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We investigated the thermal transport properties of two $\alpha$-RuCl$_3$ crystals with different degrees of stacking disorder to understand the origin of the previously reported oscillatory feature in the field dependence of thermal…

Materials Science · Physics 2024-01-17 Heda Zhang , Andrew May , Hu Miao , Brian Sales , David Mandrus , Stephen Nagler , Michael McGuire , Jiaqiang Yan

The layered honeycomb magnet $\alpha$-RuCl$_3$ has emerged as a promising candidate for realizing a Kitaev quantum spin liquid. Previous studies have reported oscillation-like anomalies in the longitudinal thermal conductivity and…

Strongly Correlated Electrons · Physics 2025-04-01 Y. Xing , R. Namba , K. Imamura , K. Ishihara , S. Suetsugu , T. Asaba , K. Hashimoto , T. Shibauchi , Y. Matsuda , Y. Kasahara

In the study of van der Waals-layered magnetic materials, the properties of CrCl$_3$ continue to attract attention. This compound is reported to undergo antiferromagnetic (AFM) ordering below $\sim$14 K, with a ferromagneticlike region…

Materials Science · Physics 2024-11-13 John A. Schneeloch , Adam A. Aczel , Feng Ye , Despina Louca

The van der Waals layered magnet $\alpha$-RuCl$_3$ offers tantalizing prospects for the realization of Majorana quasiparticles. Efforts to understand this are, however, hampered by inconsistent magnetic and thermal transport properties…

Single crystals of the Kitaev spin-liquid candidate $\alpha$-RuCl$_3$ have been studied to determine low-temperature bulk properties, structure and the magnetic ground state. Refinements of x-ray diffraction data show that the low…

Strongly Correlated Electrons · Physics 2016-04-27 H. B. Cao , A. Banerjee , J. -Q. Yan , C. A. Bridges , M. D. Lumsden , D. G. Mandrus , D. A. Tennant , B. C. Chakoumakos , S. E. Nagler

The layered transition metal trihalide $\alpha$-RuCl$_3$ has been studied extensively in recent years as a promising candidate for a proximate Kitaev quantum spin liquid state. In high quality samples, a complete structural transition from…

Materials Science · Physics 2026-01-05 Paige Harford , Ezekiel Horsley , Subin Kim , Young-June Kim

$\alpha$-RuCl$_3$ is a candidate Kitaev material that exhibits zigzag antiferromagnetic ordering below 7 K. One contentious issue regarding this material is its bulk structure in the low-temperature phase. Recently, it has become generally…

Materials Science · Physics 2026-01-27 Seung-Ju Hong , Tae Yun Kim , Cheol-Hwan Park

We present out-of-plane dielectric and magnetodielectric measurements of single crystallines $\alpha$-RuCl$_3$ with various degrees of stack faults. A frequency dependent, but field independent, dielectric anomaly appears at…

Recently, there have been increasingly hot debates on whether there exists a quantum spin liquid in the Kitaev honeycomb magnet $\alpha$-RuCl$_3$ in high magnetic field. To investigate this issue, we perform the ultralow-temperature thermal…

Strongly Correlated Electrons · Physics 2018-02-14 Y. J. Yu , Y. Xu , K. J. Ran , J. M. Ni , Y. Y. Huang , J. H. Wang , J. S. Wen , S. Y. Li

Thermal transport has been used to probe the nature of $\alpha$-RuCl$_3$, an important candidate of Kitaev material. Two remarkable observations were made under applied magnetic fields at low temperatures, and have stimulated extensive…

Strongly Correlated Electrons · Physics 2026-03-17 Zheng-Duo Fan , Xiao-Qi Sun , Jing-Yuan Chen

We study on transport and magnetic properties of hydrated and lithium-intercalated $\alpha$-RuCl$_3$, Li$_x$RuCl$_3 \cdot y$H$_2$O, for investigating the effect on mobile-carrier doping into candidate materials for a realization of a Kitaev…

Strongly Correlated Electrons · Physics 2019-06-26 Yoshinori Imai , Katsuya Konno , Yoshinao Hasegawa , Takuya Aoyama , Kenya Ohgushi

We report X-ray diffraction and magnetic susceptibility studies of the structural phase transition in $\alpha$-RuCl$_{3}$. By utilizing a single crystal sample with predominantly single twin domain, we show that $\alpha$-RuCl$_{3}$ goes…

Strongly Correlated Electrons · Physics 2023-11-08 Subin Kim , Ezekiel Horsley , Jacob P. C. Ruff , Beatriz D. Moreno , Young-June Kim

CrCl3 is a layered insulator that undergoes a crystallographic phase transition below room temperature and orders antiferromagnetically at low temperature. Weak van der Waals bonding between the layers and ferromagnetic in-plane magnetic…

The material $\alpha$-RuCl$_3$ has been the subject of intense scrutiny as a potential Kitaev quantum spin liquid, predicted to display Majorana fermions as low energy excitations. In practice, $\alpha$-RuCl$_3$ undergoes a transition to a…

$\alpha$-RuCl$_3$ is considered to be the top candidate material for the experimental realization of the celebrated Kitaev model. It is however known that additional interactions beyond the Kitaev model trigger in $\alpha$-RuCl$_3$, a…

Insulating Nb$_3$Cl$_8$ is a layered chloride consisting of two-dimensional triangular layers of $S_{eff}$ = 1/2 Nb$_3$Cl$_{13}$ clusters at room temperature. Magnetic susceptibility measurement show a sharp, hysteretic drop to a…

Strongly Correlated Electrons · Physics 2017-01-20 J. P. Sheckelton , K. W. Plumb , B. A. Trump , C. L. Broholm , T. M. McQueen

Lithium and sodium are the only solids that are known to lose crystalline order upon cooling. The seemingly-disordered low-temperature phase shows signatures of various close-packed structures. The lack of order has been attributed to a…

Mesoscale and Nanoscale Physics · Physics 2026-02-24 C. M. Wilson , R. Ganesh , K. V. Samokhin

We have investigated the longitudinal thermal conductivity of $\alpha$-RuCl$_{3}$, the magnetic state of which is considered to be proximate to a Kitaev honeycomb model, along with the spin susceptibility and magnetic specific heat. We…

Strongly Correlated Electrons · Physics 2017-06-28 Daichi Hirobe , Masahiro Sato , Yuki Shiomi , Hidekazu Tanaka , Eiji Saitoh

In the class of materials called spin liquids, a magnetically ordered state cannot be attained even at milliKelvin temperatures because of conflicting constraints on each spin (for e.g. from geometric or exchange frustration). The resulting…

The honeycomb Kitaev model in a magnetic field is a source of a topological quantum spin liquid with Majorana fermions and gauge flux excitations as fractional quasiparticles. We present experimental results for the thermal Hall effect of…

Strongly Correlated Electrons · Physics 2019-03-06 Richard Hentrich , Maria Roslova , Anna Isaeva , Thomas Doert , Wolfram Brenig , Bernd Büchner , Christian Hess
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