Related papers: Time-resolved single-particle x-ray scattering rev…
We present a method to locally probe spatially varying chemical composition of soft matter systems by use of optically controlled and elastically self-assembled plasmonic nanoantennae. Disc-shaped metal particles with sharp irregular edges…
Quantum material systems upon applying ultrashort laser pulses provide a rich platform to access excited material phases and their transformations that are not entirely like their equilibrium counterparts. The addressability and potential…
For over a century, x-ray scattering has been the most powerful tool for determining the equilibrium structure of crystalline materials. Deviations from perfect periodicity, for example due to thermal motion of the atoms, reduces the…
We report on experiments that quantify the role of a central electronic spin as a relaxation source for nuclear spins in its nanoscale environment. Our strategy exploits hyperpolarization injection from the electron as a means to…
Attosecond streaking of photoelectrons emitted by extreme ultraviolet light has begun to reveal how electrons behave during their transport within simple crystalline solids. Many sample types within nanoplasmonics, thin-film physics, and…
Free-electron laser hard X-ray light sources can provide high fluence, femtosecond pulses, enabling the time-resolved probing of structural dynamics and elementary relaxation processes in molecules. Traditional X-ray elastic scattering from…
The impulsive phase of a solar flare is known to generate strong turbulence and to transfer magnetic energy into accelerated electrons. Recognizing the importance of angular diffusion on the dynamics of the accelerated electrons, we extend…
We analyze ultrafast electron dynamics in the time domain upon optical excitation of propagating surface plasmon-polaritons (SPs) in metal-dielectric heterostructures. Developing a kinetic model where both local and non-local electron…
Motivated by recent experimental findings for an organic superconductor, charge oscillations that emerge after a strong pulse of an oscillating electric field is applied are studied in electron systems in a superconducting phase on a…
We experimentally demonstrate spatiotemporal steering of photoelectron emission in multiphoton above-threshold single ionization of atoms exposed to a phase-controlled orthogonally polarized two-color (OTC) laser pulse. Spatial and energy…
Single-molecule surface enhanced Raman scattering (SM-SERS) is one of the vital applications of plasmonic nanoparticles. The SM-SERS sensitivity critically depends on plasmonic hot-spots created at the vicinity of such nanoparticles. In…
Polaritons are quasiparticles arising from the strong coupling of electromagnetic waves in cavities and dipolar oscillations in a material medium. In this framework, localized surface plasmon in metallic nanoparticles defining optical…
In this article, we introduce a new viewpoint on electromagnetic scattering. Tailoring spectral electromagnetic response underpins important applications ranging from sensing to energy conversion, and is flourishing with new ideas from…
The irradiation of an atomic cluster with a femtosecond x-ray free-electron laser pulse results in a nanoplasma formation. This typically occurs within a few hundreds femtoseconds. By this time the x-ray pulse is over, and the direct…
We propose a framework to explore the internal charge distribution of mesoscopic quasiparticles by inelastic x-ray scattering, while also accounting for the conventional scattering from electrons. Specifically, we investigate a new…
Molecular iodine was photoexcited by a strong 800 nm laser, driving several channels of multiphoton excitation. The motion following photoexcitation was probed using time-resolved X-ray scattering, which produces a scattering map…
Tremendous enhancement of light-matter interaction in plasmon-excited molecular hybrid devices allows for non-linearities on the level of single emitters and few photons. This promises a plethora of novel applications like single photon…
The role of kinetic electrons in the excitation and sustainment of ion-bulk electrostatic waves in collisionless plasmas is investigated, with a focus on the physical mechanisms responsible for the generation of small-scale structures in…
Plasmon-exciton polaritons provide exciting possibilities to control light-matter interactions at the nanoscale by enabling closer investigation of quantum optical effects and facilitating novel technologies based, for instance, on…
Terahertz time domain spectroscopy employing free-space radiation has frequently been used to probe the elementary excitations of low-dimensional systems. The diffraction limit blocks its use for the in-plane study of individual laterally…