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An intriguingly complex phase diagram of Na-doped SrFe2As2 is uncovered using high-resolution thermal-expansion, magnetization and heat-capacity measurements. The detailed temperature dependence of the orthorhombic distortion and the…

Superconductivity · Physics 2019-10-01 L. Wang , M. He , D. D. Scherer , F. Hardy , P. Schweiss , T. Wolf , M. Merz , B. M. Andersen , C. Meingast

We study the effects of electron-electron interactions and hole doping on the electronic structure of Cu-doped NaFeAs using the density functional theory plus dynamical mean-field theory (DFT+DMFT) method. In particular, we employ an…

Strongly Correlated Electrons · Physics 2021-04-14 S. L. Skornyakov , V. I. Anisimov , I. Leonov

High pressure in-situ synchrotron X-ray diffraction experiments were performed on Ag2Te up to 42.6 GPa at room temperature and four phases were identified. Phase I ({\beta}-Ag2Te) transformed into phase II at 2.4 GPa, and phase III and…

Materials Science · Physics 2015-05-01 Zhao Zhao , Shibing Wang , Haijun Zhang , Wendy L. Mao

The phase diagram of Al-Li-Cu system in the Al-rich region was determined by means of first-principles calculations and statistical mechanics. The mixing enthalpies of many configurations for different lattices in the whole Al-Li-Cu system…

Materials Science · Physics 2022-06-29 S. Liu , J. S. Wróbel , J. LLorca

The effect of Cu substitution on the stability of the CuMnAs tetragonal phase was studied both experimentally and by ab initio calculations. Polycrystalline samples with various compositions Cu$_{1+x}$Mn$_{1-x}$As $(x = 0 - 0.5)$ were…

We report a computational survey of chemical doping of silver(II) fluoride, an oxocuprate analog. We find that the ground-state solutions exhibit strong tendency for localization of defects and for phase separation. The additional…

Materials Science · Physics 2021-01-20 Adam Grzelak , Mariana Derzsi , Wojciech Grochala

The resistive response of Ba(Fe$_{1-x}$Co$_{x}$)$_{2}$As$_{2}$ to AC mechanical deformation is considered in the multi-domain state. This resistance change depends both upon the anelastic relaxation of domain walls and upon the relation…

Strongly Correlated Electrons · Physics 2019-03-13 Alexander T. Hristov , Matthias S. Ikeda , Johanna C. Palmstrom , Ian R. Fisher

The influence of Fe content on the three-dimensional (3D) morphology of Fe-rich intermetallic phases (Fe phases), Al2Cu, and pores and mechanical properties of cast Al-5.0Cu-0.6Mn alloys with 0.5 and 1.0 wt. % Fe are characterized using…

Materials Science · Physics 2018-05-04 Yuliang Zhao , Zhi Wang , Chun Zhang , Weiwen Zhang

We report anisotropic dc magnetic susceptibility $\chi(T)$, electrical resistivity $\rho(T)$, and heat capacity $C(T)$ measurements on the single crystals of CaFe$_{2-x}$Co$_x$As$_2$ for $x$ = 0 and 0.06. Large sized single crystals were…

Superconductivity · Physics 2009-11-13 Neeraj Kumar , R. Nagalakshmi , R. Kulkarni , P. L. Paulose , A. K. Nigam , S. K. Dhar , A. Thamizhavel

The anisotropic electronic structure responsible for the antiferromagnetic transition in CeRu$_2$Al$_{10}$ at the unusually high temperature of $T_0$ = 28 K was studied using optical conductivity spectra, Ce 3d X-ray photoemission spectra,…

First principles density functional theory calculations within the GGA+U approximation were performed for LiMn$_{1-x}$M$_x$O$_{2}$, a candidate cathode material for lithium-ion batteries, with ($x=0.25$, M=Ni, Fe, Co, Mg), to investigate…

Materials Science · Physics 2008-07-01 N. N. Shukla , S. Shukla , R. Prasad , R. Benedek

AlFe$_2$B$_2$, a ternary transition metal boride doped with Ag, Ni, Sb, Ga, and Ge was investigated for the phase constituents, microstructure, and thermoelectric properties. The parent compound with 20\% excess Al (Al$_{1.2}$Fe$_2$B$_2$)…

Materials Science · Physics 2025-07-01 D. Sivaprahasam , R. Preyadarshini , Ashutosh Kumar

A comparative computational study of stability of candidate structures for an as yet unknown silver dichloride AgCl2 is presented. It is found that all considered candidates have a negative enthalpy of formation, but are unstable towards…

Materials Science · Physics 2022-01-25 A. Grzelak , W. Grochala

Systematic measurements of the resistivity, heat capacity, susceptibility and Hall coefficient are presented for single crystal samples of the electron-doped superconductor Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$. These data delineate an $x-T$ phase…

Superconductivity · Physics 2009-05-02 Jiun-Haw Chu , James G. Analytis , Chris Kucharczyk , Ian R. Fisher

We have prepared samples of nominal type Ba(8)Cu(x)Ge(46-x) by induction melting and solid state reaction. Analysis shows that these materials form type-I clathrates, with copper content between x = 4.9 and 5.3, nearly independent of the…

Materials Science · Physics 2009-11-07 Yang Li , Ji Chi , Weiping Gou , Sameer Khandekar , Joseph H. Ross

In order to improve the hydrogen storage properties of calcium hydride (CaH2), we have tuned its thermodynamical properties through fluorination. Using ab-initio total energy calculations based on density functional theory, the structural…

Materials Science · Physics 2017-06-07 R. Varunaa , P. Ravindran

We have grown single crystal samples of Co substituted CaFe2As2 using an FeAs flux and systematically studied the effects of annealing/quenching temperature on the physical properties of these samples. Whereas the as-grown samples (quenched…

Superconductivity · Physics 2015-06-04 S. Ran , S. L. Bud'ko , W. E. Straszheim , J. Soh , M. G. Kim , A. Kreyssig , A. I. Goldman , P. C. Canfield

Single crystals of Ca1-xLaxFe2As2 for x ranging from 0 to 0.25 have been grown and characterized by structural, transport and magnetic measurements. Coexistence of two superconducting phases is observed, in which the low superconducting…

Superconductivity · Physics 2013-10-21 Y. Sun , W. Zhou , L. J. Cui , J. C. Zhuang , Y. Ding , F. F. Yuan , J. Bai , Z. X. Shi

A Neutron Powder Diffraction (NPD) experiment has been performed to investigate the structural phase transition and magnetic order in CaFe1-xCoxAsF superconductor compounds (x = 0, 0.06, 0.12). The parent compound CaFeAsF undergoes a…

Superconductivity · Physics 2009-02-24 Y. Xiao , Y. Su , R. Mittal , T. Chatterji , T. Hansen , C. M. N. Kumar , S. Matsuishi , H. Hosono , Th. Brueckel

Single phase, sol-gel prepared Cu1-xFexO (0<x<0.125) are characterized in terms of structural, electronic and magnetic properties. Using dielectric and magnetic studies we investigate the coupling of electron and spin. The electrical…