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A broad effort is underway to improve the sensitivity of nuclear magnetic resonance through the use of dynamic nuclear polarization. Nitrogen-vacancy (NV) centers in diamond offer an appealing platform because these paramagnetic defects can…

In this work we present a new formalism to evaluate the nuclear spin dynamics driven by hyperfine interaction with non-equilibrium electron spins. To describe the dynamics up to second order in the hyperfine coupling, it suffices to…

Mesoscale and Nanoscale Physics · Physics 2011-07-12 J. Danon , Yu. V. Nazarov

Dynamic nuclear polarization experiments use microwave irradiation to transfer the larger electron polarization to nuclear spins of interest, and thus enhance the NMR transitions above thermal equilibrium. How the polarization transfer from…

Chemical Physics · Physics 2026-01-12 Gian-Marco Camenisch , Nino Wili , Gunnar Jeschke , Matthias Ernst

In this article, we study control of electron-nuclear spin dynamics at magnetic field strengths where the Larmor frequency of the nucleus is comparable to the hyperfine coupling strength. The quantization axis for the nuclear spin differs…

Quantum Physics · Physics 2009-11-13 Navin Khaneja

Dynamical magnetic and nuclear polarization in complex spin systems is discussed on the example of transfer of spin from exciton to the central spin of magnetic impurity in a quantum dot in the presence of a finite number of nuclear spins.…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 Ramin M. Abolfath , Anna Trojnar , Bahman Roostaei , Thomas Brabec , Pawel Hawrylak

We analytically solve the {\it Non-Markovian} single electron spin dynamics due to hyperfine interaction with surrounding nuclei in a quantum dot. We use the equation-of-motion method assisted with a large field expansion, and find that…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Changxue Deng , Xuedong Hu

We report a systematic study of the hyperfine interaction between the electron spin of a single nitrogen-vacancy (NV) defect in diamond and nearby $^{13}$C nuclear spins, by using pulsed electron spin resonance spectroscopy. We isolate a…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 A. Dréau , J. -R. Maze , M. Lesik , J. -F. Roch , V. Jacques

Optically-detected paramagnetic centers in wide-bandgap semiconductors are emerging as a promising platform for nanoscale metrology at room temperature. Of particular interest are applications where the center is used as a probe to…

Mesoscale and Nanoscale Physics · Physics 2015-12-09 Abdelghani Laraoui , Daniela Pagliero , Carlos A. Meriles

The periodical modulation of circularly polarized light with a frequency close to the electron spin resonance frequency induces a sharp change of the single electron spin orientation. Hyperfine interaction provides a feedback, thus fixing…

Mesoscale and Nanoscale Physics · Physics 2013-05-29 V. L. Korenev

Nuclear spins in the proximity of electronic spin defects in solids are promising platforms for quantum information processing due to their ability to preserve quantum states for a remarkably long time. Here we report a comprehensive study…

Quantum Physics · Physics 2023-10-03 Mykyta Onizhuk , Giulia Galli

The interplay between disorder and transport is a problem central to the understanding of a broad range of physical processes, most notably the ability of a system to reach thermal equilibrium. Disorder and many body interactions are known…

We theoretically study the interplay of spin-orbit and hyperfine interactions in dynamical nuclear polarization in two-electron semiconductor double quantum dots near the singlet $(S)$ - triplet $(T_+)$ anticrossing. The goal of the scheme…

Mesoscale and Nanoscale Physics · Physics 2016-01-20 Marko J. Rančić , Guido Burkard

We show that the hyperfine mediated dynamics of heavy hole states confined in neutral self- assembled quantum dots leads to a nuclear spin diffusion mechanism. It is found that the oftentimes neglected effective heavy hole hyperfine…

Mesoscale and Nanoscale Physics · Physics 2014-03-04 Hugo Ribeiro , Franziska Maier , Daniel Loss

The integration of NMR and high pressure technique brings unique opportunities to study electronic, structural and dynamical properties under extreme conditions. Despite a great degree of success has been achieved using coil-based schemes,…

Quantum Physics · Physics 2022-03-22 Yan-Xing Shang , Fang Hong , Jian-Hong Dai , Ya-Nan Lu , Hui Yu , Yong-Hong Yu , Xiao-Hui Yu , Xin-Yu Pan , Gang-Qin Liu

We investigate nuclear spin hyperpolarization from nitrogen vacancy centers in isotopically enriched diamonds with $^{13}$C concentrations up to 100%. $^{13}$C enrichment leads to hyperfine structure of the nitrogen vacancy electron spin…

Hybridized nuclear and electron spin excitation in a MnCO$_3$ crystal, a weakly-anisotropic antiferromagnet, has been investigated. In this material, the hyperfine interaction is strong enough to form a nuclear spin wave. We measure the…

Similar to nitrogen-vacancy centers in diamond and impurity atoms in silicon, interstitial gallium deep paramagnetic centers in GaAsN have been proven to have useful characteristics for the development of spintronic devices. Among other…

Nuclear spins in solids exhibit long coherence times due to the small nuclear gyromagnetic ratio. This weak environmental coupling comes at the expense of slow quantum gate operations, which should be as fast as possible for many…

Quantum Physics · Physics 2022-11-11 R. M. Goldblatt , A. M. Martin , A. A. Wood

The optically induced polarization of localized electron spins in an ensemble of quantum dots (QDs) dephases due to the interaction with the surrounding nuclear spins. Despite this dephasing, the spins in the QDs can be controlled to…

Mesoscale and Nanoscale Physics · Physics 2022-04-08 P. Schering , G. S. Uhrig

We determine the polarization of the bulk $^{13}$C nuclear spin system in diamond produced by interaction with optically oriented nitrogen-vacancy (NV-) defect centers. $^{13}$C nuclei are polarized into the higher energy Zeeman state with…

Other Condensed Matter · Physics 2015-05-14 Jonathan P. King , Patrick J. Coles , Jeffrey A. Reimer