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Numerous experiments on pyrochlore oxides Pr$_2$(Zr, Sn, Hf, Ir)$_2$O$_7$ with non-Kramers Pr$^{3+}$ ions suggest that they support a quantum spin liquid (QSL) ground state, but the precise nature of the QSL remains unclear. Quantum spin…

Strongly Correlated Electrons · Physics 2025-12-15 Tony An , Félix Desrochers , Yong Baek Kim

Motivated by recent experiments on $\alpha$-RuCl$_3$, we investigate a possible quantum spin liquid ground state of the honeycomb-lattice spin model with bond-dependent interactions. We consider the $K-\Gamma$ model, where $K$ and $\Gamma$…

Strongly Correlated Electrons · Physics 2018-02-15 Matthias Gohlke , Gideon Wachtel , Youhei Yamaji , Frank Pollmann , Yong Baek Kim

Frustration in magnetic interactions can give rise to disordered ground states with subtle and beautiful properties. The spin ices Ho2Ti2O7 and Dy2Ti2O7 exemplify this phenomenon, displaying a classical spin liquid state, with…

Strongly Correlated Electrons · Physics 2017-12-11 Mathieu Taillefumier , Owen Benton , Han Yan , L. D. C. Jaubert , Nic Shannon

We report detailed inelastic neutron scattering measurements on single crystals of the frustrated two-leg ladder BiCu2PO6, whose ground state is described as a spin liquid phase with no long-range order down to 6 K. Two branches of steeply…

Strongly Correlated Electrons · Physics 2013-08-09 K. W. Plumb , Zahra Yamani , M. Matsuda , G. J. Shu , B. Koteswararao , F. C. Chou , Young-June Kim

Investigation of materials that exhibit quantum phase transition provides valuable insights into fundamental problems in physics. We present neutron scattering under pressure in a triangular-lattice antiferromagnet which has a quantum…

Neutron scattering experiments on a polycrystalline sample of the frustrated pyrochlore magnet Tb2Ti2O7, which does not show any magnetic order down to 50 mK, have revealed that it shows condensation behavior below 0.4 K from a thermally…

Disordered Systems and Neural Networks · Physics 2011-12-13 Hiroshi Takatsu , Hiroaki Kadowaki , Taku J. Sato , Jeffrey W. Lynn , Yoshikazu Tabata , Teruo Yamazaki , Kazuyuki Matsuhira

The search of quantum spin liquid (QSL), an exotic magnetic state with strongly-fluctuating and highly-entangled spins down to zero temperature, is a main theme in current condensed matter physics. However, there is no smoking-gun evidence…

Strongly Correlated Electrons · Physics 2023-10-27 Z. H. Zhu , B. L. Pan , L. P. Nie , J. M. Ni , Y. X. Yang , C. S. Chen , Y. Y. Huang , E. J. Cheng , Y. J. Yu , A. D. Hillier , X. H. Chen , T. Wu , Y. Zhou , S. Y. Li , L. Shu

Quantum spin liquids (QSLs) form an extremely unusual magnetic state in which the spins are highly correlated and fluctuate coherently down to the lowest temperatures, but without symmetry breaking and without the formation of any static…

The tetratrillium lattice has recently been proposed as responsible for the dynamical properties observed in the $S=1$ langbeinite compound K$_2$Ni$_2$(SO$_4$)$_3$. Here, we study in detail the classical spin liquid properties of this…

Strongly Correlated Electrons · Physics 2025-11-14 Matías G. Gonzalez , Johannes Reuther

The layered triangular lattice owing to $1:2$ order of $B$ and $B'$ sites in the triple perovskite $A_3 B B'_2$O$_9$ family provides an enticing domain for exploring the complex phenomena of quantum spin liquids (QSLs). We report a…

Strongly Correlated Electrons · Physics 2024-08-07 K. Bhattacharya , S. Mohanty , A. D. Hillier , M. T. F. Telling , R. Nath , M. Majumder

One main theme in current condensed matter physics is the search of quantum spin liquid (QSL), an exotic magnetic state with strongly-fluctuating and highly-entangled spins down to zero temperature without static order. However, there is no…

Strongly Correlated Electrons · Physics 2023-01-10 Chengpeng Tu , Dongzhe Dai , Xu Zhang , Chengcheng Zhao , Xiaobo Jin , Bin Gao , Tong Chen , Pengcheng Dai , Shiyan Li

Collective motions in strongly interacting magnets involve many spins and are often described in terms of integer-spin excitations. However, in certain cases, the collective motion can behave as if these integer excitations break apart into…

Quantum spin liquids (QSLs) host exotic fractionalized magnetic and gauge-field excitations whose microscopic origins and experimental verification remain frustratingly elusive. In the absence of static magnetic order, the spin excitation…

Strongly Correlated Electrons · Physics 2026-03-31 Jiahang Hu , Runze Chi , Yibin Guo , B. Normand , Hai-Jun Liao , T. Xiang

Inelastic neutron experiments on the classical triangular-lattice geometrically frustrated antiferromagnet h-YMnO$_3$ reveal diffuse, gapless magnetic excitations present both below and far above the ordering temperature, $T_N$. The…

The mineral malachite, Cu2(OD)2CO3, has a quantum spin-liquid ground state and no long-range magnetic order down to at least T=0.4 K. Inelastic neutron scattering measurements show that the excitation spectrum consists of dispersive gapped…

Strongly Correlated Electrons · Physics 2015-03-05 E. Canevet , B. Fak , R. K. Kremer , J. H. Chun , M. Enderle , E. E. Gordon , J. L. Bettis , M. -H. Whangbo , J. W. Taylor , D. T. Adroja

To reveal the nature of elementary excitations in a quantum spin liquid (QSL), we measured low temperature thermal conductivity and specific heat of 1T-TaS$_2$, a QSL candidate material with frustrated triangular lattice of spin-1/2. The…

Strongly Correlated Electrons · Physics 2020-02-05 H. Murayama , Y. Sato , X. Z. Xing , T. Taniguchi , S. Kasahara , Y. Kasahara , M. Yoshida , Y. Iwasa , Y. Matsuda

Quantum fluctuations are expected to lead to highly entangled spin-liquid states in certain two-dimensional spin-1/2 compounds. We have synthesized and measured thermodynamic properties and muon spin relaxation rates in the copper-based…

A small number of superconductors are believed to exhibit intrinsic spin triplet pairing, and they are often discussed in terms of a simple, $^3$He-like picture where ferromagnetic spin fluctuations provide the "glue". However, in some…

Superconductivity · Physics 2022-04-08 Andreas Kreisel , Yundi Quan , P. J. Hirschfeld

Conventional crystalline magnets are characterized by symmetry breaking and normal modes of excitation called magnons with quantized angular momentum $\hbar$. Neutron scattering correspondingly features extra magnetic Bragg diffraction at…

Strongly Correlated Electrons · Physics 2018-10-31 K. W. Plumb , Hitesh J. Changlani , A. Scheie , Shu Zhang , J. W. Kriza , J. A. Rodriguez-Rivera , Yiming Qiu , B. Winn , R. J. Cava , C. L. Broholm

Quantum spin liquids (QSLs) represent a novel state where spins are highly entangled but do not order even at zero temperature due to strong quantum fluctuations. Such a state is mostly studied in Heisenberg models defined on geometrically…