Related papers: Ultrafast simultaneous manipulation of multiple fe…
Ferroelectric and ferromagnetic materials possess spontaneous electric and magnetic order, respectively, which can be switched by the corresponding applied electric and magnetic fields. Multiferroics combine these properties in a single…
Selective excitation of coherent high-amplitude vibrations of atoms in a solid can induce exotic nonequilibrium states, in which the character of interactions between electronic, magnetic and lattice degrees of freedom is considerably…
Given the paucity of single phase multiferroic materials (with large ferromagnetic moment), composite systems seem an attractive solution in the quest to realize magnetoelectric cou-pling between ferromagnetic and ferroelectric order…
Multifunctionality as a paradigm requires materials exhibiting multiple superior properties. Integrating second-order optical nonlinearity and large bandgap with piezoelectricity could, for example, enable broadband, strain-tunable…
We use molecular dynamics simulations with machine-learned atomistic force fields to simulate photoexcitation of BaTiO3 by a femtosecond laser pulse whose photon energy exceeds the optical gap. We demonstrate selective displacive excitation…
In the iron pnictides, the strong sensitivity of the iron magnetic moment to the arsenic position suggests a significant relationship between phonons and magnetism. We measured the phonon dispersion of several branches in the high…
Strain engineering is widely used to manipulate the electronic and magnetic properties of complex materials. An attractive route to control magnetism with strain is provided by the piezomagnetic effect, whereby the staggered spin structure…
Using time resolved ultrafast spectroscopy, we have demonstrated that the far infrared (FIR) excitations in ferroelectric crystals may be modified through an arsenal of control techniques from the fields of guided waves, geometrical and…
Magnetic order parameters in altermagnets can couple to quantized lattice vibration via both piezomagnetic and magnetoelastic effects, leading to the renormalization of phonon dispersion. Here, we demonstrate photo-induced dynamic frequency…
We realize a nondegenerate parametric amplifier in an ultrahigh $Q$ mechanical membrane resonator and demonstrate two-mode thermomechanical noise squeezing. Our measurements are accurately described by a two-mode model that attributes this…
Controlling nonequilibrium responses in optically driven quantum materials is essential for advancing applications in energy conversion, ultrafast electronics, and quantum computation. Nonlinear optical spectroscopy serves as a powerful…
Ultrafast strengthening or quenching of the ferromagnetic order of semiconducting Eu1-xGdxO was achieved by resonant photoexcitation. The modification of the magnetic order is established within 3 ps as revealed by optical second harmonic…
We describe an ultrafast coherent control of the transient structural distortion arising from nonlinear phononics in ErFeO$_3$. Using density functional theory, we calculate the structural properties as input to an anharmonic phonon model…
A continuum approach to study magnetoelectric multiferroic $\mathrm{BiFeO}_3$ (BFO) is proposed. Our modeling effort marries the ferroelectric (FE) phase field method and micromagnetic simulations in order to describe the entire…
Tailored light excitation and nonlinear control of lattice vibrations have emerged as powerful strategies to manipulate the properties of quantum materials out of equilibrium. Generalizing the use of coherent phonon-phonon interactions to…
By comparing femtosecond laser pulse induced ferro- and antiferromagnetic dynamics in one and the same material - metallic dysprosium - we show both to behave fundamentally different. Antiferromagnetic order is considerably faster and much…
Coherent control with shaped ultrafast pulses is a powerful approach for steering nonlinear light-matter interactions. Previous studies in quantum control have shown that, beyond transform-limited pulses, those with antisymmetric spectral…
Materials exhibit various wave-like excitations, among which phonons (lattice vibrations) and magnons (oscillations in ferromagnetic ordering) hold significant promise for future nanoscale technologies. Exploring the interaction between…
We develop a theoretical model for polarization-selective phonon pumping induced by magnon-phonon coupling in a ferromagnetic/non-magnetic acoustic bilayer structure, focusing on the effects arising from a misalignment between the magnetic…
Solid-state elastic-wave phonons are a promising platform for a wide range of quantum information applications. An outstanding challenge and enabling capability in harnessing phonons for quantum information processing is achieving strong…