Related papers: Intercombination line frequencies in $^{171}$Yb va…
Precise molecular transition frequencies are of great interest in the test of fundamental physics and also in various applications. Two well isolated ro-vibrational transitions of $^{12}$C$^{16}$O at 1.57 $\mu$m, R(9) and R(10) in the…
We demonstrate laser frequency stabilization with at least 6 GHz of offset tunability using an in-phase/quadrature (IQ) modulator to generate electronic sidebands (ESB) on a titanium sapphire laser at 714 nm and we apply this technique to…
An atom exposed to an electric field will experience Stark shifts of its internal energy levels, proportional to their polarizabilities. In optical frequency metrology, the Stark shift due to background black-body radiation (BBR) modifies…
We measure hyperfine structure in the metastable ${^3P}_2$ state of $^{173}$Yb and extract the nuclear magnetic octupole moment. We populate the state using dipole-allowed transitions through the ${^3P}_1$ and ${^3S}_1$ states. We measure…
Optical frequency combs are an essential tool for precision metrology experiments ranging in application from remote spectroscopic sensing of trace gases to the characterization and comparison of optical atomic clocks for precision…
We use a diode laser locked to a Rb transition as the frequency reference along with a scanning Michelson interferometer to make precise measurements on the $D_1$ and $D_2$ lines of potassium. The Rb reference frequency is known with…
The coherent interaction of solid-state spins with both optical and microwave fields provides a platform for a range of quantum technologies, such as quantum sensing, microwave-to-optical quantum transduction and optical quantum memories.…
We present a measurement of the absolute frequency of the 5s$^2$ $^1$S$_0$ to 5s5p $^3$P$_0$ transition in $^{87}$Sr, which is a secondary representation of the SI second. We describe the optical lattice clock apparatus used for the…
Hyperfine quenching rates of the lowest-energy metastable $^3P_0$ and $^3P_2$ states of Mg, Ca, Sr, and Yb atoms are computed. The calculations are carried out using ab initio relativistic many-body methods. The computed lifetimes may be…
We demonstrate a compact iodine-stabilized laser operating at 531 nm using a coin-sized light source consisting of a 1062-nm distributed-feedback diode laser and a frequency-doubling element. A hyperfine transition of molecular iodine is…
We present a spectroscopy scheme for the 7-kHz-wide 689-nm intercombination line of strontium. We rely on shelving detection, where electrons are first excited to a metastable state by the spectroscopy laser before their state is probed…
We report high-precision frequency ratio measurements between optical atomic clocks based on $^{27}$Al$^+$, $^{171}$Yb, and $^{87}$Sr. With total fractional uncertainties at or below $3.2 \times 10^{-18}$, these measurements meet an…
Historically, there has been a trade-off in spectroscopic measurements between high spectral resolution, broadband coverage, and acquisition time. Optical frequency combs, initially envisioned for precision spectroscopy of the hydrogen atom…
A two-step, two-color laser spectroscopy technique has been used to measure the hyperfine splittings of the $8p$ excited states in $^{203}$Tl and $^{205}$Tl, as well as the $7s - 8p$ transition isotope shifts. For the case of the $8p_{3/2}$…
Dissipative solitons formed in Kerr microresonators may enable chip-scale frequency combs for precision optical metrology. Here we explore the creation of an octave-spanning, 15-GHz repetition-rate microcomb suitable for both f-2f…
We demonstrate the use of trapped ytterbium ions as quantum bits for quantum information processing. We implement fast, efficient state preparation and state detection of the first-order magnetic field-insensitive hyperfine levels of…
We report measurements of absolute transition frequencies and hyperfine coupling constants for the 8S_{1/2}, 9S_{1/2}, 7D_{3/2}, and 7D_{5/2} states in ^{133}Cs vapor. The stepwise excitation through either the 6P_{1/2} or 6P_{3/2}…
We report the upgrade and operation of a frequency-comb-assisted high-resolution mid-infrared molecular spectrometer allowing us to combine high spectral purity, SI-traceability, wide tunability and high sensitivity. An optical frequency…
Absolute transition frequencies of the $2s\,^2{\rm{S}}_{1/2}$ $\rightarrow$ $2p\,^2{\rm{P}}_{1/2,3/2}$ transitions in Be$^+$ were measured with a frequency comb in stable and short-lived isotopes at ISOLDE (CERN) using collinear laser…
A measurement of the hyperfine coefficients and isotope shifts for the Dy I 421.291 nm transition [$4f^{10}6s^2 (J=8)\to4f^{10}6s6p (J=9)$] using atomic beam laser-induced fluorescence spectroscopy is presented. A King Plot analysis is…