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Electron removal in collisions of alpha particles with neon dimers is studied using an independent-atom-independent-electron model based on the semiclassical approximation of heavy-particle collision physics. The dimer is assumed to be…

Atomic Physics · Physics 2022-07-06 Tom Kirchner

We report on the experimental observation of interatomic Coulombic decay (ICD) in pure $^4$He nanoclusters of mean sizes between $N \approx$ 5000 and 30000 and the subsequent scattering of energetic He$^+$ fragments inside the neutral…

An ultrafast mechanism belonging to the family of interatomic Coulombic decay (ICD) phenomena is proposed. When two excited species are present, an ultrafast energy transfer can take place bringing one of them to its ground state and…

To exploit the high intensity of laser radiation, we propose to select frequencies at which single-photon absorption is of too low energy and two or more photons are needed to produce states of an atom that can undergo interatomic Coulombic…

Atomic and Molecular Clusters · Physics 2012-01-04 Philipp V. Demekhin , Spas D. Stoychev , Alexander I. Kuleff , Lorenz S. Cederbaum

Excited atoms and molecules can utilize their excess energy to ionize a neighboring system by a process named interatomic and intermolecular Coulombic decay (ICD). ICD is ultrafast, in the femtosecond regime, and has many modes of…

Chemical Physics · Physics 2026-03-10 Alan G. Falkowski , Alexander I. Kuleff , Lorenz S. Cederbaum

The electron removal and excitation channels in argon dimer target and helium ion projectile collision systems that facilitate interatomic Coulombic decay (ICD) are investigated. We implement an independent-atom and independent-electron…

Atomic and Molecular Clusters · Physics 2026-03-25 Darij Starko , Tom Kirchner

Interatomic Coulombic decay (ICD) plays a crucial role in weakly bound complexes exposed to intense or high-energy radiation. So far, neutral or ionic atoms or molecules have been prepared in singly excited electron or hole states which can…

Interatomic coulombic decay (ICD) is a relaxation process induced by electronic correlation. In this work we study the ICD process in a two coupled Quantum wells (QWs) nano-structure. We study a simple one-dimensional effective potential…

Mesoscale and Nanoscale Physics · Physics 2015-06-11 Tamar Goldzak , Liron Gantz , Ido Gilary , Gad Bahir , Nimrod Moiseyev

When weakly-bound complexes are multiply excited by intense electromagnetic radiation, energy can be exchanged between neighboring atoms through a type of resonant interatomic Coulombic decay (ICD). This decay mechanism due to multiple…

Photoexcitation of van der Waals complexes can lead to several decay pathways depending on the nature of the potential energy surfaces. Upon excitation of a chromophore in a complex, ionization of its weakly bound neighbour via energy…

Chemical Physics · Physics 2022-01-14 Namitha Brijit Bejoy , Nitin. K Singh , Balanarayan Pananghat , G. Naresh Patwari

Interatomic Coulombic decay (ICD) processes play a crucial role in weakly bound complexes exposed to intense or high-energy radiation. Using large helium nanodroplets, we demonstrate that ICD is efficient even when the droplets are…

We report theory for time-resolved spectator resonant Interparticle Coulombic Decay (ICD) processes. Following excitation by a short extreme ultraviolet pulse, the spectrum of the resonant ICD electron develops. Strong-field ionization is…

Quantum Physics · Physics 2020-04-29 Elke Fasshauer , Lars Bojer Madsen

We implement an independent-atom and independent-electron model to investigate the collision systems of He$^{2+}$ and He$^{+}$ ion projectiles impinging on a neon dimer target. The dimer is set to be stationary at its equilibrium bond…

Atomic and Molecular Clusters · Physics 2025-05-13 Darij Starko , Tom Kirchner

Tremendous advances in laser pump-probe techniques open the door for the observation in real time of ultrafast \textit{electronic} processes. Particularly attractive is the visualization of interatomic processes where one can follow the…

Atomic and Molecular Clusters · Physics 2007-05-23 Alexander I. Kuleff , Lorenz S. Cederbaum

Interatomic Coulombic decay (ICD) is induced in helium (He) nanodroplets by photoexciting the n=2 excited state of He^+ using XUV synchrotron radiation. By recording multiple coincidence electron and ion images we find that ICD occurs in…

Atomic and Molecular Clusters · Physics 2017-07-24 M. Shcherbinin , A. C. LaForge , V. Sharma , M. Devetta , R. Richter , R. Moshammer , T. Pfeifer , M. Mudrich

We report the first observation of intermolecular Coulombic decay (ICD) in liquid water following inner-valence ionization. By combining a monochromatized table-top high-harmonic source with a liquid micro-jet, we recorded electron-electron…

Atomic and Molecular Clusters · Physics 2022-04-05 Pengju Zhang , Conaill Perry , Tran Trung Luu , Danylo Matselyukh , Hans Jakob Wörner

During the last 15 years a novel decay mechanism of excited atoms has been discovered and investigated. This so called ''Interatomic Coulombic Decay'' (ICD) involves the chemical environment of the electronically excited atom: the…

We report on electron removal calculations for 2.81 keV/amu Li$^{3+}$ and O$^{3+}$ ion collisions with neon dimers. The target is described as two independent neon atoms fixed at the dimer's equilibrium bond length, whose electrons are…

Atomic and Molecular Clusters · Physics 2021-01-04 Dyuman Bhattacharya , Tom Kirchner

The recent availability of intense and ultrashort extreme ultraviolet sources opens the possibility to investigate ultrafast electronic relaxation processes in matter in an unprecedented regime. In this work we report on the observation of…

The emission of an Auger electron is the predominant relaxation mechanism of core-vacant states in molecules composed of light nuclei. In this non-radiative decay process, one valence electron fills the core vacancy while a second valence…

Chemical Physics · Physics 2023-01-24 Florian Matz , Thomas-C. Jagau
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