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Molecular dynamics simulations have been extensively used to predict thermal properties, but simulating different phases with similar precision using a unified force field is often difficult, due to the lack of accurate and transferrable…

Materials Science · Physics 2019-12-12 Ruiyang Li , Eungkyu Lee , Tengfei Luo

Liquid water exhibits several important anomalous properties in the vicinity of the melting temperature ($T_{\mathrm{m}}$) of ice Ih, including a higher density than ice and a density maximum at 4~$^{\circ}$C. Experimentally, an isotope…

Chemical Physics · Physics 2026-01-01 Yifan Li , Bingjia Yang , Chunyi Zhang , Axel Gomez , Pinchen Xie , Yixiao Chen , Pablo M. Piaggi , Roberto Car

The $\text{Cu}_7\text{P}\text{S}_6$ compound has garnered significant attention due to its potential in thermoelectric applications. In this study, we introduce a neuroevolution potential (NEP), trained on a dataset generated from ab initio…

Materials Science · Physics 2024-11-19 Junlan Liu , Qian Yin , Mengshu He , Jun Zhou

We demonstrate how deep convolutional neural networks can be trained to predict 2+1 D hydrodynamic simulation results for flow coefficients, mean-transverse-momentum and charged particle multiplicity from the initial energy density profile.…

High Energy Physics - Phenomenology · Physics 2024-04-04 H. Hirvonen , K. J. Eskola , H. Niemi

We show that the centroid molecular dynamics (CMD) method provides a realistic way to calculate the thermal diffusivity $a=\lambda/\rho c_{\rm V}$ of a quantum mechanical liquid such as para-hydrogen. Once $a$ has been calculated, the…

Chemical Physics · Physics 2021-05-10 Benjamin J. Sutherland , William H. D. Moore , David. E. Manolopoulos

We herein present a first-principles formulation of the Green-Kubo method that allows the accurate assessment of the non-radiative thermal conductivity of solid semiconductors and insulators in equilibrium ab initio molecular dynamics…

Materials Science · Physics 2017-05-03 Christian Carbogno , Rampi Ramprasad , Matthias Scheffler

Accurately simulating the properties of liquid water remains a central challenge in molecular simulations. In this work, we use machine learning potentials to investigate how the convergence settings of electronic structure calculations…

Chemical Physics · Physics 2026-03-24 Hubert Beck , Ondrej Marsalek

The application of a temperature gradient to an extended system generates an electromotive force that induces an electric current in conductors and a macroscopic polarization in insulators. The ratio of the electromotive force to the…

Materials Science · Physics 2024-02-01 Enrico Drigo , Stefano Baroni

We compute the thermal conductivity of water within linear response theory from equilibrium molecular dynamics simulations, by adopting two different approaches. In one, the potential energy surface (PES) is derived on the fly from the…

Materials Science · Physics 2021-12-24 Davide Tisi , Linfeng Zhang , Riccardo Bertossa , Han Wang , Roberto Car , Stefano Baroni

Given the unique optical properties of LiF, it is often used as an observation window in high-temperature and pressure experiments; and, hence, estimates of its transmission properties are necessary to interpret observations. Since direct…

Materials Science · Physics 2016-07-27 R. E. Jones , D. K. Ward

Quantitative prediction of thermodynamic properties in solution is essential for translating atomistic simulations into reliable chemical insight. As an exemplar system, the behaviour of CaCO$_3$ in water has been widely studied to…

When two phases of water are at equilibrium, the ratio of hydrogen isotopes in each is slightly altered due to their different phase affinities. This isotopic fractionation process can be utilized to analyze water's movement in the world's…

Chemical Physics · Physics 2013-07-30 Thomas E. Markland , B. J. Berne

Boiling heat transfer occurs in many situations and can be used for thermal management in various engineered systems with high energy density, from power electronics to heat exchangers in power plants and nuclear reactors. Essentially,…

Computational Engineering, Finance, and Science · Computer Science 2018-09-26 Yang Liu , Nam Dinh , Yohei Sato , Bojan Niceno

The use of deep learning methods for modeling fluid flow has drawn a lot of attention in the past few years. In situations where conventional numerical approaches can be computationally expensive, these techniques have shown promise in…

Critical heat flux is a key quantity in boiling system modeling due to its impact on heat transfer and component temperature and performance. This study investigates the development and validation of an uncertainty-aware hybrid modeling…

Machine Learning · Computer Science 2025-07-17 Aidan Furlong , Xingang Zhao , Robert Salko , Xu Wu

Recently there have been significant theoretical advances in our understanding of liquids and dense supercritical fluids based on their ability to support high frequency transverse (shear) waves. Here, we have constructed a new computer…

Soft Condensed Matter · Physics 2020-10-14 John E. Proctor

We investigate how the normal energy transport is realized in one-dimensional quantum systems using a quantum spin system. The direct investigation of local energy distribution under thermal gradient is made using the quantum master…

Chaotic Dynamics · Physics 2009-11-07 Keiji Saito

Understanding the relationship between the structure of light-harvesting systems and their excitation energy transfer properties is of fundamental importance in many applications including the development of next generation photovoltaics.…

Chemical Physics · Physics 2017-07-21 Florian Häse , Christoph Kreisbeck , Alán Aspuru-Guzik

We present Q-AMOEBA (CF), an enhanced version of the Q-AMOEBA polarizable model that integrates a geometry-dependent charge flux (CF) term while designed for an explicit treatment of nuclear quantum effects (NQE). The inclusion of CF…

Chemical Physics · Physics 2025-06-05 Nastasia Mauger , Thomas Plé , Louis Lagardère , Simon Huppert , Jean-Philip Piquemal

Hydrofluoroolefins are considered the most promising next-generation refrigerants due to their extremely low global warming potential values, which can effectively mitigate the global warming effect. However, the lack of reliable…

Machine Learning · Computer Science 2025-07-30 Gang Wang , Peng Hu