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Mid-infrared high-resolution spectroscopy has proven an invaluable tool for the study of the structure and dynamics of molecules in the gas phase. The advent of frequency combs advances the frontiers of precise molecular spectroscopy. Here…

Optics · Physics 2019-02-28 Zaijun Chen , Theodor W. Hänsch , Nathalie Picqué

Optical frequency combs have revolutionized the field of frequency metrology within the last decade and have become enabling tools for atomic clocks, gas sensing and astrophysical spectrometer calibration. The rapidly increasing number of…

Optics · Physics 2015-11-30 P. Del'Haye , T. Herr , E. Gavartin , R. Holzwarth , T. J. Kippenberg

The mid-infrared spectral range (2 to 20 \mu m) is of particular importance for chemistry, biology and physics as many molecules exhibit strong ro-vibrational fingerprints. Frequency combs - broad spectral bandwidth coherent light sources…

The impact of photodetector nonlinearity on dual-comb spectrometers is described and compared to that of Michelson-based Fourier transform spectrometers (FTS). The optical sampling occurring in the dual-comb approach, being the key…

Sub-sampling can acquire directly a passband within a broad radio frequency (RF) range, avoiding down-conversion and low-phase-noise tunable local oscillation (LO). However, sub-sampling suffers from band folding and self-image…

Instrumentation and Detectors · Physics 2017-07-29 Wenhui Hao , Yitang Dai , Feifei Yin , Yue Zhou , Jianqiang Li , Jian Dai , Wangzhe Li , Kun Xu

The sensitivity of molecular fingerprinting is dramatically improved when placing the absorbing sample in a high-finesse optical cavity, thanks to the large increase of the effective path-length. As demonstrated recently, when the…

We demonstrate broadband and sensitive cavity ring-down spectroscopy using a near infrared frequency comb and a time-resolved Fourier transform spectrometer. The cavity decays are measured simultaneously and spectrally sorted, leading to…

Optics · Physics 2022-01-28 Romain Dubreoucq , Lucile Rutkowski

We present a novel approach to realize microresonator-comb-based high resolution spectroscopy that combines a fiber-laser cavity with a microresonator. Although the spectral resolution of a chip-based comb source is typically limited by the…

Dual-comb spectroscopy has demonstrated remarkable capabilities for rapid and sensitive measurements; however, significant challenges still exist in generating high-power, mutually coherent mid-infrared combs. Here we demonstrate that a…

Broadband dual-comb spectroscopy (DCS) based on portable mode-locked fiber frequency combs is a powerful tool for in situ, calibration free, multi-species spectroscopy. While the acquisition of a single spectrum with mode-locked DCS…

Optics · Physics 2021-02-03 Nazanin Hoghooghi , Ryan K. Cole , Gregory B. Rieker

Optical-frequency synthesizers are lasers stabilized and programmed from a microwave clock for applications, especially in fundamental measurements and spectroscopy, optical-communication links, and precision sensing of numerous physical…

Direct optical frequency Comb Spectroscopy (DCS) is proving to be a fundamental tool in many areas of science and technology thanks to its unique performance in terms of ultra-broadband, high-speed detection and frequency accuracy, allowing…

We demonstrate high-resolution photonic RF filters using an RF bandwidth scaling approach based on integrated Kerr optical micro-combs. By employing both an active nonlinear micro-ring resonator (MRR) as a high-quality micro-comb source and…

Infrared spectroscopy in the spectral fingerprint region from 6-12 um accesses the largest molecular absorption cross-sections, permitting sensitive, quantitative and species-specific measurements. Here, we show how dual-comb…

Optics · Physics 2023-06-26 O. Kara , L. Maidment , T. Gardiner , P. G. Schunemann , D. T. Reid

The spectral resolution of broadband Fourier-transform coherent anti-Stokes Raman spectroscopy is limited by the maximum optical path length difference that can be scanned within a short time in an interferometer. However, alternatives to…

A miniaturized full-frequency encoded illumination (mini-FEI) chip is presented for high-throughput super-resolution imaging using the spatial frequency shift (SFS) effect. A tunable full SFS scheme is achieved through propagating and…

Spectral analysis is one of the most powerful technologies for studying and understanding matter. As the devices for spectral analysis, spectrometers are widely used in material detection, isotope analysis, trace gas detection, and the…

Frequency combs have revolutionized time and frequency metrology and in recent years, new frequency comb lasers that are highly compact or even on-chip have been demonstrated in the mid-infrared and THz regions of the electromagnetic…

Optics · Physics 2019-07-17 Giacomo Scalari , Jérôme Faist , Nathalie Picqué

The Fractional Fourier Transform (FRT) corresponds to an arbitrary-angle rotation in the phase space, e.g. the time-frequency (TF) space, and generalizes the fundamentally important Fourier Transform. FRT applications range from classical…

Optics · Physics 2024-03-06 Michał Lipka , Michał Parniak

We characterize a new mid-infrared frequency comb generator based on difference frequency generation around 3.2 microns. High power per comb mode (>10-7 W/mode) is obtained over a broad spectral span (>700 nm). The source is used for direct…