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We compare the ability of a simulated annealing program and an evolutionary algorithm to find molecules with large molecular average hyperpolarizabilities. This property is an important component of nonlinear optical materials. Both…

Computational Physics · Physics 2026-02-19 Dominic Mashak , S. A. Alexander

One central mystery of neural NLP is what neural models "know" about their subject matter. When a neural machine translation system learns to translate from one language to another, does it learn the syntax or semantics of the languages?…

Computation and Language · Computer Science 2017-08-01 Chaitanya Malaviya , Graham Neubig , Patrick Littell

Graphs provide a unified representation of semantic content and relational structure, making them a natural fit for domains such as molecular modeling, citation networks, and social graphs. Meanwhile, large language models (LLMs) have…

Machine Learning · Computer Science 2026-05-04 Haotian Xu , Yuning You , Tengfei Ma

Machine learning has the potential to accelerate materials discovery by accurately predicting materials properties at a low computational cost. However, the model inputs remain a key stumbling block. Current methods typically use…

Computational Physics · Physics 2021-01-07 Rhys E. A. Goodall , Alpha A. Lee

Recently, the remarkable capabilities of large language models (LLMs) have been illustrated across a variety of research domains such as natural language processing, computer vision, and molecular modeling. We extend this paradigm by…

Machine Learning · Computer Science 2023-09-04 Hongshuo Huang , Rishikesh Magar , Changwen Xu , Amir Barati Farimani

We present SMILES-embeddings derived from the internal encoder state of a Transformer [1] model trained to canonize SMILES as a Seq2Seq problem. Using a CharNN [2] architecture upon the embeddings results in higher quality interpretable…

Quantitative Methods · Quantitative Biology 2020-09-23 Pavel Karpov , Guillaume Godin , Igor V. Tetko

Large Language Models (LLMs) are increasingly being used to support scientific discovery. In chemistry, tasks such as reaction prediction and structure elucidation require reasoning about the structures of molecules. As such, LLM-based…

Machine Learning · Computer Science 2026-05-05 Nicholas T. Runcie , Fergus Imrie , Charlotte M. Deane

We show that large language model (LLMs) can be transformed via supervised fine-tuning (SFT) of engineered prompts into SmileyLlama for exploring the chemical space of drug molecules. We benchmark SmileyLlama against pre-trained LLMs and…

Language models (LMs) are being scaled and becoming powerful. Improving their efficiency is one of the core research topics in neural information processing systems. Tay et al. (2022) provided a comprehensive overview of efficient…

Machine Learning · Computer Science 2023-06-06 Meng Jiang , Hy Dang , Lingbo Tong

The need for analysis of toxicity in new drug candidates and the requirement of doing it fast have asked the consideration of scientists towards the use of artificial intelligence tools to examine toxicity levels and to develop models to a…

Quantitative Methods · Quantitative Biology 2021-01-27 Mriganka Nath , Subhasish Goswami

Large language models (LLMs) are beginning to reshape how chemists plan and run reactions in organic synthesis. Trained on millions of reported transformations, these text-based models can propose synthetic routes, forecast reaction…

Artificial Intelligence · Computer Science 2025-08-08 Kartar Kumar Lohana Tharwani , Rajesh Kumar , Sumita , Numan Ahmed , Yong Tang

Curriculum Learning emphasizes the order of training instances in a computational learning setup. The core hypothesis is that simpler instances should be learned early as building blocks to learn more complex ones. Despite its usefulness,…

Computation and Language · Computer Science 2016-11-21 Volkan Cirik , Eduard Hovy , Louis-Philippe Morency

Large Language Models (LLMs) excel in diverse areas, yet struggle with complex scientific reasoning, especially in the field of chemistry. Different from the simple chemistry tasks (e.g., molecule classification) addressed in previous…

Computation and Language · Computer Science 2024-02-12 Siru Ouyang , Zhuosheng Zhang , Bing Yan , Xuan Liu , Yejin Choi , Jiawei Han , Lianhui Qin

Character-based neural models have recently proven very useful for many NLP tasks. However, there is a gap of sophistication between methods for learning representations of sentences and words. While most character models for learning…

Computation and Language · Computer Science 2018-10-31 Yingwei Xin , Ethan Hart , Vibhuti Mahajan , Jean-David Ruvini

This thesis focuses on improving the pre-training of natural language models using unsupervised raw data to make them more efficient and aligned with downstream applications. In the first part, we introduce three alternative pre-training…

Computation and Language · Computer Science 2023-09-18 Luca Di Liello

The detailed analysis of molecular structures and properties holds great potential for drug development discovery through machine learning. Developing an emergent property in the model to understand molecules would broaden the horizons for…

The fields of generative AI and transfer learning have experienced remarkable advancements in recent years especially in the domain of Natural Language Processing (NLP). Transformers have been at the heart of these advancements where the…

Computation and Language · Computer Science 2024-02-28 Majd Saleh , Stéphane Paquelet

Humans can learn structural properties about a word from minimal experience, and deploy their learned syntactic representations uniformly in different grammatical contexts. We assess the ability of modern neural language models to reproduce…

Computation and Language · Computer Science 2020-10-13 Ethan Wilcox , Peng Qian , Richard Futrell , Ryosuke Kohita , Roger Levy , Miguel Ballesteros

Transformers are effective and efficient at modeling complex relationships and learning patterns from structured data in many applications. The main aim of this paper is to propose and design NLAFormer, which is a transformer-based…

Numerical Analysis · Mathematics 2025-08-28 Zhantao Ma , Yihang Gao , Michael K. Ng

Deep learning has achieved remarkable success in learning representations for molecules, which is crucial for various biochemical applications, ranging from property prediction to drug design. However, training Deep Neural Networks (DNNs)…

Machine Learning · Computer Science 2023-04-28 Jun Xia , Yanqiao Zhu , Yuanqi Du , Stan Z. Li