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This thesis investigates the mechanically controlled break junctions, with a particular emphasis on elucidating the behaviour of molecular currents at room temperature. The core of this experimental investigation involves a detailed…

Mesoscale and Nanoscale Physics · Physics 2024-09-17 Giovanna Angelis Schmidt

Metallic atomic junctions pose the ultimate limit to the scaling of electrical contacts. They serve as model systems to probe electrical and thermal transport down to the atomic level as well as quantum effects occurring in one-dimensional…

Mesoscale and Nanoscale Physics · Physics 2017-05-24 Nico Mosso , Ute Drechsler , Fabian Menges , Peter Nirmalraj , Siegfried Karg , Heike Riel , Bernd Gotsmann

Temperature ($T$) dependent conductance $G = G(T)$ data measured in molecular junctions are routinely taken as evidence for a two-step hopping mechanism. The present paper emphasizes that this is not necessarily the case. A curve of $\ln G$…

Mesoscale and Nanoscale Physics · Physics 2022-12-01 Ioan Baldea

Extensive studies on thin films indicated a generic cubic current-voltage $I-V$ dependence as a salient feature of charge transport by tunneling. A quick glance at $I-V$ data for molecular junctions suggests a qualitatively similar…

Chemical Physics · Physics 2015-09-21 Ioan Baldea

The temperature dependence of the I-V characteristics of many single-electron tunneling devices enable thermometer operation of these systems. We investigate two normal conducting kinds of them, {\sl (a)} a single junction in a…

Condensed Matter · Physics 2007-05-23 H. -O. Müller , A. Hädicke , W. Krech

We investigate how temperature affects transport through large networks of nonlinear conductances with distributed thresholds. In monolayers of weakly-coupled gold nanocrystals, quenched charge disorder produces a range of local thresholds…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Raghuveer Parthasarathy , Xiao-Min Lin , Klara Elteto , T. F. Rosenbaum , Heinrich M. Jaeger

{Analytical equations like Richardson-Dushman's or Shockley's provided a general, if simplified conceptual background, which was widely accepted in conventional electronics and made a fundamental contribution to advances in the field. In…

Mesoscale and Nanoscale Physics · Physics 2023-12-12 Ioan Baldea

The energy dependent thermoelectric response of a single molecule contains valuable information about its transmission function and its excited states. However, measuring it requires devices that can efficiently heat up one side of the…

The resonant tunneling model is the simplest model for describing electronic transport through nanoscale objects like individual molecules. A complete understanding includes not only charge transport but also thermal transport and their…

Mesoscale and Nanoscale Physics · Physics 2021-01-25 Matthias A. Popp , André Erpenbeck , Heiko B. Weber

Understanding how the mechanism of charge transport through molecular tunnel junctions depends on temperature is crucial to control electronic function in molecular electronic devices. With just a few systems investigated as a function of…

Mesoscale and Nanoscale Physics · Physics 2016-05-27 Alvar R. Garrigues , Lejia Wang , Enrique del Barco , Christian A. Nijhuis

Charge and heat transport through a single molecule tunnel-coupled to external normal electrodes have been studied. The molecule with sufficiently strong interaction between lectrons and vibrational internal degrees of freedom can be…

Mesoscale and Nanoscale Physics · Physics 2012-04-16 Karol Izydor Wysokinski

To develop next-generation electronics and high efficiency energy-harvesting devices, it is crucial to understand how charge and heat are transported at the nanoscale. Metallic atomic-size contacts are ideal systems to probe the quantum…

Mesoscale and Nanoscale Physics · Physics 2019-05-01 Nico Mosso , Alyssa Prasmusinto , Andrea Gemma , Ute Drechsler , Lukas Novotny , Bernd Gotsmann

We consider interaction effects in a granular normal metal at not very low temperatures. Assuming that all weak localization effects are suppressed by the temperature we replace the initial Hamiltonian by a proper functional of phases and…

Disordered Systems and Neural Networks · Physics 2009-11-07 K. B. Efetov , A. Tschersich

Thermal conductance of single molecular junctions at room temperature has been measured recently using picowatt-resolution scanning probes. However, fully understanding thermal transport in a much wider temperature range is needed for the…

Mesoscale and Nanoscale Physics · Physics 2022-02-15 Gen Li , Bing-Zhong Hu , Nuo Yang , Jing-Tao Lü

The tunneling conductance is calculated as a function of the gate voltage in wide temperature range for the single quantum dot systems with Coulomb interaction. We assume that two orbitals are active for the tunneling process. We show that…

Strongly Correlated Electrons · Physics 2009-10-31 Wataru Izumida , Osamu Sakai , Yukihiro Shimizu

Temperature dependence of the tunnel magnetoresistance (TMR) was calculated in range of the quantum-ballistic model in the magnetic tunnel junctions (MTJs) with embedded nanoparticles (NPs). The electron tunnel transport through NP was…

Mesoscale and Nanoscale Physics · Physics 2016-03-28 Arthur Useinov , Chih-Huang Lai

The statistical properties of the conductance of one dimensional disordered systems are studied at finite bias voltage V and temperature T, in an independent-electron picture. We calculate the complete distribution of the conductance P(G)…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Victor A. Gopar , Peter Woelfle

We investigate transport in a granular metallic system at large tunneling conductance between the grains, $g_T\gg 1$. We show that at low temperatures, $T\leq g_T\delta $, where $\delta$ is the single mean energy level spacing in a grain,…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 I. S. Beloborodov , K. B. Efetov , A. V. Lopatin , V. M. Vinokur

We present measurements of the electrical conductance $G$ at room temperature of mechanically controllable break junctions (MCBJ) fabricated from Au in different solvents (octane, DCM, DMSO, and toluene) and compare with measurements in air…

Mesoscale and Nanoscale Physics · Physics 2016-08-16 L. Grüter , M. T. González , R. Huber , M. Calame , C. Schönenberger

Interlayer tunneling measurements in the strongly correlated bilayer quantized Hall phase at $\nu_T=1$ are reported. The maximum, or critical current for tunneling at $\nu_T=1$, is shown to be a well-defined global property of the coherent…

Strongly Correlated Electrons · Physics 2013-10-22 D. Nandi , T. Khaire , A. D. K. Finck , J. P. Eisenstein , L. N. Pfeiffer , K. W. West
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