Related papers: Spin-orientation-resolved attosecond chronoscopy i…
The inhomogeneity of an electron spin ensemble as well as fluctuating environment acting upon individual spins drastically shorten the spin coherence time $T_2$ and hinder coherent spin manipulation. We show that this problem can be solved…
We consider the motion of electrons through a mesoscopic ring in the presence of spin-orbit interaction, Zeeman coupling, and magnetic flux. The coupling between the spin and the orbital degrees of freedom results in the geometric and the…
A new scheme for a double-slit experiment in the time domain is presented. Phase-stabilized few-cycle laser pulses open one to two windows (``slits'') of attosecond duration for photoionization. Fringes in the angle-resolved energy spectrum…
Multi-electron dynamics in atoms and molecules very often occur on sub- to few-femtosecond timescales. The available intensities of extreme-ultraviolet (XUV) attosecond pulses have previously only allowed the time-resolved investigation of…
We have calculated the resonant and nonresonant contributions to attosecond impulsive stimulated electronic Raman scattering (SERS) in regions of autoionizing transitions. Comparison with Multiconfiguration Time-Dependent Hartree-Fock…
This publication will deal with an explicit determination of the time evolution of the spin orientation axes and the evolution of the orbital phase in the case of circular orbits under next-to-leading order spin-orbit interactions. We…
Irradiating solids with ultrashort laser pulses is known to initiate femtosecond timescale magnetization dynamics. However, sub-femtosecond spin dynamics have not yet been observed or predicted. Here, we explore ultrafast light-driven spin…
We present the first numerical simulation of the time delay in the photoionization of the simplest diatomic molecule H$_2^+$ as observed by attosecond streaking. We show that the strong variation of the Eisenbud-Wigner-Smith time delay as a…
We used femtosecond optical spectroscopy to study ultrafast spin and orbital ordering dynamics in the antiferromagnetic Mott insulator $\alpha$-Sr$_2$CrO$_4$. This chromate system possesses multiple spin and orbital ordered phases, and…
We report measurements of energy-dependent attosecond photoionization delays between the two outer-most valence shells of N$_2$O and H$_2$O. The combination of single-shot signal referencing with the use of different metal foils to filter…
Attosecond metrology with linearly polarized light pulses is the basis of a highly successful research area. An even broader impact can be expected from a generalized metrology that covers two-dimensional polarization states, enabling…
A systematic method is presented for constructing increasingly precise sequences to refocus off-resonant spin evolution with severely limited control amplitude. Sequences obtained should be readily applicable to the case of electron spin…
We solve the three-dimensional time-dependent Schr\"{o}dinger equation for a few-cycle circularly polarized femtosecond laser pulse interacting with an oriented target exemplified by an Argon atom, initially in a $3\text{p}_{x}$ or…
A compact cryogenic Kerr microscope for operation in the small volume of high-field magnets is described. It is suited for measurements both in Voigt and Faraday configuration. Coupled with a pulsed laser source, the microscope is used to…
An exact analytical solution is derived for the wavefunction of an electron in a one-dimensional moving quantum dot in a nanowire, in the presence of time-dependent spin-orbit coupling. For cyclic evolutions we show that the spin of the…
We study laser-assisted photoionization by attosecond pulses using a time-independent formalism based on diagrammatic many-body perturbation theory. Our aim is to provide an ab inito route to the "delays" for this above-threshold ionization…
We employ the recently developed multi-photon R-matrix method for molecular above-threshold photoionization to obtain second-order ionization amplitudes that govern the interference in RABITT experiments. This allows us to extract RABITT…
In our Solar system, spin-orbit coupling is a common phenomenon in binary asteroid systems, where the mutual orbits are no longer invariant due to exchange of angular momentum between translation and rotation. In this work, dynamical…
Electronic orderings of charges, orbitals and spins are observed in many strongly correlated electron materials, and revealing their dynamics is a critical step toward understanding the underlying physics of important emergent phenomena.…
$TbMn_{6}Sn_{6}$ is a ferrimagnetic material which exhibits a highly unusual phase transition near room temperature where spins remain collinear while the total magnetic moment rotates from out-of-plane to in-plane. The mechanisms…