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Conventional superexchange rules predict ferromagnetic exchange interaction between Ni(II) and M (M=Mo(V), W(V), Nb(IV)). Recent experiments show that in some systems this superexchange is antiferromagnetic. To understand this feature, in…

Strongly Correlated Electrons · Physics 2009-11-11 Rajamani Raghunathan , Jean-Pascal Sutter , Laurent Ducasse , Cedric Desplanches , S. Ramasesha

We study the finite temperature, low energy, long wave-length spectrum of the dynamic structure factor of the spin-$1/2$ antiferromagnetic Heisenberg chain in the presence of exchange anisotropy and external magnetic fields. Using…

Strongly Correlated Electrons · Physics 2015-01-15 Yousef Rahnavard , Robin Steinigeweg , Wolfram Brenig

A comprehensive theoretical and experimental study is presented of the magnetic susceptibility versus temperature \chi(T) of spin S = 1/2 two- and three-leg Heisenberg ladders and ladder oxide compounds. Extensive quantum Monte Carlo…

We report high-resolution x-ray diffraction, muon-spin-rotation spectroscopic and specific heat measurements in the double spin-chains compound $\rm LiCu_2O_2$. The x-ray diffraction results show that the crystal structure of $\rm…

Strongly Correlated Electrons · Physics 2009-10-31 B. Roessli , U. Staub , A. Amato , D. Herlach , P. Pattison , K. Sablina , G. A. Petrakovskii

We derive a quantum spin Hamiltonian of the spin-1/2 zigzag chain realized in a rare earth ytterbium-based magnetic insulator, YbCuS2. This material undergoes a transition at 0.95K to an incommensurate magnetic phase with small moments,…

Strongly Correlated Electrons · Physics 2024-08-02 Hidehiro Saito , Hiroki Nakai , Chisa Hotta

We study few-magnon excitations in a finite-size spin-$S$ chain with ferromagnetic nearest-neighbor (NN) interaction $J>0$ and antiferromagnetic next-nearest-neighbor (NNN) interaction $J'<0$, in the presence of the single-ion (SI)…

Strongly Correlated Electrons · Physics 2024-05-03 Jiawei Li , Ye Cao , Ning Wu

To understand spin interactions in materials of the Cu$_2$Sb structure type, inelastic neutron scattering of Fe$_2$As single crystals was examined at different temperatures and incident neutron energies. The experimental phonon spectra…

The spin 1/2 Heisenberg model on a square lattice with antiferromagnetic nearest- and next-nearest neighbour interactions (the $J_1$--$J_2$ model) has long been studied as a paradigm of a two-dimensional frustrated quantum magnet. Only very…

Strongly Correlated Electrons · Physics 2007-05-23 Nic Shannon , Burkhard Schmidt , Karlo Penc , Peter Thalmeier

A neutron scattering study of the Mott-Hubbard insulator LaTiO$_{3}$ (T$_{{\rm N}}=132$ K) reveals a spin wave spectrum that is well described by a nearest-neighbor superexchange constant $J=15.5$ meV and a small Dzyaloshinskii-Moriya…

Strongly Correlated Electrons · Physics 2009-10-31 B. Keimer , D. Casa , A. Ivanov , J. W. Lynn , M. v. Zimmermann , J. P. Hill , D. Gibbs , Y. Taguchi , Y. Tokura

CaMn$_2$P$_2$ exemplifies the realization of a frustrated $J_1$-$J_2$-$J_3$ Heisenberg model of a corrugated honeycomb magnetic lattice. Previous studies show that below the N\'eel temperature ($T_{\rm N}$), the system forms a cycloidal…

We report thermodynamic measurements of the S=1/2 kagome lattice antiferromagnet ZnCu$_{3}$(OH)$_{6}$Cl$_{2}$, a promising candidate system with a spin-liquid ground state. Using single crystal samples, the magnetic susceptibility both…

Strongly Correlated Electrons · Physics 2012-04-16 Tianheng Han , Shaoyan Chu , Young S. Lee

We report a neutron diffraction and muon spin relaxation muSR study of static and dynamical magnetic properties of BaCo2V2O8, a quasi-one-dimensional spin-chain system. A proposed model for the antiferromagnetic structure includes: a…

Understanding the dynamics of interacting quantum spins has been one of the active areas of condensed matter physics research. Recently, extensive inelastic neutron scattering measurements have been carried out in an interesting class of…

Strongly Correlated Electrons · Physics 2018-08-27 Kingshuk Majumdar , S. D. Mahanti

The magnetic ground state of the quasi-one-dimensional spin-1 antiferromagnetic chain is sensitive to the relative sizes of the single-ion anisotropy ($D$) and the intrachain ($J$) and interchain ($J'$) exchange interactions. The ratios…

We investigate the resilience of spinon quasiparticles in the $J_1$-$J_2$ zig-zag spin chain ($J_2>0$) from the viewpoint of momentum-space entanglement. For small $J_2$, we show that deconfined spinons survive well past the liquid-dimer…

Strongly Correlated Electrons · Physics 2026-05-01 Tom Oeffner , Ludwig Bordfeldt , Andreas Feuerpfeil , Lukas Elter , Tobias Helbig , Tobias Hofmann , Martin Greiter , Ronny Thomale

Magnetic properties of the spin doughnut Mo_{75}V_{20}, which is a frustrated magnetic cluster with twenty spins, are studied by using the finite-temperature Lanczos method. Our model Hamiltonian consists of one ten-spin ring and two…

Strongly Correlated Electrons · Physics 2009-11-13 S. Takemura , Y. Fukumoto

We report the results of muon-spin relaxation measurements on the low-dimensional antiferromagnet Rb4Cu(MoO4)3. No long-range magnetic order is observed down to 50 mK implying a ratio T_N/J<0.005 (where J is the principal exchange strength…

Strongly Correlated Electrons · Physics 2014-01-17 T. Lancaster , P. J. Baker , F. L. Pratt , S. J. Blundell , W. Hayes , D. Prabhakaran

Elastic and inelastic neutron scattering were used to study the ordered phase of the quasi-one-dimensional spin-1/2 antiferromagnet ${\rm BaCu_{2}Si_{2}O_{7}}$. The previously proposed model for the low-temperature magnetic structure was…

Strongly Correlated Electrons · Physics 2016-08-15 M. Kenzelmann , A. Zheludev , S. Raymond , E. Ressouche , T. Masuda , P. Böni , K. Kakurai , I. Tsukada , K. Uchinokura , R. Coldea

Using inelastic neutron scattering, we have observed a quasi-one-dimensional dispersive magnetic excitation in the frustrated triangular-lattice spin-2 chain oxide Ca3Co2O6. At the lowest temperature (T = 1.5 K), this magnon is…

Strongly Correlated Electrons · Physics 2013-12-17 Anil Jain , P. Y. Portnichenko , Hoyoung Jang , G. Jackeli , G. Friemel , A. Ivanov , A. Piovano , S. M. Yusuf , B. Keimer , D. S. Inosov

The scenario of a metal-insulator transition driven by the onset of antiferromagnetic order in NaOsO$_3$ calls for a trustworthy derivation of the underlying effective spin Hamiltonian. To determine the latter we rely on {\it ab initio}…

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