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Spin defects in hexagonal boron nitride (hBN) are promising quantum systems for the design of flexible two-dimensional quantum sensing platforms. Here we rely on hBN crystals isotopically enriched with either $^{10}$B or $^{11}$B to…

Materials Science · Physics 2023-10-03 A. Haykal , R. Tanos , N. Minotto , A. Durand , F. Fabre , J. Li , J. H. Edgar , V. Ivady , A. Gali , T. Michel , A. Dréau , B. Gil , G. Cassabois , V. Jacques

Achieving long-range ferrimagnetic order in purely organic systems remains a major challenge in molecular magnetism. Here we report the synthesis and characterization of heterospin-coupling motifs, formed by covalently linking spin-1/2 and…

Mesoscale and Nanoscale Physics · Physics 2026-04-10 Elia Turco , Fupeng Wu , Annika Bernhardt , Nils Krane , Ji Ma , Roman Fasel , Michal Juriček , Xinliang Feng , Pascal Ruffieux

Measurements and modeling of electron spin transport and dynamics are used to characterize hyperfine interactions in Fe/GaAs devices with $n$-GaAs channels. Ga and As nuclei are polarized by electrically injected electron spins, and the…

Mesoscale and Nanoscale Physics · Physics 2015-05-14 M. K. Chan , Q. O. Hu , J. Zhang , T. Kondo , C. J. Palmstrøm , P. A. Crowell

Individual nuclear spin states can have very long lifetimes and could be useful as qubits. Progress in this direction was achieved on MgO/Ag(001) via detection of the hyperfine interaction (HFI) of Fe, Ti and Cu adatoms using scanning…

Mesoscale and Nanoscale Physics · Physics 2022-07-20 Sufyan Shehada , Manuel dos Santos Dias , Muayad Abusaa , Samir Lounis

[Background] Single-reference density functional theory is very successful in reproducing bulk nuclear properties like binding energies, radii, or quadrupole moments throughout the entire periodic table. Its extension to the multi-reference…

Nuclear Theory · Physics 2017-01-30 W. Satula , P. Baczyk , J. Dobaczewski , M. Konieczka

Precise characterization of a hyperfine interaction is a prerequisite for high fidelity manipulations of electron and nuclear spins belonging to a hybrid qubit register in diamond. Here, we demonstrate a novel scheme for determining a…

Quantum Physics · Physics 2013-09-11 J. H. Shim , B. Nowak , I. Niemeyer , J. Zhang , F. D. Brandao , D. Suter

Understanding the quantum dynamics of spin defects and their coherence properties requires accurate modeling of spin-spin interaction in solids and molecules, for example by using spin Hamiltonians with parameters obtained from…

Materials Science · Physics 2021-02-02 Krishnendu Ghosh , He Ma , Mykyta Onizhuk , Vikram Gavini , Giulia Galli

The formalism based on correlated basis functions and the cluster expansion technique has been recently employed to derive an effective interaction from a realistic nuclear hamiltonian. To gauge the reliability of this scheme, we perform a…

Nuclear Theory · Physics 2015-08-17 Angela Mecca , Alessandro Lovato , Omar Benhar , Artur Polls

Hyperfine interaction (HFI) in carbon nanotube and graphene quantum dots is due to the presence of 13C atoms. We theoretically show that in these structures the short-range nature of the HFI gives rise to a coupling between the valley…

Mesoscale and Nanoscale Physics · Physics 2009-11-27 András Pályi , Guido Burkard

Hyperfine-changing collisions are of fundamental interest for the studying of ultracold heteronuclear mixtures. Here, we report the state-to-state study of the hyperfine-changing-collision dynamics in a Bose-Fermi mixture of $^6$Li and…

Quantum Gases · Physics 2020-04-08 Xiao-Qiong Wang , Yu-Xuan Wang , Xiang-Pei Liu , Ran Qi , Xing-Can Yao , Yu-Ao Chen , Jian-Wei Pan

Ultra-cold alkali atoms trapped in two distinct hyperfine states in an external magnetic field can mimic magnetic systems of spin 1/2 particles. We describe the spin-dependent effective interaction as a spin-spin interaction. As a…

Statistical Mechanics · Physics 2011-11-09 D. H. Santamore , Eddy Timmermans

Molecular spin qubits with long spin coherence time as well as non-invasive operation methods on such qubits are in high demand. It was shown that both molecular electronic and nuclear spin levels can be used as qubits. In solid state…

Materials Science · Physics 2020-10-28 Robert L. Smith , Aleksander L. Wysocki , Kyungwha Park

The electronic and magnetic structures of $ {\rm ScFe_2} $ and of its dihydride $ {\rm ScFe_2H_2} $ are self-consistently calculated within the density functional theory (DFT) using the all electron augmented spherical wave (ASW) method…

Materials Science · Physics 2008-04-17 A. F. Al Alam , S. F. Matar , N. Ouaini , M. Nakhl

The transferred hyperfine interaction between nuclear and electron spins in an heavy fermion material depends on the hybridization between the $f$-electron orbitals and those surrounding a distant nucleus. In CeMIn$_5$ (M=Rh, Ir, Co), both…

Strongly Correlated Electrons · Physics 2021-08-04 P. Menegasso , J. C. Souza , I. Vinograd , Z. Wang , S. P. Edwards , P. G. Pagliuso , N. J. Curro , R. R. Urbano

We show how hydrogenation of graphene nanoribbons at small concentrations can open new venues towards carbon-based spintronics applications regardless of any especific edge termination or passivation of the nanoribbons. Density functional…

Mesoscale and Nanoscale Physics · Physics 2015-05-14 D. Soriano , F. Muñoz-Rojas , J. Fernández-Rossier , J. J. Palacios

The nitrogen-vacancy (NV) centers (NCVSi) - in 4H silicon carbide (SiC) constitute an ensemble of spin S = 1 solid state qubits interacting with the surrounding 14N and 29Si nuclei. As quantum applications based on a polarization transfer…

The study of state-to-state spin-exchange collisions in the vicinity of $p$-wave Feshbach resonances offer great opportunities to explore many-body interactions and novel quantum phases. Here, we report the observation of a spin-exchange…

Quantum Gases · Physics 2024-06-04 Shuai Peng , Tangqian Shu , Bowen Si , Sijia Peng , Yixin Guo , Yongchang Han , Jiaming Li , Gaoren Wang , Le Luo

Nuclear magnetic resonance (NMR) and transport measurements have been performed at high magnetic fields and low temperatures in a series of $n$-type Bi$_{2}$Se$_{3}$ crystals. In low density samples, a complete spin polarization of the…

The control of recently observed spintronic effects in topological-insulator/ferromagnetic-metal (TI/FM) heterostructures is thwarted by the lack of understanding of band structure and spin texture around their interfaces. Here we combine…

Mesoscale and Nanoscale Physics · Physics 2017-09-28 J. M. Marmolejo-Tejada , K. Dolui , P. Lazic , P. -H. Chang , S. Smidstrup , D. Stradi , K. Stokbro , B. K. Nikolic

Weakly interacting Fermi gases exhibit rich collective dynamics in spin-dependent potentials, arising from correlations between spin degrees of freedom and conserved single atom energies, offering broad prospects for simulating many-body…

Quantum Gases · Physics 2021-01-28 S. Pegahan , J. Kangara , I. Arakelyan , J. E. Thomas