Related papers: Efficient Pathway to NaCs Ground State Molecules
Large-scale fault-tolerant superconducting quantum computation needs rapid quantum communication to network qubits fabricated on different chips and long-range couplers to implement efficient quantum error-correction codes. Quantum channels…
A scanning tunneling microscope is used to generate the electroluminescence of phthalocyanine molecules deposited on NaCl/Ag(111). Photon spectra reveal an intense emission line at 1.9 eV that corresponds to the fluorescence of the…
We have successfully prepared an optically trapped ultracold mixture of $^{23}$Na and $^{87}$Rb atoms and studied their interspecies Feshbach resonances. Using two different spin combinations, several s-wave and p-wave resonances are…
Adiabatic manipulation of the quantum state is an essential tool in modern quantum information processing. Here we demonstrate the speed-up of the adiabatic population transfer in a three-level superconducting transmon circuit by…
Acquiring quantitative information on charge transfer (CT) dynamics at the nanoscale remains an important scientific challenge. In particular, CT processes in single molecules at surfaces needs to be investigated to be properly controlled…
Using an ultracold gas of $^{87}$Rb$^{133}$Cs molecules, we perform hyperfine-resolved spectroscopy of transitions from the vibronic ground state to the lowest rovibrational states of the electronic state $\mathrm{b}\,^3\Pi_0$, as a…
We demonstrate a versatile, rotational-state dependent trapping scheme for the ground and first excited rotational states of $^{23}$Na$^{40}$K molecules. Close to the rotational manifold of a narrow electronic transition, we determine…
Robust stimulated Raman exact passages are requisite for controlling nonlinear quantum systems, with the wide applications ranging from ultracold molecules, non-linear optics to superchemistry. Inspired by shortcuts to adiabaticity, we…
We perform two-photon photoassociation spectroscopy of the heteronuclear CsYb molecule to measure the binding energies of near-threshold vibrational levels of the $X~^{2}\Sigma_{1/2}^{+}$ molecular ground state. We report results for…
We generalize the idea of chainwise stimulated Raman adiabatic passage (STIRAP) [Kuznetsova \textit{et al.} Phys. Rev. A \textbf{78}, 021402(R) (2008)] to a photoassociation-based chainwise atom-molecule system, with the goal of directly…
We produce an ultracold and dense sample of rovibronic ground state Cs_2 molecules close to the regime of quantum degeneracy, in a single hyperfine level, in the presence of an optical lattice. The molecules are individually trapped, in the…
We demonstrate the direct formation of vibronic ground state RbCs molecules by photoassociation of ultracold atoms followed by radiative stabilization. The photoassociation proceeds through deeply-bound levels of the (2)^{3}\Pi_{0^{+}}…
We present precision measurements with MHz uncertainty of the energy gap between asymptotic and well bound levels in the electronic ground state X $^1\Sigma_{\mathrm{g}}^+$ of the $^{39}$K$_2$ molecule. The molecules are prepared in a…
Since Purcell's seminal report 75 years ago, electromagnetic resonators have been used to control light-matter interactions to make brighter radiation sources and unleash unprecedented control over quantum states of light and matter.…
We report adiabatic passage experiments with a single trapped $^{40}$Ca$^+$ ion. By applying a frequency chirped laser pulse with a Gaussian amplitude envelope we reach a transfer efficiency of 0.990(10) on an optical transition from the…
We propose an improved photoassociation scheme to produce ultracold molecules in their vibronic ground state for the generic case where non-adiabatic effects facilitating transfer to deeply bound levels are absent. Formation of molecules is…
We demonstrate the formation of a single NaCs molecule in an optical tweezer by magnetoassociation through an s-wave Feshbach resonance at 864.11(5)G. Starting from single atoms cooled to their motional ground states, we achieve conversion…
Precise control over rotational angular momentum is at the heart of recent advances in quantum chemistry, quantum simulation, and quantum computation with ultracold bialkali molecules. Each rotational state comprises a rich manifold of…
Using numerical simulations of two-photon electronic absorption with femtosecond pulses in Na$_2$ we show that: i) it is possible to avoid the characteristic saturation or dumped Rabi oscillations in the yield of absorption by time-delaying…
The B^1\Pi <- X^1\Sigma^+ system of NaCs molecule is investigated experimentally by polarization labelling spectroscopy technique. The inverted perturbation approach method is used to construct the potential energy curve of the B^1\Pi…