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Recently it was realized that the zigzag magnetic order in Kitaev materials can be stabilized by small negative off-diagonal interactions called the $\Gamma'$ terms. To fully understand the effect of the $\Gamma'$ interactions, we…

Strongly Correlated Electrons · Physics 2020-10-21 Jiucai Wang , Qirong Zhao , Xiaoqun Wang , Zheng-Xin Liu

In addition to the Kitaev ($K$) interaction, candidate Kitaev materials also possess Heisenberg ($J$) and off-diagonal symmetric ($\Gamma$) couplings. We investigate the quantum ($S = 1/2$) $K$-$J$-$\Gamma$ model on the honeycomb lattice by…

Strongly Correlated Electrons · Physics 2019-11-14 Jiucai Wang , B. Normand , Zheng-Xin Liu

Layered honeycomb magnets are of interest as potential realizations of the Kitaev quantum spin liquid (KQSL), a quantum state with long-range spin entanglement and an exactly solvable Hamiltonian. Conventional magnetically ordered states…

Strongly Correlated Electrons · Physics 2020-01-28 Ruidan Zhong , Tong Gao , Nai Phuan Ong , Robert J. Cava

Motivated by the three-dimensional structure of Kitaev materials we explore multilayer Kitaev models. The magnetic properties of a multilayer of an arbitrary number of Kitaev honeycomb layers stacked on top of each other coupled through a…

Strongly Correlated Electrons · Physics 2025-03-05 Jaime Merino , Arnaud Ralko

We explore the potential experimental realization of the mixed-spin Kitaev model in materials such as Zr$_{0.5}$Ru$_{0.5}$Cl$_3$, where spin-1/2 and spin-3/2 ions occupy distinct sublattices of a honeycomb lattice. By developing a…

Strongly Correlated Electrons · Physics 2025-05-09 Willian Natori , Yang Yang , Hui-Ke Jin , Johannes Knolle , Natalia B. Perkins

The search for Kitaev's quantum spin liquid (KQSL) state in real materials has recently expanded with the prediction that honeycomb lattices of divalent, high-spin cobalt ions could host the dominant bond-dependent exchange interactions…

Recent experiments reveal that the honeycomb ruthenium trichloride {\alpha}-RuCl3 is a prime candidate of the Kitaev quantum spin liquid (QSL). However, there is no theoretical model which can properly describe its experimental dynamical…

Strongly Correlated Electrons · Physics 2017-08-16 Y. S. Hou , H. J. Xiang , X. G. Gong

Co$^{2+}$ ions in an octahedral crystal field, stabilise a j$_{eff}$ = 1/2 ground state with an orbital degree of freedom and have been recently put forward for realising Kitaev interactions, a prediction we have tested by investigating…

We explore the phase diagram of the Kitaev-Heisenberg model with nearest neighbor interactions on the honeycomb lattice using the exact diagonalization of finite systems combined with the cluster mean field approximation, and supplemented…

Strongly Correlated Electrons · Physics 2017-02-01 Dorota Gotfryd , Juraj Rusnačko , Krzysztof Wohlfeld , George Jackeli , Jiří Chaloupka , Andrzej M. Oleś

The $S=1/2$ Kitaev honeycomb model has attracted significant attention as an exactly solvable example with a quantum spin liquid ground state. In a properly oriented external magnetic field, chiral Majorana edge modes associated with a…

Strongly Correlated Electrons · Physics 2022-03-23 Pedro M. Cônsoli , Eric C. Andrade

The Kitaev model, which hosts a quantum spin liquid (QSL) in the ground state, was originally defined on a two-dimensional honeycomb lattice, but can be straightforwardly extended to any tricoordinate lattices in any spatial dimensions. In…

Strongly Correlated Electrons · Physics 2023-05-29 Kiyu Fukui , Yasuyuki Kato , Yukitoshi Motome

We discuss the discovery by variational Monte Carlo (VMC) methods of a series of multinode quantum spin liquids (QSLs) in extended Kitaev models on the honeycomb lattice. Like the gapless Kitaev spin liquid with its two nodes at K and…

Strongly Correlated Electrons · Physics 2024-12-03 Jiucai Wang , B. Normand , Zheng-Xin Liu

Magnetic materials are composed of the simple building blocks of magnetic moments on a crystal lattice that interact via magnetic exchange. Yet from this simplicity emerges a remarkable diversity of magnetic states. Some reveal the deep…

Motivated by the largely unexplored domain of multi-polar ordered spin states in the Kitaev-Heisenberg (KH) systems we investigate the ground state dynamics of the spin-$\frac{1}{2}$ KH model, focusing on quadrupolar (QP) order in 2-leg…

Strongly Correlated Electrons · Physics 2025-03-28 Manodip Routh , Sayan Ghosh , Jeroen van den Brink , Satoshi Nishimoto , Manoranjan Kumar

The Kitaev honeycomb model plays a pivotal role in the quest for quantum spin liquids, in which fractional quasiparticles would provide applications in decoherence-free topological quantum computing. The key ingredient is the bond-dependent…

Strongly Correlated Electrons · Physics 2024-10-11 Seong-Hoon Jang , Yukitoshi Motome

We show that the topological Kitaev spin liquid on the honeycomb lattice is extremely fragile against the second-neighbor Kitaev coupling $K_2$, which has recently been shown to be the dominant perturbation away from the nearest-neighbor…

Strongly Correlated Electrons · Physics 2015-12-08 Ioannis Rousochatzakis , Johannes Reuther , Ronny Thomale , Stephan Rachel , N. B. Perkins

The pursuit of quantum spin liquid (QSL) in the Kitaev honeycomb magnets has drawn intensive attention recently. In particular, $\alpha$-RuCl$_3$ has been widely recognized as a promising candidate for the Kitaev QSL. Although the compound…

Strongly Correlated Electrons · Physics 2023-03-29 Han Li , Wei Li , Gang Su

Kitaev exchange, a new paradigm in quantum magnetism research, occurs for 90$^{\circ}$ metal-ligand-metal links, $t_{2g}^5$ transition ions, and sizable spin-orbit coupling. It is being studied in honeycomb compounds but also on triangular…

Strongly Correlated Electrons · Physics 2023-10-11 Pritam Bhattacharyya , Nikolay A. Bogdanov , Satoshi Nishimoto , Stephen D. Wilson , Liviu Hozoi

The layered honeycomb magnet $\alpha$-Li$_2$IrO$_3$ has been theoretically proposed as a candidate to display novel magnetic behaviour associated with Kitaev interactions between spin-orbit entangled $j_{\rm eff}=1/2$ magnetic moments on a…

Strongly Correlated Electrons · Physics 2017-02-17 S. C. Williams , R. D. Johnson , F. Freund , Sungkyun Choi , A. Jesche , I. Kimchi , S. Manni , A. Bombardi , P. Manuel , P. Gegenwart , R. Coldea

Quantum spin liquids (QSLs) represent exotic states of matter where quantum spins interact strongly yet evade long-range magnetic order down to absolute zero. Characterized by non-local quantum entanglement and resultant fractionalized…

Strongly Correlated Electrons · Physics 2025-12-05 Yuji Matsuda , Takasada Shibauchi , Hae-Young Kee
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