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Using molecular dynamics computer simulations we investigate the structural and dynamical properties of a simple model for a colloidal gel at low volume fraction. We find that at low T the system is forming an open percolating cluster,…

Disordered Systems and Neural Networks · Physics 2015-06-25 Emanuela Del Gado , Walter Kob

A Rayleigh-Taylor-like instability of a dense colloidal layer under gravity in a capillary of microfluidic dimensions is considered. We access all relevant lengthscales with particle-level microscopy and computer simulations which…

We develop and validate a simulation framework for colloidal gelation. We first reproduce the benchmark results of Santos, Campanella, and Carignano for spherical, gel-forming particles, then extend the methodology to more complex systems…

Soft Condensed Matter · Physics 2025-11-24 Johannes Krotz

In this letter, we investigate several aspects related to the effect of hydrodynamics interactions on phase separation-induced gelation of colloidal particles. We explain physically the observation of Tanaka and Araki[Phys. Rev. Lett. {\bf…

Soft Condensed Matter · Physics 2007-05-23 R. Yamamoto , K. Kim , Y. Nakayama , K. Miyazaki , D. R. Reichman

Gels in soft-matter systems are an important nonergodic state of matter. We study a colloid-polymer mixture which is quenched by increasing the polymer concentration, from a fluid to a gel. Using confocal microscopy, we study both the…

Soft Condensed Matter · Physics 2009-04-20 Takehiro Ohtsuka , C. Patrick Royall , Hajime Tanaka

The aggregation of binary colloids of same size and balanced charges is studied by Brownian dynamics simulations for dilute suspensions. It is shown that, under appropriate conditions, the formation of colloidal crystals is dominated by…

Soft Condensed Matter · Physics 2015-06-12 D. Bochicchio , A. Videcoq , R. Ferrando

Colloidal gels constitute an important class of materials found in many contexts and with a wide range of applications. Yet as matter far from equilibrium, gels exhibit a variety of time-dependent behaviours, which can be perplexing, such…

Soft Condensed Matter · Physics 2021-09-22 C. Patrick Royall , Malcolm A. Faers , Sian L. Fussell , James E. Hallett

The effects of particle roughness and short-ranged non-central forces on colloidal gels are studied using computer simulations in which particles experience a sinusoidal variation in energy as they rotate. The number of minima $n$ and…

Soft Condensed Matter · Physics 2019-09-05 Hong T. Nguyen , Alan L. Graham , Peter H. Koenig , Lev D. Gelb

All liquids (except helium due to quantum effects) crystallize at low temperatures, forming ordered structures. The competition between disorder, which stabilizes the liquid phase, and energy, which favors the ordered crystalline structure,…

Soft Condensed Matter · Physics 2013-07-09 Frank Smallenburg , Francesco Sciortino

The observed rapid onset of star formation in molecular clouds requires rapid formation of dense fragments which can collapse individually before being overtaken by global gravitationally-driven flows. Many previous investigations have…

Astrophysics · Physics 2009-11-13 F. Heitsch , L. Hartmann , A. Burkert , ;

Glasses and gels are the two dynamically arrested, disordered states of matter. Despite their importance, their similarities and differences remain elusive, especially at high density. We identify dynamical and structural signatures which…

Soft Condensed Matter · Physics 2014-09-22 C. Patrick Royall , Stephen R. Williams , Hajime Tanaka

We have carried out molecular dynamics simulations of the crystallization of hard spheres modelling colloidal systems that are studied in conventional and space-based experiments. We use microscopic probes to investigate the effects of…

Condensed Matter · Physics 2009-11-07 Igor Volkov , Marek Cieplak , Joel Koplik , Jayanth R. Banavar

Confined granular fluids, placed in a shallow box that is vibrated vertically, can achieve homogeneous stationary states thanks to energy injection mechanisms that take place throughout the system. These states can be stable even at high…

Soft Condensed Matter · Physics 2015-06-12 Ricardo Brito , Dino Risso , Rodrigo Soto

Colloid-polymer mixtures can undergo spinodal decomposition into colloid-rich and colloid-poor regions. Gelation results when interconnected colloid-rich regions solidify. We show that this occurs when these regions undergo a glass…

Soft Condensed Matter · Physics 2009-11-10 S. Manley , H. M. Wyss , K. Miyazaki , J. C. Conrad , V. Trappe , L. J. Kaufman , D. R. Reichman , D. A. Weitz

The normal modes and relaxation rates of weak colloidal gels are investigated in computations employing different models of the hydrodynamic interactions between colloids. The eigenspectrum is computed for freely draining,…

Fluid Dynamics · Physics 2018-01-17 Zsigmond Varga , James W. Swan

In non-dilute colloidal suspensions, gradients in particle volume fraction result in gradients in electrical conductivity and permittivity. An externally applied electric field couples with gradients in electrical conductivity and…

Fluid Dynamics · Physics 2015-05-13 Carlos L. Perez , Jonathan D. Posner

We investigate the stationary flow of a colloidal gel under an inhomogeneous external shear force using adaptive Brownian dynamics simulations. The interparticle forces are derived from the Stillinger-Weber potential, where the three-body…

Soft Condensed Matter · Physics 2025-07-15 Florian Sammüller , Daniel de las Heras , Matthias Schmidt

Water droplet freezing is a common phenomenon in our daily life. In both natural scenarios and industrial production, different surface inclinations bring distinctive deformation and freezing dynamics to frozen droplets. We explore the…

Fluid Dynamics · Physics 2022-10-05 Hao Zeng , Sijia Lyu , Dominique Legendre , Chao Sun

Colloidal model systems allow studying crystallization kinetics under fairly ideal conditions with rather well characterized pair interactions and minimized external influences. In complementary approaches therefore experiment, analytic…

Soft Condensed Matter · Physics 2015-06-19 Thomas Palberg

Recent theories predict that when a supercooled liquid approaches the glass transition, particle clusters with a special "amorphous order" nucleate within the liquid, which lead to static correlations dictating the dramatic slowdown of…

Soft Condensed Matter · Physics 2016-03-04 Bo Zhang , Xiang Cheng