution coherent control of a four-level atomic system in a closed (diamond) type configuration. A femtosecond frequency comb is used to establish phase coherence between a pair of two-photon…

Quantum Physics · Physics 2009-11-13 Matthew C. Stowe , Avi Pe'er , Jun Ye

We report on the characterization of sub-Doppler resonances detected by probing the 6S$_{1/2}$-7P$_{1/2}$ transition of Cs atom at 459 nm in a microfabricated vapor cell. The dependence of the sub-Doppler resonance (linewidth, amplitude) on…

Mid-infrared femtosecond optical frequency combs were produced by difference frequency generation of the spectral components of a near-infrared comb in a 3-mm-long MgO:PPLN crystal. We observe strong pump depletion and 9.3 dB parametric…

We study resonance redistribution mechanisms inside a hot vapor cell. This is achieved by pumping atoms on the first cesium resonance, 6S1/2-->6P1/2, and subsequently probing the velocity distribution of the 6P1/2 population by a linear…

Chip-scale optical frequency combs can provide broadband spectroscopy for diagnosing complex organic molecules. They are also promising as miniaturized laser spectrometers in applications ranging from atmospheric chemistry to geological…

Optical cavities provide high sensitivity to dispersion since their resonance frequencies depend on the index of refraction. We present a direct, broadband, and accurate measurement of the modes of a high finesse cavity using an optical…

Two-dimensional electronic spectroscopy provides information on coupling and energy transfer between excited states on ultrafast timescales. Only recently, incoherent fluorescence detection has made it possible to combine this method with…

Optics · Physics 2025-05-14 Sanchayeeta Jana , Simon Durst , Lucas Ludwig , Markus Lippitz

Frequency comb-referenced measurements of sub-Doppler laser saturation dip absorption lines in the $v_1+v_3$ band of acetylene near $1.5\,\mu \mathrm{m}$ are reported. These measurements include transitions involving higher rotational…

Chemical Physics · Physics 2020-03-10 Sylvestre Twagirayezu , Gregory E. Hall , Trevor J. Sears

We show that a thermal vapor confined in a nanostructure is of spectroscopic interest. We perform reflection spectroscopy on a Cs vapour cell whose window is covered with a thin opal film (typically, 10 or 20 layers of ~ 1{\mu}m diameter…

Atomic Physics · Physics 2013-06-13 Philippe Ballin , Elias Moufarej , Isabelle Maurin , Athanasios Laliotis , Daniel Bloch

Optically detected magnetic resonance (ODMR) has become a well-established and powerful technique for measuring the spin state of solid-state quantum emitters, at room temperature. Relying on spin-dependent recombination processes involving…

Quantum Physics · Physics 2024-05-30 Dylan G. Stone , Benjamin Whitefield , Mehran Kianinia , Carlo Bradac