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Related papers: Lu-H-N phase diagram from first-principles calcula…

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Evolutionary crystal structure prediction searches have been employed to explore the ternary Li-F-H system at 300 GPa. Metastable phases were uncovered within the static lattice approximation, with LiF$_3$H$_2$, LiF$_2$H, Li$_3$F$_4$H,…

Materials Science · Physics 2021-04-07 Tiange Bi , Andrew Shamp , Tyson Terpstra , Russell J. Hemley , Eva Zurek

Motivated by the recent report of room-temperature superconductivity at near-ambient pressure in N-doped lutetium hydride by Dasenbrock et al. [Nature 615, 244 (2023)], we performed a comprehensive, detailed study of the phase diagram of…

The recent report of near-ambient superconductivity in nitrogen-doped lutetium hydrides (Lu-N-H) has generated a great interest. However, conflicting results have raised doubts regarding superconductivity. Here, we combine high-throughput…

Superconductivity · Physics 2024-06-12 Yue-Wen Fang , Ðorđe Dangić , Ion Errea

This paper presents the results of an extensive structural search of ternary solids containing lutetium, nitrogen and hydrogen. Based on thousands of thermodynamically stable structures, available online, the convex hull of the formation…

Superconductivity · Physics 2024-12-06 Moritz Gubler , Marco Krummenacher , Jonas A. Finkler , Stefan Goedecker

Recently, Grockowiak $\textit{et al.}$ reported "hot superconductivity" in ternary or multinary compounds based on lanthanum hydride [A. D. Grockowiak $\textit{et al.}$, Front. Electron. Mater. $\textbf{2}$, 837651 (2022)]. In this paper,…

Superconductivity · Physics 2023-12-05 Takahiro Ishikawa , Yuta Tanaka , Shinji Tsuneyuki

In recent years, there has been a fervent search for room-temperature superconductivity within the binary hydrides. However, as the number of untested compounds dwindled, it became natural to begin searching within the ternary hydrides.…

Structural investigations conducted using transmission electron microscopy (TEM) on LuH2 synthesized under atmospheric pressure (AP-LuH2) and nitrogen-doped LuH2 synthesized under high pressure (HP-LuH2) have revealed numerous…

The stability of ($R$, Zr)(Fe, Co, Ti)$_{12}$ with a ThMn$_{12}$ structure is investigated using first-principles calculations. We consider energetic competition with multiple phases that have the Th$_2$Zn$_{17}$ structure and the unary…

Materials Science · Physics 2022-03-29 Taro Fukazawa , Yosuke Harashima , Takashi Miyake

The structure of the material responsible for the room temperature and near ambient pressure superconductivity reported in an N-doped lutetium hydride [Nature, 615, 244 (2023)] has not been conclusively determined. Herein, density…

Superconductivity · Physics 2023-08-09 Katerina P. Hilleke , Xiaoyu Wang , Dongbao Luo , Nisha Geng , Busheng Wang , Eva Zurek

Hydrogen-rich ternary hydrides are promising candidates for high-Tc superconductivity at megabar pressures, yet their chemical space is vast and largely unexplored. Combining evolutionary structure searches with first-principles…

In the nitrogen-doped lutetium hydride (Lu-H-N) system, the presence of Lu-N chemical bonds plays a key role in the emergence of possible room-temperature superconductivity at near ambient pressure. However, due to the synthesis of…

In this work, global search for crystal structures of ternary Mg-Sc-H hydrides (Mg$_x$Sc$_y$H$_z$) under high pressure ($100 \le P \le 200$ GPa) were performed using the evolutionary algorithm and first-principles calculations. Based on…

Uranium nitrides have been the subject of intense research owing to their potential applications as advanced nuclear fuels. However, the phase diagram of the U-N system at low temperature and high pressure still remains unclear. In this…

Computational Physics · Physics 2018-04-03 Dawei Zhou , JiaHui Yu , Chunying Pu , Yuling Song

Motivated by the recent discovery of near-room temperature superconductivity in high-pressure superhydrides, we investigate from first-principles the high-pressure superconducting phase diagram of the ternary Ca-B-H system, using ab-initio…

Superconductivity · Physics 2020-08-26 Simone Di Cataldo , Wolfgang von der Linden , Lilia Boeri

The research on hydrogen-rich ternary compounds attract tremendous attention for it paves new route to room-temperature superconductivity at lower pressures. Here, we study the crystal structures, electronic structures, and superconducting…

Superconductivity · Physics 2023-12-19 Juefei Wu , Bangshuai Zhu , Chi Ding , Cuiying Pei , Qi Wang , Jian Sun , Yanpeng Qi

We present an evolutionary construction technique of formation energy convex hull to search for thermodynamically stable compounds. In this technique, candidates with a wide variety of chemical compositions and crystal structures are…

Materials Science · Physics 2020-07-01 Takahiro Ishikawa , Takashi Miyake

Motivated by recent discovery of yttrium-based high-temperature ternary superconducting hydrides (e.g., CaYH$_{12}$, LaYH$_{12}$, and ScYH$_{6}$), we have employed evolutionary algorithm and first-principles calculations to comprehensively…

Ternary or more complex hydrogen-rich hydrides are the main hope of reaching room-temperature superconductivity at high pressures. Their chemical space is vast and its exploration is challenging. Here we report the investigation of the…

Superconductivity · Physics 2023-12-13 Grigoriy Shutov , Dmitrii Semenok , Ivan A. Kruglov , Artem R. Oganov

Structural changes in REMnO3 (RE= Y, Ho, Lu) under high pressure were examined by synchrotron x-ray diffraction methods at room temperature. Compression occurs more readily in the ab plane than along the c-axis. Under hydrostatic pressure…

Materials Science · Physics 2015-05-20 P. Gao , Z. Chen , T. A. Tyson , T. Wu , K. H. Ahn , Z. Liu , R. Tappero , S. B. Kim , S. -W. Cheong

LP-N and HLP-N are promising high-energy-density materials. However, these materials synthesized under high pressure cannot be maintained stable at ambient conditions. The mechanism behind their instability remains unclear. Our research,…

Materials Science · Physics 2025-03-17 Guo Chen , Xianlong Wang
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