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Related papers: Emergent Trion-Phonon Coupling in Atomically-Recon…

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The optical properties of semiconducting transition metal dichalcogenides are dominated by both neutral excitons (electron-hole pairs) and charged excitons (trions) that are stable even at room temperature. While trions directly influence…

Mesoscale and Nanoscale Physics · Physics 2016-07-26 Kai Hao , Lixiang Xu , Philipp Nagler , Akshay Singh , Kha Tran , Chandriker Kavir Dass , Christian Schüller , Tobias Korn , Xiaoqin Li , Galan Moody

Moire superlattices in twisted transition metal dichalcogenide bilayers have emerged as a rich platform for exploring strong correlations using optical spectroscopy. Despite observation of rich Mott-Wigner physics stemming from an interplay…

Mesoscale and Nanoscale Physics · Physics 2021-11-10 Ido Schwartz , Yuya Shimazaki , Clemens Kuhlenkamp , Kenji Watanabe , Takashi Taniguchi , Martin Kroner , Ataç Imamoğlu

We present the Raman scattering results on layered 2D semiconducting ferromagnetic compound CrSiTe$_3$. Four Raman active modes, predicted by symmetry, have been observed and assigned. The experimental results are supported by DFT…

Materials Science · Physics 2018-10-16 A. Milosavljević , A. Šolajić , J. Pešić , Yu Liu , C. Petrovic , N. Lazarević , Z. V. Popović

Photoluminescence experiments from monolayer transition-metal dichalcogenides often show that the binding energy of trions is conspicuously similar to the energy of optical phonons. This enigmatic coincidence calls into question whether…

Materials Science · Physics 2019-05-31 Dinh Van Tuan , Aaron M. Jones , Min Yang , Xiaodong Xu , Hanan Dery

Layered two-dimensional (2D) semiconductors such as molybdenum disulfide (MoS2) have recently attracted remarkable attention because of their unique physical properties. Here, we use photoluminescence (PL) and Raman spectroscopy to study…

Doped van der Waals heterostructures host layer-hybridized trions, i.e. charged excitons with layer-delocalized constituents holding promise for highly controllable optoelectronics. Combining a microscopic theory with photoluminescence (PL)…

Mesoscale and Nanoscale Physics · Physics 2024-08-08 Raul Perea-Causin , Samuel Brem , Fabian Buchner , Yao Lu , Kenji Watanabe , Takashi Taniguchi , John M. Lupton , Kai-Qiang Lin , Ermin Malic

We present experimental and theoretical results on the high-quality single-layer MoS$_{2}$ which reveal the fine structure of charged excitons, i.e., trions. In the emission spectra we resolve and identify two trion peaks, T$_{1}$ and…

We present a fully analytical model of hybridization between magnon, and phonons observed experimentally in magneto-Raman scattering in van der Waals (vdW) antiferromagnets (AFM). Here, the representative material, FePS3, has been shown to…

Mesoscale and Nanoscale Physics · Physics 2025-01-03 Somsubhra Ghosh , Mainak Palit , Sujan Maity , Subhadeep Datta

Moir\'{e} superlattices in transition metal dichalcogenide heterostructures provide a platform to engineer many-body interactions. Here, we realize a bichromatic moir\'{e} superlattice in an asymmetric WSe$_2$/WS$_2$/WSe$_2$ heterotrilayer…

Hybrid structures incorpora1ng both III-nitride and Transi1on Metal Dichalcogenide (TMD) semiconductors have strong applica1on poten1al for light harves1ng and optoelectronics. Here we have inves1gated the proper1es of hybrid structures…

Materials Science · Physics 2025-09-09 D. Chen , D. Lagarde , L. Hemmen , L. Lombez , P. Renucci , M. Mauguet , L. Ren , C. Robert , N. Grandjean , X. Marie

Transition-metal dichalcogenide bilayers exhibit a rich exciton landscape including layer-hybridized excitons, i.e. excitons which are of partly intra- and interlayer nature. In this work, we study hybrid exciton-exciton interactions in…

Mesoscale and Nanoscale Physics · Physics 2023-06-28 Daniel Erkensten , Samuel Brem , Raul Perea-Causin , Joakim Hagel , Fedele Tagarelli , Edoardo Lopriore , Andras Kis , Ermin Malic

We introduce density imbalanced electron-hole bilayers at a commensurate 2 : 1 density ratio as a platform for realizing novel phases involving electrons, excitons and trions. Three length scales are identified which characterize the…

Strongly Correlated Electrons · Physics 2024-05-28 David D. Dai , Liang Fu

We report the experimental observation of quadrupolar exciton states in the reflectance contrast spectrum of 2$H$-stacked bilayer MoSe$_2$. The application of a vertical electric field results in a quadratic energy redshift of these…

Layered materials such as graphite and transition metal dichalcogenides have extremely anisotropic mechanical properties owing to orders of magnitude difference between in-plane and out-of-plane interatomic interaction strengths. Although…

Materials Science · Physics 2017-11-10 Jae-Ung Lee , Sungjong Woo , Jaesung Park , Hee Chul Park , Young-Woo Son , Hyeonsik Cheong

We analyze the lineshape of the quasiparticle photoluminescence of monolayer and bilayer molybdenum ditelluride in temperature- and excitation intensity-dependent experiments. We confirm the existence of a negatively charged trion in the…

Twisted bilayer two-dimensional transition-metal dichalgocenides (TMDCs) exhibit a range of novel phenomena such as the formation of moir\'e excitons and strongly correlated phases. The coupling between the layers is crucial for the…

Materials Science · Physics 2024-09-27 Eileen Schneider , Kenji Watanabe , Takashi Taniguchi , Janina Maultzsch

We investigated interlayer phonon modes of mechanically exfoliated few-layer 2H-SnS2 samples by using room temperature low-frequency micro-Raman spectroscopy. Raman measurements were performed using laser wavelength of 441.6, 514.4, 532 and…

Materials Science · Physics 2018-07-16 Tharith Sriv , Kangwon Kim , Hyeonsik Cheong

We investigate the ultralow-frequency Raman response of atomically thin ReS2, a special type of two-dimensional (2D) semiconductors with unique distorted 1T structure. Bilayer and few-layer ReS2 exhibit rich Raman spectra at frequencies…

Mesoscale and Nanoscale Physics · Physics 2016-02-16 Rui He , Jia-An Yan , Zongyon Yin , Zhipeng Ye , Gaihua Ye , Jason Cheng , Ju Li , C. H. Lui

Moir\'e patterns with angular mismatch in van der Waals heterostructures composed of atomically thin semiconducting materials are a fascinating platform to engineer the optically generated excitonic properties towards novel quantum…

Mesoscale and Nanoscale Physics · Physics 2020-12-17 Keisuke Shinokita , Yuhei Miyauchi , Kenji Watanabe , Takashi Taniguchi , Kazunari Matsuda

Photoluminescence spectra, shows that monolayer Transition-metal dichalcogenides (MLTMDCs), possess charged exciton binding energies, conspicuously similar to the energy of optical phonons. This enigmatic coincidence has offered…

Mesoscale and Nanoscale Physics · Physics 2020-09-16 Sabrine Ayari , Sihem Jaziri , Robson Ferreira , Gerald Bastard