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We conduct first-principles theoretical studies to investigate the temperature-dependent phonon properties of orthorhombic SrZrO$_3$ (SZO) perovskite. Our calculations include the quasiharmonic approximation, in which we explored mode…

Materials Science · Physics 2023-09-06 P. K. Verma

Light-induced ferroelectricity in quantum paraelectrics is a new avenue of achieving dynamic stabilization of hidden orders in quantum materials. In this work, we explore the possibility of driving transient ferroelectric phase in the…

Materials Science · Physics 2023-04-05 Bing Cheng , Patrick L. Kramer , Zhi-Xun Shen , Matthias. C. Hoffmann

Emergent cooperative motions of individual degrees of freedom, i.e. collective excitations, govern the low-energy response of system ground states under external stimulations and play essential roles for understanding many-body phenomena in…

Terahertz (THz) spin waves or their quanta, magnons, can be efficiently excited by acoustic phonons because these excitations have similar wavevectors in the THz regime. THz acoustic phonons can be produced using photoacoustic phenomena but…

Mesoscale and Nanoscale Physics · Physics 2024-08-07 Shihao Zhuang , Xufeng Zhang , Yujie Zhu , Nian X. Sun , Chang-Beom Eom , Paul G. Evans , Jia-Mian Hu

Development of topological insulating phases in IV-VI compounds under dynamic lattice deformations is studied using first-principles methods. Unlike the static state of topological phases at equilibrium conditions, we show that non-trivial…

Materials Science · Physics 2015-09-30 Jinwoong Kim , Seung-Hoon Jhi

The long carrier lifetime and defect tolerance in metal halide perovskites (MHPs) are major contributors to the superb performance of MHP optoelectronic devices. Large polarons were reported to be responsible for the long carrier lifetime.…

Thermal runaway in lithium-ion batteries is governed by the poorly-understood initiation phase, where localised heating introduces instability. Here we identify the three key components that trigger thermal runaway, decreases in local…

The caged compound LaRu2Zn20 exhibits a structural transition at TS =150 K, whose driving mechanism remains elusive. We have investigated atomic dynamics by the measurements of specific heat C and inelastic X-ray scattering (IXS). The…

Strongly Correlated Electrons · Physics 2017-05-18 K. Wakiya , T. Onimaru , S. Tsutsui , K. T. Matsumoto , N. Nagasawa , A. Q. R. Baron , T. Hasegawa , N. Ogita , M. Udagawa , T. Takabatake

The lattice dynamics of members of the M2Mo6Se6 family of materials with guest ions M = K, Rb, Cs, In, and Tl has been studied using inelastic x-ray scattering and Raman spectroscopy at room temperature, as well as by ab-initio…

We investigate the effect of tuning the phonon energy on the correlation effects in models of electron-phonon interactions using DMFT. In the regime where itinerant electrons, instantaneous electron-phonon driven correlations and static…

Strongly Correlated Electrons · Physics 2015-05-13 J. P. Hague , N. d'Ambrumenil

In this work we analyze a particular setup with ultracold atoms trapped in state-dependent lattices. We show that any asymmetry in the contact interaction translates into one of two classes of correlated hopping. After deriving the…

Other Condensed Matter · Physics 2009-12-21 Maria Eckholt , Juan Jose Garcia-Ripoll

Many complex crystals show a flattening or even increasing lattice thermal conductivity at high temperatures, which deviates from the traditional 1/T decay trend given by conventional phonon theory. In this work, we predict the thermal…

Materials Science · Physics 2023-12-20 Janak Tiwari , Tianli Feng

Understanding spin-lattice coupling represents a key challenge in modern condensed matter physics, with crucial importance and implications for ultrafast and 2D-magnetism. The efficiency of angular momentum and energy transfer between spins…

Strong coupling of light to a collective spin excitation in antiferromagnets gives rise to hybrid modes called magnon-polaritons. They are highly promising for data manipulation and transfer at terahertz rates, much faster than in the case…

Here we report an ultrafast optical spectroscopic study of the nodal-line semimetal ZrSiTe. Our measurements reveal that, converse to other compounds of the family, the sudden injection of electronic excitations results in a strongly…

We present Raman and terahertz absorbance spectra of methylammonium lead halide single crystals (MAPbX3, X = I, Br, Cl) at temperatures between 80 and 370 K. These results show good agreement with density-functional-theory phonon…

Indium iodides, which adopt layered or molecular-crystal-like arrangements depending on composition, are expected to exhibit low lattice thermal conductivity because of their heavy constituent atoms and weak In-I bonding. In this work, we…

Materials Science · Physics 2026-01-06 Takuma Shiga , Yoshikazu Mizuguchi , Hiroshi Fujihisa

The temperature dependent Hall mobility data from La-doped SrTiO3 thin films has been analyzed and modeled considering various electron scattering mechanisms. We find that a ~6 meV transverse optical phonon (TO) deformation potential…

Mesoscale and Nanoscale Physics · Physics 2015-06-19 Amit Verma , Adam P. Kajdos , Tyler A. Cain , Susanne Stemmer , Debdeep Jena

Superconducting transition temperature $T_C$ of some of the cubic $\beta$-phase Mo$_{1-x}$Re$_x$ alloys with x > 0.10 is an order of magnitude higher than that in the elements Mo and Re. We investigate this rather enigmatic issue of the…

Intense, few-cycle pulses in the terahertz frequency range have strong potential for schemes of control over vibrational modes in solid-state materials in the electronic ground-state. Here we report an experiment using single cycle…

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