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We present a novel theory and implementation for computing coupled electronic and quantal nuclear subsystems on a single potential energy surface, moving beyond the standard Born-Oppenheimer (BO) separation of nuclei and electrons. We…

Chemical Physics · Physics 2021-11-15 Ziyong Chen , Jun Yang

Electron captures on nuclei play an important role in the dynamics of the collapsing core of a massive star that leads to a supernova explosion. Recent calculations of these capture rates were based on microscopic models which account for…

Nuclear Theory · Physics 2010-11-23 A. Juodagalvis , K. Langanke , W. R. Hix , G. Martínez-Pinedo , J. M. Sampaio

Within the Dirac-Brueckner-Hartree-Fock approach, using the Bonn potentials, we investigate the properties of dense, asymmetric nuclear matter and apply it to neutron stars. In the actual calculations of the nucleon self-energies and the…

Nuclear Theory · Physics 2013-10-02 Tetsuya Katayama , Koichi Saito

The treatment of atomic anions with Kohn-Sham density functional theory (DFT) has long been controversial since the highest occupied molecular orbital (HOMO) energy, $E_{HOMO}$, is often calculated to be positive with most approximate…

Chemical Physics · Physics 2019-03-20 Lindsey N. Anderson , M. Belén Oviedo , Bryan M. Wong

X-ray photoelectron spectroscopy (XPS) measures electron removal energies, providing direct access to core and valence electron binding energies, hence probing the electronic structure. In this work, we benchmark for the first time the ab…

Other Condensed Matter · Physics 2023-10-11 Iskander Mukatayev , Benoît Sklénard , Valerio Olevano , Jing Li

A self-consistent calculation scheme for correlated electron systems is created based on the density-functional theory (DFT). Our scheme is a multi-reference DFT (MR-DFT) calculation in which the electron charge density is reproduced by an…

Strongly Correlated Electrons · Physics 2009-11-13 Koichi Kusakabe , Naoshi Suzuki , Shusuke Yamanaka , Kizashi Yamaguchi

We propose a new approximation for the cyclo-synchrotron emissivity of a single electron. In the second part of this work, we discuss a simple application for our approximation, and investigate the heating of electrons through the…

Astrophysics · Physics 2009-11-11 K. Katarzynski , G. Ghisellini , R. Svensson , J. Gracia

Fully numerical mesh solutions of 2D and 3D quantum equations of Schroedinger and Hartree-Fock type allow us to work with wavefunctions which possess a very flexible geometry. This flexibility is especially important for calculations of…

Atomic Physics · Physics 2007-05-23 Mikhail V. Ivanov

Fully numerical mesh solutions of 2D quantum equations of Schroedinger and Hartree-Fock type allow us to work with wavefunctions which possess a very flexible geometry. This flexibility is especially important for calculations of atoms and…

Atomic Physics · Physics 2015-06-26 Mikhail V. Ivanov , Peter Schmelcher

We introduce and demonstrate a new approach to measuring coherent electron wave packets using high-harmonic spectroscopy. By preparing a molecule in a coherent superposition of electronic states, we show that electronic coherence opens…

Chemical Physics · Physics 2014-07-09 P. M. Kraus , S. B. Zhang , A. Gijsbertsen , R. R. Lucchese , N. Rohringer , H. J. Wörner

Magnetic form factors corresponding to elastic electron scattering from odd-A nuclei are presented. The calculations are carried out in plane-wave Born approximation. The one-body properties are obtained in a deformed self-consistent…

Electron capture rates on neutron-rich nuclei (A>65) were calculated within the Random Phase Approximation with partial number formalism, including allowed and forbidden transitions. The partial occupation numbers were provided as a…

Nuclear Theory · Physics 2015-06-26 J. M. Sampaio , K. Langanke , G. Martinez-Pinedo , E. Kolbe , D. J. Dean

For solar conditions, we numerically integrate the density matrix equation for a thermal electron in the field of a Be-7 ion and other plasma ions and smeared-out electrons. Our results are in agreement with previous calculations that are…

Astrophysics · Physics 2009-10-30 Andrei V. Gruzinov , John N. Bahcall

Three decades ago, the measurement of the electron neutrino mass in atomic electron capture (EC) experiments was scrutinized in its two variants: single EC and neutrino-less double EC. For certain isotopes an atomic resonance enormously…

High Energy Physics - Phenomenology · Physics 2013-05-22 A. De Rújula

The electron-to-nucleon ratio or electron fraction is a key parameter in many astrophysical studies. Its value is determined by weak-interaction rates that are based on theoretical calculations subject to several nuclear physics…

Solar and Stellar Astrophysics · Physics 2010-12-15 A. Arcones , G. Martinez-Pinedo , L. F. Roberts , S. E. Woosley

We present a method which computes many-electron energies and eigenfunctions by a full configuration interaction which uses a basis of atomistic tight-binding wave functions. This approach captures electron correlation as well as atomistic…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 Erik Nielsen , Rajib Rahman , Richard P. Muller

The determination of the electron neutrino mass by electron capture in $^{163}$Ho relies on a precise understanding of the deexcitation of a core hole after an electron capture event. We here present an \textit{ab intio} calculation of the…

Atomic Physics · Physics 2018-06-06 M. Braß , C. Enss , L. Gastaldo , M. W. Haverkort

Dielectronic recombination resonance strengths, energy-differential cross sections, and recombination rate coefficients are calculated fully relativistically for Fe$^{2+}$ ions. The ground-state and resonance energies are determined using…

Atomic Physics · Physics 2025-04-03 S. Singh , Z. Harman

The alignment of nuclear states resonantly formed in nuclear excitation by electron capture (NEEC) is studied by means of a density matrix technique. The vibrational excitations of the nucleus are described by a collective model and the…

Atomic Physics · Physics 2008-11-26 Adriana Pálffy , Zoltán Harman , Andrey Surzhykov , Ulrich D. Jentschura

An electron density functional approach for the calculation of the nuclear multipole moments is presented. The electronic matrix elements entering the experimentally observed hyperfine electron-nucleus interaction constants in atoms are…

Nuclear Theory · Physics 2007-05-23 R. L. Pavlov , P. P. Raychev , V. P. Garistov , M. Dimitrova-Ivanovich , J. Maruani