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Promising pathways for photoassociative formation of ultracold heteronuclear alkali metal dimers in their lowest rovibronic levels (denoted X(0,0)) are examined using high quality ab initio calculations of potential energy curves currently…

Atomic Physics · Physics 2016-09-28 W. C. Stwalley , J. RayMajumder , M. Bellos , R. Carollo , M. Recore , M. Mastroianni

We have studied the effect of resonant electronic state coupling on the formation of ultracold ground-state $^{85}$Rb$_2$. Ultracold Rb$_2$ molecules are formed by photoassociation (PA) to a coupled pair of $0_u^+$ states, $0_u^+(P_{1/2})$…

Atomic Physics · Physics 2008-10-31 H. K. Pechkis , D. Wang , Y. Huang , E. E. Eyler , P. L. Gould , W. C. Stwalley , C. P. Koch

We study dynamics of a two-color photoassociation of atoms into diatomic molecules via nonlinear Stimulated Raman adiabatic passage (STIRAP) process. This system has a famous counterpart in (linear) quantum mechanics, and been discussed…

Other Condensed Matter · Physics 2007-12-13 A. P. Itin , S. Watanabe

Ultracold LiCs molecules in the absolute ground state X$^1\Sigma^+$, v"=0, J"=0 are formed via a single photo-association step starting from laser-cooled atoms. The selective production of v"=0, J"=2 molecules with a 50-fold higher rate is…

Quantum Physics · Physics 2010-08-09 J. Deiglmayr , A. Grochola , M. Repp , K. Mörtlbauer , C. Glück , J. Lange , O. Dulieu , R. Wester , M. Weidemüller

We experimentally demonstrate a one-color two-photon transition from the $5\mathit{S}_{1/2}$ ground state to the $6\mathit{S}_{1/2}$ excited state in rubidium (Rb) vapor using a continuous wave laser at 993 nm. The Rb vapor contains both…

Atomic Physics · Physics 2019-02-22 Thomas Nieddu , Tridib Ray , Krishnapriya S. Rajasree , Ritayan Roy , Síle Nic Chormaic

Helium atoms have been prepared in the circular $|n=55,\ell=54,m_{\ell}=+54\rangle$ Rydberg state using the crossed electric and magnetic fields method. The atoms, initially travelling in pulsed supersonic beams, were photoexcited from the…

Atomic Physics · Physics 2016-11-07 V. Zhelyazkova , S. D. Hogan

We create an ultracold dense quantum gas of ground state molecules bound by more than 1000 wavenumbers by stimulated two-photon transfer of molecules associated on a Feshbach resonance from a Bose-Einstein condensate of cesium atoms. The…

We study the growth dynamics of ordered structures of strongly interacting polar molecules in optical lattices. Using dipole blockade of microwave excitations, we map the system onto an interacting spin-1/2 model possessing ground states…

Quantum Gases · Physics 2012-09-17 Mikhail Lemeshko , Roman V. Krems , Hendrik Weimer

We prepare mixtures of ultracold CaF molecules and Rb atoms in a magnetic trap and study their inelastic collisions. When the atoms are prepared in the spin-stretched state and the molecules in the spin-stretched component of the first…

We analyze excitation of two ground state atoms to a double Rydberg state by a two-photon chirped optical pulse in the regime of adiabatic rapid passage. For intermediate Rydberg-Rydberg interaction strengths, relevant for atoms separated…

Quantum Physics · Physics 2015-06-11 Elena Kuznetsova

We report on photoassociation spectroscopy probing the $c^3\Sigma_{1}^+$ potential of the bi-alkali NaCs molecule, identifying eleven vibrational lines between $v' = 0$ and $v' = 25$ of the excited $c^3\Sigma_{1}^+$ potential, and resolving…

We investigate magnetoassociation of ultracold fermionic Feshbach molecules in a mixture of $^{40}$K and $^{87}$Rb atoms, where we can create as many as $7\times 10^4$ $^{40}$K$^{87}$Rb molecules with a conversion efficiency as high as 45%.…

Quantum Gases · Physics 2013-09-12 Tyler D. Cumby , Ruth A. Shewmon , Ming-Guang Hu , John D. Perreault , Deborah S. Jin

We have numerically simulated quantum tomography of single-qubit and two-qubit quantum gates with qubits represented by mesoscopic ensembles containing random numbers of atoms. Such ensembles of strongly interacting atoms in the regime of…

We report on the observation of highly excited ($\nu \sim 100)$ vibrational states of a trilobite ultralong-range Rydberg molecule in $^{87}$Rb. These states manifest spectroscopically in a regularly spaced series of peaks red-detuned from…

A robust quantum protocol has been developed that achieves highly efficient entanglement transfer from a three-atom Rydberg system, initially in a W state (|rrg>+|rgr>+|grr>)/3^0.5, to an equivalent photonic W state…

Quantum Physics · Physics 2024-09-25 Aneesh Ramaswamy , Svetlana Malinovskaya

This work theoretically investigates possibilities of using the Stimulated Raman Adiabatic Passage (STIRAP) and its variants to control a coherent superposition of quantum states. We present a generalization of the so-called fractional…

Quantum Physics · Physics 2026-01-14 Miguel A. Alarcón , Karl Hauser , Nikolay V. Golubev

We have studied hetero- and homonuclear excited state/ground state collisions by loading both $^{85}$Rb and $^{87}$Rb into a far off resonant trap (FORT). Because of the relatively weak confinement of the FORT, we expect the hyperfine…

This paper deals with the electronic structure of RbSr, a molecule possessing both a permanent magnetic and electric dipole moment in its own frame allowing its manipulation with external fields. Two complementary ab-initio approaches are…

Chemical Physics · Physics 2014-07-16 Piotr S. Żuchowski , Romain Guerout , Olivier Dulieu

We report on precision measurements of spin-dependent interaction-strengths in the 87Rb spin-1 and spin-2 hyperfine ground states. Our method is based on the recent observation of coherence in the collisionally driven spin-dynamics of…

Other Condensed Matter · Physics 2007-05-23 Artur Widera , Fabrice Gerbier , Simon Foelling , Tatjana Gericke , Olaf Mandel , Immanuel Bloch

Circular Rydberg states with $n=70$ have been prepared in helium using a modified version of the crossed-fields method. This approach to the preparation of high-$n$ circular Rydberg states overcomes limitations of the standard…

Atomic Physics · Physics 2018-10-26 A. A. Morgan , V. Zhelyazkova , S. D. Hogan
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