Related papers: Nonlinear dynamics of molecular superrotors
We present a method to design a finite decay rate for excited rotational states in polar molecules. The setup is based on a hybrid system of polar molecules with atoms driven into a Rydberg state. The atoms and molecules are coupled via the…
We present a theoretical study of the rotational dynamics of asymmetry top molecules in an electric field and a parallel non-resonant linearly polarized laser pulse. The time-dependent Schr\"odinger equation is solved within the rigid rotor…
We investigate the steady states of a lossy array of nonlinear optical resonators that are driven by lasers and interact via mutual photon tunneling. For weak nonlinearities, we find two-mode squeezing of polaritons in modes whose…
Orientation states of two coupled polar molecules controlled by laser pulses are studied theoretically. By varying the period of a series of periodically applied laser pulse, transition from regular to chaotic behavior may occur. Schmidt…
Laser excitation of nanometer-sized atomic and molecular clusters offers various opportunities to explore and control ultrafast many-particle dynamics. Whereas weak laser fields allow the analysis of photoionization, excited-state…
We theoretically consider the phenomenon of field-free long-lasting orientation of symmetric-top molecules ionized by two-color laser pulses. The anisotropic ionization produces a significant long-lasting orientation of the surviving…
A new mode of effective interaction of molecular rotational degrees of freedom with an intense, nonresonant, ultrashort laser pulse is explored. Transient nonadiabatic charge redistribution (TNCR) in larger molecules or molecular ions…
A theoretical study of the rotational dynamics of a linear polar molecule in a two-color non-resonant cw laser field is presented. By systematically considering the interactions of this field with the electric dipole moment, polarizability…
The field of attosecond science was first enabled by nonlinear compression of intense laser pulses to a duration below two optical cycles. Twenty years later, creating such short pulses still requires state-of-the-art few-cycle laser…
Depending on its adsorption conformation on the Au(111) surface, a zwitterionic single-molecule machine works in two different ways under bias voltage pulses. It is a unidirectional rotor while anchored on the surface. It is a fast-drivable…
We consider deflection of polarizable molecules by inhomogeneous optical fields, and analyze the role of molecular orientation and rotation in the scattering process. It is shown that molecular rotation induces spectacular rainbow-like…
We discuss the influence of periodic orbits on the dissociation of a model diatomic molecule driven by a strong bichromatic laser fields. Through the stability of periodic orbits we analyze the dissociation probability when parameters like…
Adding spin-polarized carriers to semiconductor lasers strongly changes their properties and, through the transfer of angular momentum, leads to the emission of circularly polarized light. In such spin-lasers, the polarization of the…
The possibility of realizing the superradiant regime of electromagnetic emission by the assembly of quantum dots is considered. The overall dynamical process is analyzed in detail. It is shown that there can occur several qualitatively…
We analyze the dynamics of a solid-state laser driven by an injected sinusoidal field. For this type of laser, the cavity round-trip time is much shorter than its fluorescence time, yielding a dimensionless ratio of time scales $\sigma \ll…
An ab initio simulation of strong-field photodissociation of diatomic molecules was developed, inspired by recent dissociation experiments of F2-. The transition between electronic states was modeled, including the laser pulse and…
We discuss harmonic generation in the case of laser field-dressed Hamiltonians that are invariant under so-called dynamical symmetry operations. Examples for such systems are molecules which exhibit a discrete rotational symmetry of order N…
Resonant optical excitation of lowest-energy excitonic transitions in self-assembled quantum dots lead to nuclear spin polarization that is qualitatively different from the well known optical orientation phenomena. By carrying out a…
We solve the superradiant laser model in two limiting cases. First the stationary low-pumping regime is considered where a first-order phase transition in the semiclassical solution occurs. This discontinuity is smeared out in the quantum…
We report the experimental observation of superradiant emission emanating from an elongated dense ensemble of laser cooled two-level atoms, with a radial extent smaller than the transition wavelength. In the presence of a strong driving…