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We introduce high-harmonic sideband spectroscopy (HHSS) and show that it can be a robust probe of attosecond charge migration (CM) in a halogenated carbon-chain molecule. We simulate both the CM and harmonic-generation (HHG) dynamics using…

Charge migration (CM) is a coherent attosecond process that involves the movement of localized holes across a molecule. To determine the relationship between a molecule's structure and the CM dynamics it exhibits, we perform systematic…

In this paper, we have explored the charge transfer mechanism in transition metal dichalcogenide (TMDC) quantum dots (QDs) of molybdenum disulfide ($\rm{MoS_2}$) and tungsten disulfide ($\rm{WS_2}$). Rhodamine 6G (R6G), a dye from the…

Applied Physics · Physics 2024-09-20 Praveen Mishra , Arun Singh Patel , Sanjay Kumar Chauhan , Anirban Chakraborti

We study the magnetic-field-induced frequency shift (MFS) of the clock (``0--0'') transition in coherent-population-trapping (CPT) microwave atomic clock. It is shown that the use of the Pound-Drever-Hall-like (PDH) technique for frequency…

Atomic Physics · Physics 2025-06-09 Denis Brazhnikov , Vladislav Vishnyakov , Mikhail Skvortsov

We investigate the magnetic-field-induced frequency shift (MFS) of the clock "0-0" transition in the microwave quantum frequency standard (atomic clock) based on coherent population trapping (CPT) in $^{87}$Rb vapor. To scan the CPT…

Atomic Physics · Physics 2025-04-28 V. I. Vishnyakov , D. V. Brazhnikov , M. N. Skvortsov

We present an alternative approach to pump-probe spectroscopy for measuring fast charge dynamics with an atomic force microscope (AFM). Our approach is based on coherent multifrequency lock-in measurement of the intermodulation between a…

Mesoscale and Nanoscale Physics · Physics 2019-01-30 Riccardo Borgani , David B. Haviland

We propose a time-resolved optical measurement scheme for sampling transient charge and spin currents in a bulk centrosymmetric semiconductor. The technique relies on emission of second harmonic light triggered by a pulsed below-gap optical…

Mesoscale and Nanoscale Physics · Physics 2024-06-18 Amin Lakhal , Stéphane Virally , Jacob B. Khurgin , Denis V. Seletskiy

We present a new method that combines fluorescence correlation spectroscopy (FCS) on the microsecond time scale with fluorescence antibunching measurements on the nanosecond time scale for measuring photophysical rate constants of…

Chemical Physics · Physics 2022-03-28 Damir Sakhapov , Ingo Gregor , Narain Karedla , Jörg Enderlein

A novel broadband microwave (MW) spectrum measurement (BMSM) scheme based on code-free optical undersampling and homodyne detection is proposed. The fully analog generation of optical pulses with a far-less-than-Nyquist rate is only through…

Signal Processing · Electrical Eng. & Systems 2019-08-02 Guangyu Gao , Xueshuang Xiang , Qijun Liang , Naijin Liu

We present a hybrid laser frequency stabilization method combining modulation transfer spectroscopy (MTS) and frequency modulation spectroscopy (FMS) for the cesium D2 transition. In a typical pump-probe setup, the error signal is a…

The CMS Beam Conditions and Radiation Monitoring System, BRM, will support beam tuning, protect the CMS detector from adverse beam conditions, and measure the accumulated dose close to or inside all sub-detectors. It is composed of…

Instrumentation and Detectors · Physics 2014-11-20 A. Bell , E. Castro , R. Hall-Wilton , W. Lange , W. Lohmann , A. Macpherson , M. Ohlerich , N. Rodriguez , V. Ryjov , R. S. Schmidt , R. L. Stone

We propose a novel scheme for probing vibronic coherence in charge migration in molecules utilizing strong field sequential double ionization. To demonstrate the feasibility of this approach, we perform full simulations of a pump-probe…

Atomic Physics · Physics 2024-01-09 C. H. Yuen , C. D. Lin

The Field-Transformation Hybrid Monte-Carlo (FTHMC) algorithm potentially mitigates the issue of critical slowing down by combining the HMC with a field transformation, originally proposed by L\"{u}scher and motivated as trivializing the…

High Energy Physics - Lattice · Physics 2025-02-11 Shuhei Yamamoto , Peter Boyle , Taku Izubuchi , Luchang Jin , Christoph Lehner , Nobuyuki Matsumoto

A new method, FM-FTS, combining Frequency Modulation heterodyne laser spectroscopy and Fourier Transform Spectroscopy is presented. It provides simultaneous sensitive measurement of absorption and dispersion profiles with broadband spectral…

Optics · Physics 2007-09-24 Julien Mandon , Guy Guelachvili , Nathalie Picqué

Frequency-modulated (FM) combs are produced by mode-locked lasers in which the electric field has a linearly chirped frequency and nearly constant amplitude. This regime of operation occurs naturally in certain laser systems and constitutes…

We report, for the first time, a multi-confocal Fluorescence Correlation Spectroscopy (mFCS) technique which allows parallel measurements at different locations, by combining a Spatial Light Modulator (SLM), with an Electron Multiplying-CCD…

Precision space inertial sensors are imperative for Earth geodesy missions, gravitational wave observations, and fundamental physics experiments in space. In these missions, free-falling test masses(TMs) are susceptible to parasitic…

Instrumentation and Detectors · Physics 2024-12-16 Fangchao Yang , Wei Hong , Yujie Zhao

A photonics-enabled wavelet-like transform system, characterized by multi-resolution time-frequency analysis, is proposed based on a typical stimulated Brillouin scattering (SBS) pump-probe setup using an optical nonlinear frequency-sweep…

Optics · Physics 2022-08-22 Pengcheng Zuo , Dong Ma , Yang Chen

We present a hybrid method based on a combination of quantum/classical molecular dynamics (MD) simulations and a mod el Hamiltonian approach to describe charge transport through bio-molecular wires with variable lengths in presence o f a…

Soft Condensed Matter · Physics 2015-05-13 R. Gutierrez , R. Caetano , P. B. Woiczikowski , T. Kubar , M. Elstner , G. Cuniberti

Conformational dynamics of biomolecules are of fundamental importance for their function. Single-molecule F\"orster Resonance Energy Transfer (smFRET) is a powerful approach to inform on the structure and the dynamics of labeled molecules.…

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