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As it is known from visible light experiments, silicon under femtosecond pulse irradiation can undergo the so-called 'nonthermal melting' if the density of electrons excited from the valence to the conduction band overcomes a certain…

Materials Science · Physics 2015-04-21 Nikita Medvedev , Zheng Li , Beata Ziaja

Laser melting of semiconductors has been observed for almost 40 years; surprisingly, it is not well understood where most theoretical simulations show a laser-induced thermal process. $\textit{Ab initio}$ nonadiabatic simulations based on…

Materials Science · Physics 2016-12-06 Chao Lian , S. B. Zhang , Sheng Meng

X-ray laser-induced structural changes in silicon undergoing femtosecond melting have been investigated by using an x-ray pump-x-ray probe technique. The experimental results for different initial sample temperatures reveal that the onset…

We predict ultrafast modulation of the pure molten metal surface stress fields under the irradiation of the single femtosecond laser pulse through the two-temperature model molecular-dynamics simulations. High-resolution and precision…

Materials Science · Physics 2022-07-13 Chenhao Li , Hongtao Liang , Yang Yang , Zhiyong Yu , Xin Zhang , Xiangming Ma , Wenliang Lu , Zhenrong Sun , Ya Cheng

Extreme electron-ion non-equilibrium states, generated by ultrafast laser excitation, lead to melting processes that are fundamentally different from those under conventional thermal equilibrium and remain not fully understood. Through…

Computational Physics · Physics 2025-11-27 Qiyu Zeng , Xiaoxiang Yu , Bo Chen , Shen Zhang , Kaiguo Chen , Dongdong Kang , Jiayu Dai

Femtosecond, 8.04 KeV x-ray pulses are used to probe the lattice dynamics of 150 nm Cu (111) single crystal on mica substrate irradiated with 400 nm, 100 fs laser pulses. For pump fluencies below the damage and melting threshold, we…

Materials Science · Physics 2017-03-08 Runze Li , Omar A. Ashour , Jie Chen , H. E. Elsayed-Ali , Peter M. Rentzepis

Ultrafast electron dynamics of solids after an absorption of femtosecond laser pulse is governed by electron-electron, electron-phonon, phonon-electron, and phonon-phonon collisions. It is of importance to construct a framework for…

Materials Science · Physics 2019-01-16 Shota Ono

The ultrafast laser-induced solid-liquid phase transition in metals is still not clearly understood and its accurate quantitative description remains a challenge. Here we systematically investigated, both experimentally and theoretically,…

We investigate photoinization, energy deposition, plasma formation and the ultrafast optical breakdown in crystalline silicon irradiated by intense near-infrared laser pulses with pulse duration $\tau \le $ 100 fs. The occurrence of…

Materials Science · Physics 2021-11-24 Tzveta Apostolova , Boyan Obreshkov

The ultrafast dynamics of ions in solids following intense femtosecond laser excitation is governed by two fundamentally distinct yet interplaying effects. On one hand, the significant generation of hot electron-hole pairs by the light…

Computational Physics · Physics 2024-01-22 Bernd Bauerhenne , Martin E. Garcia

The mechanisms of ripple formation on silicon surface by femtosecond laser pulses are investigated. We demonstrate the transient evolution of the density of the excited free-carriers. As a result, the experimental conditions required for…

Materials Science · Physics 2015-06-15 Thibault J. -Y. Derrien , Tatiana E. Itina , Rémi Torres , Thierry Sarnet , Marc Sentis

The absorbed laser energy of a femtosecond laser pulse in a transparent material induces a warm dense matter region which relaxation may lead to structural modifications in the surrounding cold matter. The modeling of the…

Femtosecond pulses have been used to reveal hidden broken symmetry states and induce transitions to metastable states. However, these states are mostly transient and disappear after laser removal. Photoinduced phase transitions towards…

Materials Science · Physics 2023-10-13 Stefano Mocatti , Giovanni Marini , Matteo Calandra

We present an atomistic-continuum model to simulate ultrashort laser-induced melting processes in semiconductor solids on the example of silicon. The kinetics of transient non-equilibrium phase transition mechanisms is addressed with a…

Materials Science · Physics 2015-11-26 V. P. Lipp , B. Rethfeld , M. E. Garcia , D. S. Ivanov

We present a theoretical study of the ultrafast electron dynamics in transition metals using ultrashort pulsed laser beams. The significant influence of the contribution of the dynamics of produced nonthermal electrons to electron…

Materials Science · Physics 2016-12-14 George D. Tsibidis

This paper describes the effects of electronic nonequilibrium in a simulation of ultrafast laser irradiation of materials. The simulation scheme based on tight-binding molecular dynamics, in which the electronic populations are traced with…

Materials Science · Physics 2023-12-29 Nikita Medvedev

Plasma dynamics critically depends on density and temperature, thus well-controlled experimental realizations are essential benchmarks for theoretical models. The formation of an ultracold plasma can be triggered by ionizing a tunable…

Exciting electrons in solids with intense light pulses offers the possibility of generating new states of matter through nonthermal means and controlling their macroscopic properties on femto- to picosecond timescales. One way to manipulate…

Materials Science · Physics 2021-10-07 Alfred Zong , Anshul Kogar , Nuh Gedik

Ultrafast lasers create extreme, non-equilibrium thermodynamic conditions that can transiently reach pressures and temperatures comparable to interior core of the earth. Here we show that femtosecond excitation of amorphous silica-hafnia…

Electron dynamics in the bulk of large band gap dielectric crystals induced by intense femtosecond laser pulses at 800 nm is studied. With laser intensities under the ablation threshold (a few 10 TW/cm\textsuperscript{2}), electrons with…

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