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Intramolecular energy transport is generally responsible for chemical energy balance in molecular systems. The transport is fast and efficient if energy is transferred by optical phonons in periodic oligomers, but its efficiently is limited…

Chemical Physics · Physics 2024-06-11 Alexander L. Burin , Igor V. Rubtsov

We investigate ballistic vibrational energy transport through optical phonon band in oligomeric chains in the presence of decoherence. An exact solution is obtained for the excitation density in the space-time representation in the…

Chemical Physics · Physics 2015-05-20 Arkady A. Kurnosov , Igor V. Rubtsov , Alexander L. Burin

Understanding phonon transport at a molecular scale is fundamental to the development of high-performance thermoelectric materials for the conversion of waste heat into electricity. We have studied phonon and electron transport in alkane…

Mesoscale and Nanoscale Physics · Physics 2015-11-13 Hatef Sadeghi , Sara Sangtarash , Colin J. Lambert

The Dirac dispersion of graphene limits the phase space available for energy transport between electrons and acoustic phonons at temperatures above the Bloch-Grueneisen temperature. Consequently, energy transport can be dominated by…

Mesoscale and Nanoscale Physics · Physics 2014-06-18 Pauli Virtanen

The low temperature transport of electron, or vibrational or electronic exciton towards polymer chains turns out to be dramatically sensitive to its interaction with transverse acoustic vibrations. We show that this interaction leads to…

Mesoscale and Nanoscale Physics · Physics 2021-06-23 Alexei Boulatov , Alexander L. Burin

Properties of phonons - quanta of the crystal lattice vibrations - in graphene have attracted strong attention of the physics and engineering communities. Acoustic phonons are the main heat carriers in graphene near room temperature while…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 Denis L. Nika , Alexander A. Balandin

A time-dependent inelastic electron transport theory for strong electron-phonon interaction is established via the equations of motion method combined with the small polaron transformation. In this work, the dissipation via electron-phonon…

Mesoscale and Nanoscale Physics · Physics 2015-05-21 Yu Zhang , ChiYung Yam , GuanHua Chen

In a network of interacting quantum systems achieving fast coherent energy transfer is a challenging task. While quantum systems are susceptible to a wide range of environmental factors, in many physical settings their interactions with…

Quantum Physics · Physics 2014-05-09 James Lim , Mark Tame , Ki Hyuk Yee , Joong-Sung Lee , Jinhyoung Lee

The transport of sound and heat, in the form of phonons, can be limited by disorder-induced scattering. In electronic and optical settings the introduction of chiral transport, in which carrier propagation exhibits parity asymmetry, can…

Optics · Physics 2017-10-12 Seunghwi Kim , Xunnong Xu , Jacob M. Taylor , Gaurav Bahl

Bulk AlN possesses high thermal conductivity due to long phonon mean-free-paths, high group velocity, and long lifetimes. However, the thermal transport scenario becomes very different in a thin AlN film due to phonon-defect and…

Thermal conductivity of aligned polymer molecules can be exceptionally high along the alignment direction due to energy transport through strong covalent bonds. At the same time, it is highly sensitive to molecular conformation, varying by…

Chemical Physics · Physics 2026-04-29 Igor V. Parshin , Igor V. Rubtsov , Alexander L. Burin

Recent advances in cavity-optomechanics have now made it possible to use light not just as a passive measuring device of mechanical motion, but also to manipulate the motion of mechanical objects down to the level of individual quanta of…

Mesoscale and Nanoscale Physics · Physics 2023-08-17 Hengjiang Ren , Tirth Shah , Hannes Pfeifer , Christian Brendel , Vittorio Peano , Florian Marquardt , Oskar Painter

Electronic and thermal transport properties in two-dimensional (2D) semiconductors have been extensively investigated due to their potential to miniaturize transistors. Microscopically, electron-phonon interactions are considered the…

Mesoscale and Nanoscale Physics · Physics 2024-11-25 Yujie Quan , Bolin Liao

Non-reciprocal devices, with one-way transport properties, form a key component for isolating and controlling light in photonic systems. Optomechanical systems have emerged as a potential platform for optical non-reciprocity, due to ability…

Quantum Physics · Physics 2017-01-11 Xunnong Xu , Jacob M. Taylor

The concept of coherence is one of the fundamental phenomena in electronics and optics. In addition to electron and photon, phonon, is another important energy and information carrier in nature. Without any doubt, exploration of the phonon…

Mesoscale and Nanoscale Physics · Physics 2018-09-03 Guofeng Xie , Ding Ding , Gang Zhang

It is generally understood that Fourier's law does not describe ballistic phonon transport, which is important when the length of a material is similar to the phonon mean-free-path. Using an approach adapted from electron transport, we…

Mesoscale and Nanoscale Physics · Physics 2015-06-22 Jesse Maassen , Mark Lundstrom

Atomic mass and interatomic interaction are the two key quantities that significantly affect the heat conduction carried by phonons. Here, we study the effects of long-range (LR) interatomic interaction and mass-disorder on the phonon…

Mesoscale and Nanoscale Physics · Physics 2016-11-23 Hangbo Zhou , Gang Zhang , Jian-Sheng Wang , Yong-Wei Zhang

We use ultrafast x-ray diffraction to quantify the transport of energy in laser-excited nanoscale Au/Ni bilayers. Electron transport and efficient electron-phonon coupling in Ni convert the laser-deposited energy in the conduction electrons…

Mesoscale and Nanoscale Physics · Physics 2022-04-07 M. Herzog , A. von Reppert , J. -E. Pudell , C. Henkel , M. Kronseder , C. H. Back , A. Maznev , M. Bargheer

Time-domain femtosecond laser spectroscopic measurements of the ultrafast lattice dynamics in 2H-MoTe2 bulk crystals were carried out to understand the carrier-phonon interactions that govern electronic transport properties. An unusually…

The long carrier lifetime and defect tolerance in metal halide perovskites (MHPs) are major contributors to the superb performance of MHP optoelectronic devices. Large polarons were reported to be responsible for the long carrier lifetime.…

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