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The participation of oxygen or other anionic species in redox activities in cathode materials for lithium and sodium-ion battery systems is known to play a role in governing the useful capacity of these batteries. Directly probing anionic…

Materials Science · Physics 2024-08-20 M. Hussein N. Assadi , Dorian A. H. Hanaor

Tungsten (W) is considered a leading candidate for structural and functional materials in future fusion energy devices. The most attractive properties of tungsten for magnetic and inertial fusion energy reactors are its high melting point,…

Materials Science · Physics 2024-10-15 Yichen Qian , Mark R. Gilbert , Lucile Dezerald , Duc Nguyen-Manh , David Cereceda

The spin, charge, and lattice degrees of freedom and their interplay in high entropy oxides were intensively investigated in recent years. However, how the orbital degree of freedom is affected by the extreme disorder in high entropy oxides…

Materials Science · Physics 2024-01-17 Jiaqiang Yan , Abinash Kumar , Miaofang Chi , Matthew Brahlek , Thomas Z Ward , Michael McGuire

We study the electronic and structural properties of the low-temperature ordered phase of hydrogen-bonded molecular conductors, $\kappa$-D$_3$(Cat-EDT-TTF)$_2$ and its selenium-substituted analog $\kappa$-D$_3$(Cat-EDT-ST)$_2$, by means of…

Strongly Correlated Electrons · Physics 2020-01-17 Takao Tsumuraya , Hitoshi Seo , Tsuyoshi Miyazaki

LixTMO2 (TM=Ni, Co, Mn) forms an important family of cathode materials for Li-ion batteries, whose performance is strongly governed by Li composition-dependent crystal structure and phase stability. Here, we use LixCoO2 (LCO) as a model…

Computational Engineering, Finance, and Science · Computer Science 2023-02-20 G. H. Teichert , S. Das , M. Faghih Shojaei , J. Holber , T. Mueller , L. Hung , V. Gavini , K. Garikipati

The design of novel cathode materials for Li-ion batteries would greatly benefit from accurate first-principles predictions of structural, electronic, and magnetic properties as well as intercalation voltages in compounds containing…

Materials Science · Physics 2022-11-03 Iurii Timrov , Francesco Aquilante , Matteo Cococcioni , Nicola Marzari

A low-order nonconforming finite element discretization of a smooth de Rham complex starting from the $H^2$ space in three dimensions is proposed, involving an $H^2$-nonconforming finite element space, a new tangentially continuous…

Numerical Analysis · Mathematics 2025-12-05 Xuewei Cui , Xuehai Huang

Recent research in multi-principal element alloys (MPEAs) has increasingly focused on the exploration and exploitation of short-range order (SRO) to enhance material performance. However, the understanding of SRO formation and the precise…

In Lithium ion batteries (LIBs), proper design of cathode materials influences its intercalation behavior, overall cost, structural stability, and its impact on environment. At present, the most common type of cathode materials, NCA , has…

Materials Science · Physics 2018-04-03 Kamalika Ghatak , Hemant Kumar , Siva Nadimpalli , Dibakar Datta

This article reviews the development of cathode materials for secondary lithium ion batteries since its inception with the introduction of lithium cobalt oxide in early 1980s. The time has passed and numerous cathode materials are designed…

Materials Science · Physics 2021-09-07 Ambesh Dixit

Metal-oxide-metal devices based on amorphous VOx are shown to exhibit one of two distinct negative differential resistance (NDR) characteristics depending on the maximum current employed for electroforming. For low compliance currents they…

Applied Physics · Physics 2021-02-03 Sanjoy Kumar Nandi , Sujan Kumar Das , Caleb Estherby , Angus Gentle , Robert G. Elliman

Contradictory theoretical results for oxygen vacancies in SrTiO$_3$ (STO) were often related to the peculiar properties of STO, which is a $d^0$ transition metal oxide with mixed ionic-covalent bonding. Here, we apply, for the first time,…

Materials Science · Physics 2020-07-01 Chiara Ricca , Iurii Timrov , Matteo Cococcioni , Nicola Marzari , Ulrich Aschauer

Challenges associated with in-service mechanical degradation of Li-ion battery cathodes has prompted a transition from polycrystalline to single crystal cathode materials. Whilst for single crystal materials, dislocation-assisted crack…

Materials Science · Physics 2023-08-15 Siyang Wang , Zonghao Shen , Aigerim Omirkhan , Oriol Gavalda-Diaz , Mary P. Ryan , Finn Giuliani

Recent experiments on Kagome metals AV$_3$Sb$_5$ (A=Cs,Rb,K) indicated spontaneous time-reversal symmetry breaking in the charge density wave state in the absence of static magnetization. The loop current order (LCO) is proposed as its…

Strongly Correlated Electrons · Physics 2024-04-08 Heqiu Li , Yong Baek Kim , Hae-Young Kee

In recent years, the Na-ion SuperIonic CONductor (NASICON) based polyanionics are considered the pertinent cathode materials in sodium-ion batteries due to their 3D open framework, which can accommodate a wide range of Na content and can…

Chemical Physics · Physics 2024-05-10 Simranjot K. Sapra , Jeng-Kuei Chang , Rajendra S. Dhaka

Recently, considerable efforts have been made on research and improvement for Ni-rich lithium-ion batteries to meet the demand from vehicles and grid-level large-scale energy storage. Development of next-generation high-performance…

Resonant-magnetic x-ray scattering (RMXS) near the vanadium $L_{2,3}$-absorption edges has been used to investigate the low temperature magnetic structure of high quality \bvs\ single crystals. Below $T_N$ = 31 K, the strong resonance…

Strongly Correlated Electrons · Physics 2011-04-27 Ph. Leininger , V. Ilakovac , Y. Joly , E. Schierle , E. Weschke , O. Bunau , H. Berger , J. -P. Pouget , P. Foury-Leylekian

Charge ordering of V4+ and V5+ in NaV2O5 has been studied by an X-ray diffraction technique using anomalous scattering near a vanadium K-absorption edge to critically enhance a contrast between the two ions. A dramatic energy dependence of…

Strongly Correlated Electrons · Physics 2009-10-31 H. Nakao , K. Ohwada , N. Takesue , Y. Fujii , M. Isobe , Y. Ueda , M. v. Zimmermann , J. P. Hill , D. Gibbs , J. C. Woicik , I. Koyama , Y. Murakami

We discuss electronic and magnetic properties of Na$_x$Fe$_{1/2}$Mn$_{1/2}$O$_2$, a promising Na-ion battery cathode material. Using x-ray Compton scattering, SQUID magnetometry, and density-functional-theory based modeling, we probe how…

The cathode properties of Na2MTiO4 (M: transition-metal element) are investigated by means of density-functional-theory calculations. The stability between the layered structure and the disordered structure are focused in comparison with…

Materials Science · Physics 2022-02-23 Kunihiko Yamauchi , Hiroyoshi Momida , Tamio Oguchi
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