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We report new techniques for driving high-fidelity stimulated Raman transitions in trapped ion qubits. An electro-optic modulator induces sidebands on an optical source, and interference between the sidebands allows coherent Rabi…

Long-lived (symmetry protected) hyperpolarized spin states offer important new opportunities (for example, in clinical MR imaging), but existing methods for producing these states are limited by either excess energy dissipation or high…

Chemical Physics · Physics 2015-06-17 Thomas Theis , Yesu Feng , Tung-Lin Wu , Warren S. Warren

Benefiting from both molecular tunability and versatile methods for deployment, optically interfaced molecular spins are a promising platform for quantum technologies such as sensing and imaging. Room-temperature optically detected coherent…

We report on coherent control of excitation processes of translationally ultracold rubidium dimers in a magneto-optical trap by using shaped femtosecond laser pulses. Evolution strategies are applied in a feedback loop in order to optimize…

A single-seed, module-based compact laser system is demonstrated on a transportable $^{87}\text{Rb}$-based high-precision atomic gravimeter. All the required laser frequencies for the atom interferometry are provided by free-space…

Atomic Physics · Physics 2022-10-24 Fong En Oon , Rainer Dumke

A simplified analytical model of the resonant interaction of the beam of Larmor electrons drifting in the crossed constant fields of a magnetron with a synchronous wave providing a phase grouping of the drifting charge was developed to…

Accelerator Physics · Physics 2018-07-27 G. Kazakevich , R. Johnson , V. Lebedev , V. Yakovlev , V. Pavlov

We describe a method for improving coherent control through the use of detailed knowledge of the system's Hamiltonian. Precise unitary transformations were obtained by strongly modulating the system's dynamics to average out unwanted…

Electron spins in quantum dots under coherent control exhibit a number of novel feedback processes. Here, we present experimental and theoretical evidence of a feedback process between nuclear spins and a single electron spin in a single…

We report on the coherent optical excitation of electron spin polarization in the ground state of charged GaAs quantum dots via an intermediate charged exciton (trion) state. Coherent optical fields are used for the creation and detection…

We report successful manipulation of non-classical atomic spin states. We generate squeezed spin states by a spin quantum nondemolition measurement, and apply an off-resonant circularly-polarized light pulse to the atoms. By changing the…

Quantum Physics · Physics 2015-05-14 Tetsushi Takano , Shin-Ichi-Ro Tanaka , Ryo Namiki , Yoshiro Takahashi

A central prospect of antiferromagnetic spintronics is to exploit magnetic properties that are unavailable with ferromagnets. However, this poses the challenge of accessing such properties for readout and control. To this end, light-induced…

We present an X-ray based stimulated Raman approach to control the preparation of optically dark electronic states in generic molecular systems. Leveraging on the unique properties of core-level excited states, we demonstrate that optically…

The coherent excitation of an optically active spin system is one of the key elements in the engineering of a spin-photon interface. Using the novel SUPER scheme, we coherently control the main optical transition of a tin-vacancy color…

Manipulation of single spins is essential for spin-based quantum information processing. Electrical control instead of magnetic control is particularly appealing for this purpose, since electric fields are easy to generate locally on-chip.…

Mesoscale and Nanoscale Physics · Physics 2008-03-10 K. C. Nowack , F. H. L. Koppens , Yu. V. Nazarov , L. M. K. Vandersypen

Stokes Raman scattering is known to be a particularly robust nonlinearity, occurring in virtually every material, with spectra defined by the material and strengths dependent on the material as well as light intensities. This ubiquity has…

Optics · Physics 2021-08-10 Xiao Liu , Zelin Ma , Aku Antikainen , Siddharth Ramachandran

Detecting and controlling nuclear spin nano-ensembles is crucial for the further development of nuclear magnetic resonance (NMR) spectroscopy and for the emerging solid state quantum technology. Here we present the fabrication of a…

The key information about any nanoscale system are orientations and conformations of its parts. Unfortunately, these details are often hidden below the diffraction limit and elaborate techniques must be used to optically probe them. Here,…

A hole spin is a potential solid-state q-bit, that may be more robust against nuclear spin induced dephasing than an electron spin. Here we propose and demonstrate the sequential preparation, control and detection of a single hole spin…

The manipulation and metrology of light beams are pivotal for optical science and applications. In particular, achieving ultra-high precision in the measurement of light beam rotations has been a long-standing challenge. Instead of…

Quantum Physics · Physics 2025-10-13 Binke Xia , Jingzheng Huang , Hongjing Li , Zhongyuan Luo , Guihua Zeng

In recent years, unshielded atomic systems have been attracting researchers' attention, in which decoherence is one of the major problems, especially for high precision measurements. The nonlinear Zeeman effect and magnetic field gradient…

Atomic Physics · Physics 2021-07-28 Peiyu Yang , Guzhi Bao , L. Q. Chen , Weiping Zhang
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