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Optical nonlinearities - how light-matter interactions are influenced by previous interactions with photons, are key resources in the contemporary photonics toolbox, relevant to quantum gate operations and all-optical switches. Optical…

Electronically excited states of molecules are at the heart of photochemistry, photophysics, as well as photobiology and also play a role in material science. Their theoretical description requires highly accurate quantum chemical…

Chemical Physics · Physics 2021-03-15 Julia Westermayr , Philipp Marquetand

Entanglement generation in polariton systems is fundamentally constrained by high losses and decoherence, which typically outweigh polariton nonlinearities. Here, we propose a conceptually different approach that uses optomechanical…

Exciton-polaritons are mixed light-matter particles offering a versatile solid state platform to study many-body physical effects. In this work we demonstrate an electrically controlled polariton laser, in a compact, easy-to-fabricate and…

Exciton-polaritons in organic materials are hybrid states that result from the strong interaction of photons and the bound excitons that these materials host. Organic polaritons hold great interest for optoelectronic applications, however…

We introduce stochastic techniques that enable the simulations of polaritons resulting from placing giant 2D molecular aggregate crystals with $10^8$ interacting excitonic dyes in realistic multi-mode cavities. We show that the…

Chemical Physics · Physics 2024-06-06 Nadine Bradbury , Raphael Ribeiro , Justin R. Caram , Daniel Neuhauser

Experimental evidence of strong coupling between excitons confined in a quantum well and the photonic modes of a two-dimensional dielectric lattice is reported. Both resonant scattering and photoluminescence spectra at low temperature show…

Strong optical nonlinearities play a central role in realizing quantum photonic technologies. In solid state systems, exciton-polaritons, which result from the hybridization of material excitations and cavity photons, are an attractive…

Polaritonic chemistry relies on the strong light-matter interaction phenomena for altering the chemical reaction rates inside optical cavities. To explain and to understand these processes, the development of reliable theoretical models is…

Chemical Physics · Physics 2022-09-14 Fabijan Pavošević , Angel Rubio

Strong light-matter coupling between molecules and plasmonic nanoparticles give rise to new hybrid eigenstates of the coupled system, commonly referred to as polaritons, or more precisely, plexcitons. Over the last decade it has been amply…

Chemical Physics · Physics 2024-02-06 Marco Romanelli , Stefano Corni

This thesis studies light-matter interactions in strong and weak coupling regimes. In the first part, we study the formation and propagation of exciton-polariton condensates in different microcavities in the strong coupling regime.…

Mesoscale and Nanoscale Physics · Physics 2024-01-19 Dogyun Ko

We show theoretically that polariton pairs with a high degree of polarization entanglement can be produced through parametric scattering. We demonstrate that it can emerge in coincidence experiments, even at low excitation densities where…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 S. Portolan , O. Di Stefano , S. Savasta , V. Savona

A theoretical framework is presented for the computation of rovibrational polaritonic states of a molecule in a lossless infrared (IR) microcavity. In the proposed approach the quantum treatment of the rotational and vibrational motion of…

Chemical Physics · Physics 2023-10-30 Tamás Szidarovszky

Strong coupling in the conventional sense requires that the Rabi cycling process between two interacting states is faster than other dissipation rates. Some recent experimental findings show intriguing properties that were attributed to…

Materials Science · Physics 2026-03-09 Ben Johns , Nitin Yadav , Anand Vinod , Kuljeet Kaur , Jino George

A photon-magnon hybrid system can be realised by coupling the electron spin resonance of a magnetic material to a microwave cavity mode. The quasiparticles associated with the system dynamics are the cavity magnon polaritons, which arise…

Quantum Physics · Physics 2020-10-26 N. Crescini , C. Braggio , G. Carugno , A. Ortolan , G. Ruoso

In this theoretical work, we study a double quantum dot interacting strongly with a microcavity, while undergoing resonant tunneling. Effects of interdot tunneling on the light-matter hybridized states are determined, and tunability of…

Quantum Physics · Physics 2018-11-08 Marlon S. Domínguez , David F. Macias-Pinilla , Hanz Y. Ramírez

We study the resonant electronic excitation dynamics for ultracold atoms trapped in a deep optical lattice prepared in a Mott insulator state. Excitons in these artificial crystals are similar to Frenkel excitons in Noble atom or molecular…

Quantum Physics · Physics 2009-08-11 Hashem Zoubi , Helmut Ritsch

Polaritonic chemistry is an interdisciplinary emerging field that presents several challenges and opportunities in chemistry, physics, and engineering. A systematic review of polaritonic response theory is presented, following a chemical…

Chemical Physics · Physics 2023-05-08 Matteo Castagnola , Rosario R. Riso , Alberto Barlini , Enrico Ronca , Henrik Koch

This perspective provides a brief introduction into the theoretical complexity of polaritonic chemistry, which emerges from the hybrid nature of strongly coupled light-matter states. To tackle this complexity, the importance of ab initio…

Chemical Physics · Physics 2022-06-29 Dominik Sidler , Michael Ruggenthaler , Christian Schäfer , Enrico Ronca , Angel Rubio

Exciton-polaritons formed inside optical cavities offer a highly tunable platform for exploring novel quantum phenomena. Here, we introduce and theoretically characterize a light-matter moir\'e effect (LMME) that arises when a 2D material…