Related papers: Ultrafast control over chiral sum-frequency genera…
One of the main difficulties to efficiently generating high-order harmonics in long neutral-gas targets is to reach the phase-matching conditions. One issue is that the medium cannot be sufficiently ionized by the driving laser due to…
All-optical devices are essential for next generation ultrafast, ultralow-power and ultrahigh bandwidth information processing systems. Silicon microring resonators (SiMRR) provide a versatile platform for all-optical switching and…
An all-optical measurement of high-order fractional molecular echoes is demonstrated by using high-order harmonic generation (HHG). Excited by a pair of time-delayed short laser pulses, the signatures of full and high order fractional (1/2…
The topological response of matter to electromagnetic fields is a property in high demand in materials design and metrology due to its robustness against noise and decoherence, stimulating recent advances in ultrafast photonics. Embedding…
Designing objects with predefined optical properties is a task of fundamental importance for nanophotonics, and chirality is a prototypical example of such a property, with applications ranging from photochemistry to nonlinear photonics. A…
Ultrafast processes in matter can be captured and even controlled by using sequences of few-cycle optical pulses, which need to be well characterized, both in amplitude and phase. The same degree of control has not yet been achieved for…
Silicon photonics lacks a second-order nonlinear optical response in general because the typical constituent materials are centro-symmetric and lack inversion symmetry, which prohibits second-order nonlinear processes such as second…
Chiral nonlinear response has been explored for decades due to its extreme sensitivity to molecular and structural dissymmetry. Conventional approaches often require bulky systems and produce only static nonlinear chirality. Here, we report…
Holographic optical tweezers can be applied to manipulate microscopic particles in arbitrary optical patterns, which classical optical tweezers cannot do. This ability relies on accurate computer-generated holography (CGH), yet most CGH…
It is demonstrated that the non-instantaneous response of the optically induced coherent polarization tremendously influences the real-space shift of electronic charges in semiconductors. The possibility to coherently control this…
We resolve the real-time electric field of a femtosecond third-order nonlinear optical signal in the molecular frame. The electric field emitted by the induced third-order polarization from impulsively pre-aligned gas-phase molecules at…
The ability to use coherent light for material science and applications is directly linked to our ability to measure short optical pulses. While free-space optical methods are well-established, achieving this on a chip would offer the…
Ultrafast mid-infrared (MIR) imaging is a key enabling capability for monitoring transient thermal and plasma phenomena in scientific diagnostics and industrial safety. However, conventional cryogenic MIR cameras face a fundamental…
We propose a new concept to generate efficient one-third harmonic light from an unseeded third harmonic process in optical fibers. Our concept is based on the dynamic constant (Hamiltonian) of the nonlinear third harmonic generation in…
Tailoring optical nonlinear effects (e.g. harmonic generation, sum-frequency mixing, etc.) in the recently emerging all-dielectric platform is important for both the fundamental science and industrial development of high-efficiency,…
We experimentally demonstrate sum-frequency generation (SFG) with entangled photon-pairs, generating as many as 40,000 SFG photons per second, visible even to the naked eye. The nonclassical nature of the interaction is exhibited by a…
We demonstrate second order optical nonlinearity in aluminum nitride on insulator substrates. Using sputter-deposited aluminum nitride thin films we realize nanophotonic waveguides coupled to micro-ring resonators that simultaneously…
Controlling femtosecond optical pulses with temporal precision better than one cycle of the carrier field has a profound impact on measuring and manipulating interactions between light and matter. We explore pulses that are carved from a…
High harmonic generation traditionally combines ~100 near-infrared laser photons, to generate bright, phase matched, extreme ultraviolet beams when the emission from many atoms adds constructively. Here we show that by guiding a…
The possibility of creating and manipulating nanostructured materials encouraged the exploration of new strategies to control electromagnetic properties. Among the most intriguing nanostructures are those that respond differently to helical…