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Access to the electron spin is at the heart of many protocols for integrated and distributed quantum-information processing [1-4]. For instance, interfacing the spin-state of an electron and a photon can be utilized to perform quantum gates…

We report the first demonstration of a direct interaction between the extraordinary transverse spin angular momentum in evanescent waves and the intrinsic orbital angular momentum in optical vortex beams. By tapping the evanescent wave of…

Optics · Physics 2018-05-09 Zengkai Shao , Jiangbo Zhu , Yujie Chen , Yanfeng Zhang , Siyuan Yu

The regular structures obtained by optical lattice technology and their behaviour are analysed from the quantum information perspective. Initially, we demonstrate that a triangular optical lattice of two atomic species, bosonic or…

Due to their intrinsic electric dipole moments and rich internal structure, ultracold polar molecules are promising candidate qubits for quantum computing and for a wide range of quantum simulations. Their long-lived molecular rotational…

The great success of point defects and dopants in semiconductors for quantum information processing has invigorated a search for molecules with analogous properties. Flexibility and tunability of desired properties in a large chemical space…

Materials Science · Physics 2023-01-11 Karolina Janicka , Aleksander L. Wysocki , Kyungwha Park

Optically connecting quantum bits can effectively reduce decoherence and facilitate long-distance communication. Optically addressable spin-bearing molecules have been demonstrated to have a good potential for quantum computing. In this…

Quantum Physics · Physics 2023-03-28 Jiawei Chang , Tianhong Huang , Lin Ma , Taoyu Zou , Hai Wang , Wei Wu

In semiconductors, the T2* coherence time of a single confined spin is limited either by the fluctuating magnetic environment (via the hyperfine interaction), or by charge fluctuations (via the spin-orbit interaction). We demonstrate that…

Mesoscale and Nanoscale Physics · Physics 2012-04-13 K. M. Weiss , J. M. Elzerman , Y. L. Delley , J. Miguel-Sanchez , A. Imamoglu

Molecular platforms are regarded as promising candidates in the generation of units of information for quantum computing. Herein, a strategy combining spin-crossover metal ions and radical ligands is proposed from a model Hamiltonian first…

Quantum Physics · Physics 2022-12-07 Roseiro Pablo , Petit Louis , Robert Vincent , Yalouz Saad

We introduce a novel optical interface between a singlet-triplet spin qubit and a photonic qubit which would offer new prospects for future quantum communication applications. The interface is based on a 220 nm thick GaAs/Al-GaAs…

Hybrid quantum photonic systems connect classical photonics to the quantum world and promise to deliver efficient light-matter quantum interfaces while leveraging the advantages of both, the classical and the quantum, subsystems. However,…

Tunnel-coupled optically active quantum dot molecules (QDMs), have the potential to operate as spin-photon-interfaces with coupled spins that interact with two different photon frequencies at the same time. A prerequisite is to…

We report on the local control of the transition frequency of a spin-$1/2$ encoded in two Rydberg levels of an individual atom by applying a state-selective light shift using an addressing beam. With this tool, we first study the spectrum…

Molecular spins are a versatile platform for quantum sensing. Not only are the spin-bearing molecules themselves widely tunable, they are also capable of being used as sensors as crystals, films and in solution. Using thin-films offers the…

Materials Science · Physics 2026-01-21 Adrian Mena , Nicholas P. Sloane , Max R. Bonengel , Dane R. McCamey

Understanding the interplay between a quantum system and its environment lies at the heart of quantum science and its applications. To-date most efforts have focused on circumventing decoherence induced by the environment by either…

Nuclear magnetic resonance (NMR) is a powerful tool for applications ranging from chemical analysis to quantum information processing. Achieving optical initialization and detection of molecular nuclear spins promises new opportunities -…

Scaling-up optical quantum technologies requires to combine highly efficient multi-photon sources and integrated waveguide components. Here, we interface these scalable platforms: a quantum dot based multi-photon source and a reconfigurable…

Strong long-distance spin-magnon coupling is essential for solid-state quantum information processing and single qubit manipulation. Here, we propose an approach to realize strong spin-magnon coupling in a hybrid optomechanical…

Quantum Physics · Physics 2023-04-05 Wei Xiong , Mingfeng Wang , Guo-Qiang Zhang , Jiaojiao Chen

Molecular nanostructures are promising building blocks for future quantum technologies, provided methods of harnessing their multiple degrees of freedom can be identified and implemented. Due to low decoherence rates nuclear spins are…

Quantum Physics · Physics 2011-11-15 Marcus Schaffry , Brendon W. Lovett , Erik M. Gauger

We propose an approach to probe coherent spin-state dynamics of molecules using circularly polarized hard x-ray pulses. For the dynamically aligned nitric oxide molecules in a coherent superposition spin-orbit coupled electronic state that…

Optics · Physics 2024-01-02 Xiaoyu Mi , Ming Zhang , Zheng Li

Strongly interacting spins underlie many intriguing phenomena and applications ranging from magnetism to quantum information processing. Interacting spins combined with motion display exotic spin transport phenomena, such as superfluidity…