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Entanglement of high dimensional states is becoming increasingly important for quantum communication and computing. The most common source of entangled photons is spontaneous parametric down conversion (SPDC), where the degree of frequency…

Quantum Physics · Physics 2020-01-22 C. Okoth , E. Kovlakov , F. Boensel , A. Cavanna , S. Straupe , S. P. Kulik , M. V. Chekhova

Particle entanglement is a fundamental resource upon which are based many quantum technologies. However, the up-to-now best sources of entangled photons rely on parametric down-conversion processes, which are optimal only at certain…

Path-entangled multi-photon states allow optical phase-sensing beyond the shot-noise limit, provided that an efficient parity measurement can be implemented. Realising this experimentally is technologically demanding, as it requires…

We describe two-photon absorption processes excited by entangled pairs, but not by non-entangled pairs of the same energy and polarization. Photon states are selected for destructive interference in the non-entangled process between…

Quantum Physics · Physics 2010-12-21 Keith Kastella , Ralph S. Conti

Entangled photons have the remarkable ability to be more sensitive to signal and less sensitive to noise than classical light. Joint photons can sample an object collectively, resulting in faster phase accumulation and higher spatial…

Optics · Physics 2015-09-04 Chien-Hung Lu , Matthew Reichert , Xiaohang Sun , Jason W. Fleischer

Fluorescence lifetime experiments are a standard approach for measuring excited state dynamics and local environment effects. Here, we show that entangled photon pairs produced from a continuous-wave (CW) laser diode can replicate pulsed…

Quantum Physics · Physics 2023-05-15 Nathan Harper , Bryce P. Hickam , Manni He , Scott K. Cushing

The most important problem of spectroscopic chiral analysis is the inherently weak chiral signals are easily overwhelmed by the environment noises. Enormous efforts had been spent to overcome this problem by enhancing the symmetry break in…

Quantum Physics · Physics 2023-10-05 Chong Ye , Yifan Sun , Xiangdong Zhang

We theoretically investigate the spectral property of biphoton state from the cascade emissions from a Doppler-broadened atomic ensemble. This biphoton state is spontaneously created in the four-wave-mixing process. The upper transition of…

Quantum Physics · Physics 2019-06-14 T. H. Chang , G. -D. Lin , H. H. Jen

Two-photon absorption (TPA) and other nonlinear interactions of molecules with time-frequency-entangled photon pairs (EPP) has been predicted to display a variety of fascinating effects. Therefore, their potential use in practical…

Quantum Physics · Physics 2021-09-15 Michael G. Raymer , Tiemo Landes , Andrew H. Marcus

Spectroscopy with entanglement has shown great potential to break limitations of traditional spectroscopic measurements, yet the role of entanglement in spectroscopic multi-parameter joint measurement, particularly in the infrared optical…

Quantum Physics · Physics 2025-02-25 Xue Zhang , Zhucheng Zhang , Hui Dong

Entanglement--one of the most delicate phenomena in nature--is an essential resource for quantum information applications. Large entangled cluster states have been predicted to enable universal quantum computation, with the required single-…

Ultrafast optical spectroscopy is a powerful technique for studying the dynamic processes of molecular systems in condensed phases. However, in molecular systems containing many dye molecules, the spectra can become crowded and difficult to…

Chemical Physics · Physics 2025-02-05 Yuta Fujihashi , Akihito Ishizaki , Ryosuke Shimizu

Single-photon entanglement may be the simplest type of entanglement but it is of vice importance in quantum communication. Here we present a practical protocol for distilling the single-photon entanglement from both photon loss and…

Quantum Physics · Physics 2013-06-12 Yu-Bo Sheng , Lan Zhou

We propose a novel femtosecond stimulated Raman spectroscopy (FSRS) technique that combines entangled photons with interference detection to select matter pathways and enhance the resolution. Following photo excitation by an actinic pump,…

Quantum Physics · Physics 2014-07-15 Konstantin E. Dorfman , Frank Schlawin , Shaul Mukamel

We report how the unique temporal and spectral features of pulsed entangled photons from a parametric downconversion source can be utilized for manipulating electronic excitations through the optimization of their spectral phase. A new…

Chemical Physics · Physics 2024-09-18 Sajal Kumar Giri , George C. Schatz

Most experimental demonstrations of entanglement require nonclassical states and correlated measurements of single-photon detection events. It is shown here that entanglement can produce a large decrease in the rate of two-photon absorption…

Quantum Physics · Physics 2009-11-11 J. D. Franson

The entanglement spectroscopy, initially introduced by Li and Haldane in the context of the fractional quantum Hall effects, has stimulated an extensive range of studies. The entanglement spectrum is the spectrum of the reduced density…

Strongly Correlated Electrons · Physics 2015-10-28 N. Regnault

We image with cameras entangled photon light transmitted through a random medium. Near-field and far-field spatial quantum correlations show that entangled photon pairs (bi-photons) generated by spontaneous optical parametric…

Quantum Physics · Physics 2019-07-09 Soro Gnatiessoro , Alexis Mosset , Eric Lantz , Fabrice Devaux

We report on an experimental investigation of the dynamics of entanglement between a single qubit and its environment, as well as for pairs of qubits interacting independently with individual environments, using photons obtained from…

Quantum Physics · Physics 2009-09-29 A. Salles , F. Melo , M. P. Almeida , M. Hor-Meyll , S. P. Walborn , P. H. Souto Ribeiro , L. Davidovich

The generation of high-fidelity polarization-entangled photon pairs, to date, has been demonstrated on specific spatial modes or over relatively narrow apertures. We put forward and demonstrate an experimental scheme to extend the temporal…

Quantum Physics · Physics 2021-06-15 Salem F. Hegazy , Salah S. A. Obayya