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In this study, we conducted experiments on CaC6 for elucidating the Na-catalyzed formation mechanism and achieving rapid mass synthesis of graphite intercalation compounds (GICs). Rapidly synthesized CaC6 was characterized by analysis of…

The discovery of superconductivity in CaC6 with a critical temperature (Tc) of 11.5 K reignites much interest in exploring high-temperature superconductivity in graphite intercalation compounds (GICs). Here we identify a GIC NaC4,…

Graphite intercalation compounds (GICs) have long been recognized as promising candidates for high-temperature superconductivity by intercalation or charge doping, yet experimental progress has stalled with transition temperatures (Tc)…

In this letter, we report the discovery of superconductivity in Li3Ca2C6. Several graphite intercalation compounds (GICs) with electron donors, are well known as superconductors. It is probably not astonishing, since it is generally…

Lanthanides ($Ln$) are notoriously difficult to intercalate into graphite. We investigated the possibility of using Na to catalyze the formation of $Ln$-intercalated graphite and successfully synthesized $Ln$C$_6$ ($Ln$ = Sm, Eu, and Yb)…

We show using scanning tunneling microscopy, spectroscopy, and ab initio calculations that several intercalation structures exist for Na in epitaxial graphene on SiC(0001). Intercalation takes place at room temperature and Na electron-dopes…

Mesoscale and Nanoscale Physics · Physics 2011-12-01 Andreas Sandin , Thushari Jayasekera , J. E. , Rowe , Ki Wook Kim , M. Buongiorno Nardelli , Daniel B. Dougherty

The process of anion intercalation in graphite and its reversibility plays a crucial role in the next generation energy-storage devices. Herein the reaction mechanism of the aluminum graphite dual ion cell by operando X-ray scattering from…

Materials Science · Physics 2024-02-21 Giorgia Greco , Giuseppe Antonio Elia , Daniel Hermida-Merino , Robert Hahn , Simone Raoux

A recent ab initio investigation of Na-C binary compounds under moderate pressures has uncovered a possible stable NaC$_4$ superconductor with an estimated critical temperature up to 41K. We revisit this promising binary system by…

Using density functional theory calculations, we have investigated the structural, energetic, and electronic properties of ternary graphite intercalation compounds (GICs) containing alkali atoms (AM) and normal alkylamine molecules (nC$x$),…

Materials Science · Physics 2017-09-20 Gum-Chol Ri , Chol-Jun Yu , Jin-Song Kim , Song-Nam Hong , Un-Gi Jong , Mun-Hyok Ri

The cointercalation of sodium with the solvent organic molecule into graphite can resolve difficulty of forming the stage-I Na-graphite intercalation compound, which is a predominant anode of Na-ion battery. To clarify the mechanism of such…

Materials Science · Physics 2017-09-26 Chol-Jun Yu , Song-Bok Ri , Song-Hyok Choe , Gum-Chol Ri , Yun-Hyok Kye , Sung-Chol Kim

We report experimental results indicating possible high-temperature superconductivity in graphite intercalation compounds synthesized with lithium-based alloys. Temperature-dependent measurements of magnetization, trapped magnetic flux, and…

Graphite is a ubiquitous electrode material with particular promise for use in e.g., energy storage and desalination devices, but very little is known about the properties of the graphite-electrolyte double layer at technologically relevant…

Materials Science · Physics 2021-09-03 Aaron R. Finney , Ian J. McPherson , Patrick R. Unwin , Matteo Salvalaglio

We have experimentally investigated the expansion mechanism induced by laser irradiation of H2SO4 intercalated graphite. Intercalated graphite materials irradiated by laser allows to study reactions occurring in confined chemical…

Materials Science · Physics 2014-07-24 G. Carotenuto , A. Longo , L. Nicolais , S. De Nicola , E. Pugliese , M. Ciofini , M. Locatelli , A. Lapucci , R. Meucci

The pressure effect on the superconducting transition temperature ($T_c$) of the newly-discovered Ca-intercalated graphite compound CaC$_6$ has been investigated up to $\sim$ 16 kbar. $T_c$ is found to increase under pressure with a large…

Superconductivity · Physics 2015-06-25 J. S. Kim , L. Boeri , R. K. Kremer , F. S. Razavi

The deposition and intercalation of metal atoms can induce superconductivity in monolayer and bilayer graphenes. For example, it has been experimentally proved that Li-deposited graphene is a superconductor with critical temperature $T_{c}$…

Superconductivity · Physics 2024-05-07 Jin-Han Tan , Hao Wang , Ying-Jie Chen , Na Jiao , Meng-Meng Zheng , Hong-Yan Lu , Ping Zhang

Although not an intrinsic superconductor, it has been long--known that, when intercalated with certain dopants, graphite is capable of exhibiting superconductivity. Of the family of graphite--based materials which are known to superconduct,…

Superconductivity · Physics 2016-08-16 Gabor Csányi , P. B. Littlewood , A. H. Nevidomskyy , Chris J. Pickard , B. D. Simons

On the basis of the model that was successfully applied to KC8, RbC8, and CsC8 in 1982, we have calculated the superconducting transition temperature Tc for CaC6 and YbC6 to find that the same model reproduces the observed Tc in those…

Superconductivity · Physics 2016-01-13 Yasutami Takada

In this work, we have comprehensively studied the effect of auxiliary intercalating agents on the thermal conductivity of expanded graphite (EG) polymer composites. We report an ultra-high enhancement of 4030% in thermal conductivity of…

Alkali intercalated graphite compounds represent a compelling modification of carbon with significant application potential and various fundamentally important phases. We report on the intercalation of graphite with alkali atoms (Li and K)…

Strongly Correlated Electrons · Physics 2019-12-19 B. G. Márkus , S. Kollarics , P. Szirmai , B. Náfrádi , L. Forró , J. C. Chacón-Torres , T. Pichler , F. Simon

We describe the reversible intercalation of Na under graphene on Ir(111) by photo-dissociation of a previously adsorbed NaCl overlayer. After room temperature evaporation, NaCl adsorbs on top of graphene forming a bilayer. With a…

Materials Science · Physics 2019-04-26 I. Palacio , L. Aballe , M. Foerster , D. G. de Oteyza , M. García-Hernández , J. A. Martín-Gago
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