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Zircaloy-4 is used extensively as nuclear fuel cladding materials and hydride embrittlement is a major failure mechanism. To explore the effect of {\delta}-hydride on plastic deformation and performance of Zircaloy-4, in situ high angular…

Materials Science · Physics 2019-03-28 Siyang Wang , Szilvia Kalácska , Xavier Maeder , Johann Michler , Finn Giuliani , T. Ben Britton

The long-term safety of water-based nuclear reactors relies in part on the reliability of zirconium-based nuclear fuel. Yet the progressive ingress of hydrogen during service makes zirconium alloys subject to delayed hydride cracking. Here,…

Microstructure and crystallography of {\delta} phase hydrides in as-received fine grain and 'blocky' alpha large grain Zircaloy-4 (average grain size ~11 {\mu}m and >200 {\mu}m, respectively) were examined using electron backscatter…

Materials Science · Physics 2019-09-04 Siyang Wang , Finn Giuliani , T. Ben Britton

The interaction of hydrogen and metals continues to be industrially relevant and is a critical part of creating and supporting a safety case for nuclear reactor operation. In the present work, we explore hydrogen storage and hydride…

Materials Science · Physics 2021-09-24 Wenjun Lu , Paraskevas Kontis , Siyang Wang , Ruth Birch , Mark Wenman , Baptiste Gault , T. Ben Britton

The interactions between {\delta}-hydrides and plastic slip in a commercial zirconium alloy, Zircaloy-4, under stress were studied using in situ secondary electron microscope (SEM) micropillar compression tests of single crystal samples and…

Materials Science · Physics 2020-08-17 Siyang Wang , Finn Giuliani , T. Ben Britton

Microstructural analysis with electron backscatter diffraction (EBSD) involves sectioning and polishing to create a flat and preparation-artifact free surface. The quality of EBSD analysis is often dependant on this step, and this motivates…

Materials Science · Physics 2022-03-31 Ning Fang , Ruth Birch , T. Ben Britton

Zirconium alloys are used as nuclear fuel cladding material due to their mechanical and corrosion resistant properties together with their favorable cross-section for neutron scattering. At running conditions, however, there will be an…

Materials Science · Physics 2017-10-25 Jakob Blomqvist , Johan Olofsson , Anna-Maria Alvarez , Christina Bjerkén

Zircaloy-4 (Zr-1.5%Sn-0.2%Fe-0.1%Cr wt. %) was electrochemically charged with deuterium to create deuterides and subsequently analysed with atom probe tomography and scanning transmission electron microscopy to understand zirconium hydride…

High-energy synchrotron X-ray diffraction was utilized to study the mechanical response of the f.c.c $\delta$-hydride phase, the intermetallic precipitation with hexagonal C14 lave phase and the $\alpha$-Zr phase in the Zircaloy-4 materials…

Materials Science · Physics 2016-04-20 Jun-li Lin , Xiaochun Han , Brent J. Heuser , Jonathan D. Almer

One of the main degradation mechanisms of the zirconium alloys used in nuclear reactors is hydrogen embrittlement and hydride formation. The formation of zirconium hydrides is accompanied by a transformation strain, the effects of which on…

Materials Science · Physics 2023-09-28 Masoud Taherijam , Saiedeh Marashi , Alireza Tondro , Hamidreza Abdolvand

We explore the distribution, morphology and structure of zirconium hydrides formed using different cooling rates through the solid state Zr+[H] --> Zr + hydride transus, in fine and blocky alpha Zircaloy-4. We observe that cooling rate and…

Materials Science · Physics 2018-12-05 Ruth Birch , Siyang Wang , Vivian Tong , Thomas Benjamin Britton

Zirconium alloys are widely used in the nuclear industry because of their high strength, good corrosion resistance and low neutron absorption cross-section. However, zirconium has strong affinity for hydrogen which leads to hydrogen…

Materials Science · Physics 2014-08-21 T. Maimaitiyili , A. Steuwer , J. Blomquist , B. Matthew , Z. Olivier , J. Andrieux , C. Bjerken , R. Fabienne

Zirconium alloys are widely used in nuclear reactors as fuel cladding materials. Fuel cladding is used to contain the nuclear fuel and cladding tubes are typically sealed using welds. Welding of zirconium alloys can result in changes in the…

Materials Science · Physics 2024-02-28 Ruth M. Birch , T. Ben Britton

A recently developed full field level-set model of continuous dynamic recrystallization is applied to simulate zircaloy-4 recrystallization during hot compression and subsequent heat treatment. The influence of strain rate, final strain and…

Materials Science · Physics 2023-04-21 Victor Grand , Baptiste Flipon , Alexis Gaillac , Marc Bernacki

The fabrication of bulk delta-phase Zirconium Hydride ($\delta$-ZrH) using Zircaloy-4 as a precursor is herein reported. Characterization using electron-microscopy methods indicate that the fabricated material is of a single-phase. Sn-rich…

Materials Science · Physics 2024-01-30 D. Parkison , M. A. Tunes , T. J. Nizolek , T. A. Saleh , P. Hosemann , C. A. Kohnert

We used by in-situ high energy X-ray diffraction to inestigate the deformation behavior of Grade 2 commercially pure titanium that was hydrogen charged to form hydrides. The results showed that the peak broadening in the diffraction…

Materials Science · Physics 2022-01-26 Qing Tan , Zhiran Yan , Runguang Li , Yang Ren , Yandong Wang , Baptiste Gault , Stoichko Antonov

Analysis of distortions of the crystal lattice within individual mineral grains is central to the investigation of microscale processes that control and record tectonic events. These distortions are generally combinations of lattice…

Materials Science · Physics 2019-06-04 David Wallis , Lars N. Hansen , T. Ben Britton , Angus J. Wilkinson

For high (angular) resolution electron backscatter diffraction (HR-EBSD), the selection of a reference diffraction pattern (EBSP0) significantly affects the precision of the calculated strain and rotation maps. This effect was demonstrated…

Materials Science · Physics 2023-02-21 Abdalrhaman Koko , Vivian Tong , Angus J. Wilkinson , T. James Marrow

Hafnium hydride is a promising material for next-generation nuclear reactors, particularly as control rods for fast fission and shielding in fusion systems. The material's intrinsic brittleness encourages its use in the form of…

Materials Science · Physics 2026-03-17 Di Wang , Catriona M McGilvery , James O Douglas , Siyang Wang

Understanding deformation in polycrystalline metals is critical to use them in high-value high-risk applications. We present in-situ characterisation of plastic deformation of zirconium, a hexagonal closed packed (HCP), metal. Analysis of…

Materials Science · Physics 2019-10-11 Vivian Tong , Euan Wielewski , Ben Britton
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