Related papers: Efficient Pathway to NaCs Ground State Molecules
We investigated transition strengths from ultracold weakly bound 41K87Rb molecules produced via the photoassociation of laser-cooled atoms. An accurate potential energy curve of the excited state (3)1Sigma+ was constructed by carrying out…
We produce ${^{84}\mathrm{Sr}_2}$ molecules using Bose-enhanced Raman photoassociation. We apply the stimulated Raman adiabatic passage (STIRAP) technique on a Bose-Einstein condensate (BEC) to produce more than $8 \times 10^3$ ultracold…
Achieving a high population of antihydrogen/hydrogen atoms in the 2S level is essential for spectroscopy measurements testing similarities between matter and antimatter. We propose and examine the efficiency of applying the STIRAP…
Subwavelength ring-shaped structures of quantum emitters exhibit outstanding radiation properties and are useful for antennas, excitation transport, and storage. Taking inspiration from the oligomeric geometry of biological light-harvesting…
Astrophysical modeling of processes in environments that are not in local thermal equilibrium requires the knowledge of state-to-state rate coefficients of rovibrational transitions in molecular collisions. These rate coefficients can be…
Quantum emitters with a $\Lambda$-type level structure enable numerous protocols and applications in quantum science and technology. Understanding and controlling their dynamics is, therefore, one of the central research topics in quantum…
The technique of stimulated Raman adiabatic passage (STIRAP), which allows efficient and selective population transfer between quantum states without suffering loss due to spontaneous emission, was introduced in 1990 (Gaubatz \emph{et al.},…
We experimentally demonstrate transitions between electronic angular momentum states with a difference in magnetic quantum numbers $\Delta \mathrm{m_J} = $ 3, 4, and 5 via resonant four- and six-photon stimulated Raman transitions in a…
Coherent manipulation of quantum states is of crucial importance in accurate control of a quantum system. A fundamental goal is coherently transferring the population of a desired state with near-unit fidelity. For this propose, we…
Starting from an ultracold sample of ground-state $^{23}$Na$^{87}$Rb molecules, we investigate the lowest ro-vibrational level of the $b^3\Pi$ state with high resolution laser spectroscopy. This electronic spin-forbidden $X^1\Sigma^+…
By two-color photoassociation of $^{40}$Ca four weakly bound vibrational levels in the Ca$_2$ \Xpot ground state potential were measured, using highly spin-forbidden transitions to intermediate states of the coupled system $^3\Pi_{u}$ and…
Polar molecules in selected quantum states can be guided, decelerated, and trapped using electric fields created by microstructured electrodes on a chip. Here we explore how transitions between two of these quantum states can be induced…
We demonstrate a new spectroscopic method for studying electronic transitions in molecules with extremely broad range of angular momentum. We employ an optical centrifuge to create narrow rotational wave packets in the ground electronic…
With a microwave-regime cyclic three-state configuration, an enantiomer-selective state transfer~(ESST) is carried out through the two-path interference between a direct one-photon coupling and an effective two-photon coupling. The…
Efficient preparation and detection of the motional state of trapped ions is important in many experiments ranging from quantum computation to precision spectroscopy. We investigate the stimulated Raman adiabatic passage (STIRAP) technique…
We describe a quantum information architecture consisting of a hybrid array of optically-trapped molecules and atoms. This design leverages the large transition dipole moments of Rydberg atoms to mediate fast, high-fidelity gates between…
We report on scanning tunneling microscopy (STM) topographs of individual metal phthalocyanines (MPc) on a thin salt (NaCl) film on a gold substrate, at tunneling energies within the molecule's electronic transport gap. Theoretical models…
We propose a two-qubit gate based on dipolar exchange interactions between individually addressable ultracold polar molecules in an array of optical dipole traps. Our proposal treats the full Hamiltonian of the $^1\Sigma^+$ molecule NaCs,…
We have investigated rovibronic levels of the strongly mixed $b^3\Pi_1-c^3\Sigma^+_1-B^1\Pi_1$ states [the 2(1), 3(1), and 4(1) states in Hund's case (c) notation] of $^{85}$Rb$^{133}$Cs in the energy range of 13950$-$14200 cm$^{-1}$ using…
The stimulated Raman adiabatic passage (STIRAP) shows an efficient technique that accurately transfers population between two discrete quantum states with the same parity, in three-level quantum systems based on adiabatic evolution. This…