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We report on a comprehensive experimental and theoretical study of optical third harmonic generation (THG) on the exciton-polariton resonances in the zinc-blende semiconductors GaAs, CdTe, and ZnSe subject to an external magnetic field,…

Grain boundary engineering via dopant segregation can dramatically change the properties of a material. For metallic systems, most current studies concerning interfacial segregation and subsequent transitions of grain boundary structure are…

Materials Science · Physics 2018-12-26 Yang Hu , Timothy J. Rupert

Fe$_{3}$Ga$_{4}$ displays a complex magnetic phase diagram that is sensitive and tunable with both electronic and crystallographic structure changes. In order to explore this tunability, vanadium-doped (Fe$_{1-x}$V$_{x}$)$_{3}$Ga$_{4}$ has…

Dielectric metasurfaces provide a unique platform for efficient harmonic generation and optical wavefront manipulation at the nanoscale. While several approaches are available for performing wavefront shaping, the one exploiting geometric…

We observe strongly anisotropic third-harmonic generation mediated by resonant sum-frequency driving of Raman phonons with THz light, extending light-induced dual control of structural and optical properties in solids. Either strong…

Optics · Physics 2024-05-03 Jiaoyang Zheng , Guru Khalsa , Jeffrey Moses

In this work, nonlinear optical properties of Na: ZnO thin films (Na: ZnO) have been experimentally elaborated. The principal possibility to operate the nonlinear optical features using external laser beams is shown. The Na: ZnO films were…

All-solid-state lithium batteries promise significant improvements in energy density and safety over traditional liquid electrolyte batteries. The Al-doped AlxLi7-3xLa3Zr2O12 (LLZO) solid-state electrolyte shows excellent potential given…

We obtain the non-collinear ground states of a triangular-lattice antiferromagnet with exchange interactions up to third nearest neighbors as a function of the single-ion anisotropy $D$. At a critical value of $D$, the collinear $\uudd $…

Materials Science · Physics 2015-05-14 Randy S. Fishman , Satoshi Okamoto

Classical nonlocality in conducting nanostructures has been shown to dramatically alter the linear optical response, by placing a fundamental limit on the maximum field enhancement that can be achieved. This limit directly extends to all…

Mesoscale and Nanoscale Physics · Physics 2013-11-14 Cristian Ciracì , Michael Scalora , David R. Smith

The spin-dependent electronic structures of aluminum-(Al) doped zigzag silicene nanoribbons (ZSiNRs) are investigated by first-principles calculations. When ZSiNRs are substitutionally doped by a single Al atom on different sites in every…

Materials Science · Physics 2014-09-01 Y. J. Dong , X. F. Wang , P. Vasilopoulos , M. X. Zhai , X. M. Wu

Notwithstanding its long history, the study of nonlinear optics from metal surfaces is still an active field of research. For instance, in view of the presence of absorption questions remain concerning the possibility of significantly…

A nonequilibrium Green's function technique combined with density functional theory is used to study the spin-dependent electronic band structure and transport properties of zigzag silicene nanoribbons (ZSiNRs) doped with aluminum (Al) or…

Materials Science · Physics 2014-09-01 J. Chen , X. F. Wang , P. Vasilopoulos , A. B. Chen , J. C. Wu

Nonlinear metasurfaces have become prominent tools for controlling and engineering light at the nanoscale. Usually, the polarization of the total generated third harmonic is studied. However, diffraction orders may present different…

We have studied the dynamic effect of nonlinearity on lasing in disordered medium. The third-order nonlinearity not only changes the frequency and size of lasing modes, but also modifies the laser emission intensity and laser pulse width.…

Disordered Systems and Neural Networks · Physics 2009-11-10 B. Liu , A. Yamilov , Y. Ling , J. Y. Xu , H. Cao

The effective linear and third-order nonlinear susceptibility of graded metallic films with weak nonlinearity have been investigated. Due to the simple geometry, we were able to derive exactly the local field inside the graded structures…

Materials Science · Physics 2007-05-23 J. P. Huang , K. W. Yu

We compute from first principles the infrared dispersion of the nonlinear susceptibility $\chi^{(2)}$ in zincblende semiconductors. At terahertz frequencies the nonlinear susceptibility depends not only on the purely electronic response…

Materials Science · Physics 2009-12-17 Eric Roman , Jonathan R. Yates , Marek Veithen , David Vanderbilt , Ivo Souza

We study nonlinear effects in two-dimensional photonic metasurfaces supporting topologically-protected helical edge states at the nanoscale. We observe strong third-harmonic generation mediated by optical nonlinearities boosted by…

A series of MnxZn1-xO (x=0.03, 0.05) nanostructures have been grown via the solution based chemical spray pyrolysis technique. Electron beam induced modifications on structural, linear and nonlinear optical and surface morphological…

Rigorous electrodynamical simulations based on the nonlinear Drude model are performed to investigate the influence of strong coupling on high harmonic generation by periodic metal gratings. It is shown that a thin dispersive material with…

Mesoscale and Nanoscale Physics · Physics 2019-08-13 Elena Drobnyh , Ruth Pachter , Maxim Sukharev

The non-uniform ground state of the two-dimensional three-band Hubbard model for the oxide high-Tc superconductors is investigated using a variational Monte Carlo method. We examine the effect produced by holes doped into the…

Strongly Correlated Electrons · Physics 2009-11-07 Takashi Yanagisawa , Soh Koike , Mitake Miyazaki , Kunihiko Yamaji