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For fast and accurate calculations of band gaps of solids, we present an {\it ab initio} method that extends the density functional theory plus on-site Hubbard interaction (DFT+$U$) to include inter-site Hubbard interaction ($V$). This…

Materials Science · Physics 2021-01-14 Sang-Hoon Lee , Young-Woo Son

Computational screening for new and improved catalyst materials relies on accurate and low-cost predictions of key parameters such as adsorption energies. Here, we use recently developed compressed sensing methods to identify descriptors…

Materials Science · Physics 2019-02-21 Mie Andersen , Sergey V. Levchenko , Matthias Scheffler , Karsten Reuter

The selection rules of high harmonic generation (HHG) are investigated using three-dimensional time-dependent density functional theory (TDDFT). From the harmonic spectra obtained with various real molecules and different forms of laser…

Atomic Physics · Physics 2016-09-28 Xi Liu , Xiaosong Zhu , Liang Li , Yang Li , Qingbin Zhang , Pengfei Lan , Peixiang Lu

We present an efficient method for incorporating the dynamical effects of the screening of the Hubbard U by electronic degrees of freedom in the solid into the single site dynamical mean field approximation. The formalism is illustrated by…

Strongly Correlated Electrons · Physics 2010-04-08 Philipp Werner , Andrew J. Millis

A central problem in systems biology is to identify parameter values such that a biological model satisfies some behavioral constraints (\eg, time series). In this paper we focus on parameter synthesis for hybrid (continuous/discrete)…

Logic in Computer Science · Computer Science 2014-09-11 Bing Liu , Soonho Kong , Sicun Gao , Paolo Zuliani , Edmund M. Clarke

Accurate prediction for the electronic structure properties of halide perovskites plays a significant role in the design of highly efficient and stable solar cells. While density functional theory (DFT) within the generalized gradient…

Chemical Physics · Physics 2023-06-27 Qi Ou , Ping Tuo , Wenfei Li , Xiaoxu Wang , Yixiao Chen , Linfeng Zhang

We generalize the Bergman-Milton spectral representation, originally derived for a two-component composite, to extract the spectral density function for the effective dielectric constant of a graded composite. This work has been motivated…

Soft Condensed Matter · Physics 2007-05-23 L. Dong , Mikko Karttunen , K. W. Yu

Two-dimensional (2D) hexagonal boron nitride (BN) nanosheets are excellent dielectric substrate for graphene, molybdenum disulfide and many other 2D nanomaterials based electronic and photonic devices. To optimize the performance of these…

Palladium diselenide (PdSe$_2$) -- a layered van der Waals material -- is attracting significant attention for optoelectronics due to the wide tunability of its band gap from the infrared through the visible range as a function of the…

The screening problem for the Coulomb potential of a charge located in a two-dimensional (2D) system has an intriguing solution with a power law distance screening factor due to out-of-plane electrical fields. This is crucially different…

Mesoscale and Nanoscale Physics · Physics 2024-09-10 K. A. Baryshnikov , A. V. Gert , Yu. B. Vasilyev , A. P. Dmitriev

Recently, two nonempirical hybrid functionals, dielectric-dependent range-separated hybrid functional based on the Coulomb-attenuating method (DD-RSH-CAM) and doubly screened hybrid functional (DSH), have been suggested by [Chen et al,…

Materials Science · Physics 2020-01-08 Peitao Liu , Cesare Franchini , Martijn Marsman , Georg Kresse

Quantum chemistry methods exploiting density-functional approximations for short-range electron-electron interactions and second-order M{{\o}}ller-Plesset (MP2) perturbation theory for long-range electron-electron interactions have been…

We explore quantitative descriptors that herald when a many-particle system in $d$-dimensional Euclidean space $\mathbb{R}^d$ approaches a hyperuniform state as a function of the relevant control parameter. We establish quantitative…

Soft Condensed Matter · Physics 2021-05-26 Salvatore Torquato

The nucleus-nucleus potential is calculated in the frame work of the double folding model (DFM) to obtain the Coulomb barrier parameters (barrier position and height), starting from M3Y-Reid nucleon-nucleon interaction and realistic nuclear…

Nuclear Theory · Physics 2020-01-22 M. Ismail , A. Y. Ellithi , A. Adel , A. R. Abdulghany

Density matrix embedding theory (DMET) [Phys. Rev. Lett., 109, 186404 (2012)], introduced a new approach to quantum cluster embedding methods, whereby the mapping of strongly correlated bulk problems to an impurity with finite set of bath…

Strongly Correlated Electrons · Physics 2015-06-24 George H. Booth , Garnet Kin-Lic Chan

The dynamic Friedel sum rule (FSR) is derived within the second-order Born (B2) approximation for an ion that moves in a fully degenerate electron gas and for an arbitrary spherically-symmetric electron-ion interaction potential. This…

Other Condensed Matter · Physics 2015-12-09 Hrachya B. Nersisyan , José M. Fernández-Varea , Néstor R. Arista

Range separated hybrid density functionals are very successful in describing a wide range of molecular and solid state properties accurately. Range separated hybrid functionals are designed from spherically averaged or system averaged…

Materials Science · Physics 2017-12-15 Subrata Jana , Prasanjit Samal

Density functional theory (DFT) embedding provides a formally exact framework for interfacing correlated wave-function theory (WFT) methods with lower-level descriptions of electronic structure. Here, we report techniques to improve the…

Chemical Physics · Physics 2015-06-12 Jason D. Goodpaster , Taylor A. Barnes , Frederick R. Manby , Thomas F. Miller

In our article we report first quantitative measurements of imaging performance for the current generation of hybrid pixel detector, Medipix3, as direct electron detector. Utilising beam energies of 60 & 80 keV, measurements of modulation…

We consider the effect of interactions on the line shape of the two-photon 1s-2s transition in a (doubly) spin-polarized atomic hydrogen gas in terms of the interatomic interaction potentials. We show that the frequency-weighted sum rule…

Statistical Mechanics · Physics 2014-10-13 C. J. Pethick , H. T. C. Stoof
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