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Ultrafast laser measurements probe the non-equilibrium dynamics of excited electrons in metals with increasing temporal resolution. Electronic structure calculations can provide a detailed microscopic understanding of hot electron dynamics,…

Computational Physics · Physics 2016-08-12 Ana M. Brown , Ravishankar Sundararaman , Prineha Narang , William A. Goddard , Harry A. Atwater

We study the nonequilibrium dynamics of photoinduced phase transitions in charge ordered (CO) systems with a strong electron-lattice interaction and analyze the interplay between electrons, periodic lattice distortions, and a phonon thermal…

Strongly Correlated Electrons · Physics 2018-03-22 Linghua Zhu , Tsezar F. Seman , Michel van Veenendaal , Keun Hyuk Ahn

The physical mechanism for metal ablation induced by femtosecond laser irradiation was investigated. Results of calculations based on finite-temperature density functional theory (FTDFT) indicate that condensed copper becomes unstable at…

Materials Science · Physics 2018-04-04 Yuta Tanaka , Shinji Tsuneyuki

We combine femtosecond electron diffuse scattering experiments and first-principles calculations of the coupled electron-phonon dynamics to provide a detailed momentum-resolved picture of the ultrafast lattice thermalization in a thin film…

The atomistic resolution recently achieved by ultrafast spectroscopies demands corresponding theoretical advances. Real-time time-dependent density-functional theory (RT-TDDFT) with Ehrenfest dynamics offers an optimal trade-off between…

Materials Science · Physics 2022-10-19 Jannis Krumland , Matheus Jacobs , Caterina Cocchi

We present an exact Monte Carlo method to simulate the nonequilibrium dynamics of electron-phonon models in the adiabatic limit of zero phonon frequency. The classical nature of the phonons allows us to sample the equilibrium phonon…

Strongly Correlated Electrons · Physics 2022-02-16 Manuel Weber , James K. Freericks

We investigate the effects of acceleration during non-linear electron-beam relaxation in magnetized plasma in the case of electron transport in solar flares. The evolution of electron distribution functions is computed using a…

Solar and Stellar Astrophysics · Physics 2015-06-05 M. Karlicky , E. P. Kontar

The ultrafast dynamics of ions in solids following intense femtosecond laser excitation is governed by two fundamentally distinct yet interplaying effects. On one hand, the significant generation of hot electron-hole pairs by the light…

Computational Physics · Physics 2024-01-22 Bernd Bauerhenne , Martin E. Garcia

Thermal instability in an electron-ion magnetized plasma, which is relevant in the intragalactic medium (IGM) of galaxy clusters, solar corona, and other two-component plasma objects is investigated. We apply the multicomponent plasma…

Astrophysics of Galaxies · Physics 2015-05-28 Anatoly K. Nekrasov

We investigate electron correlation effects in internuclear-distance-dependent enhanced ionization of $\mathrm{H}_2$, $\mathrm{LiH}$, and $\mathrm{HF}$ molecules by intense near-infrared laser pulses using a 3D description of the systems…

Atomic Physics · Physics 2019-02-27 Siddhartha Chattopadhyay , Lars Bojer Madsen

We investigate the laser-induced dynamics of electronically driven charge-density-wave order. A comprehensive mean-field analysis of the attractive Hubbard model in the weak-coupling regime reveals ultrafast switching and ultrafast melting…

Strongly Correlated Electrons · Physics 2018-04-25 Michael Schüler , Yuta Murakami , Philipp Werner

We present a comprehensive investigation of nonequilibrium effects and self heating in single electron transfer devices based primarily on the Coulomb blockade effect. During an electron trapping process, a hot electron may be deposited in…

Condensed Matter · Physics 2008-02-03 Chiu Liu , Qian Niu

The accurate treatment of electronic effects in multi-million atom simulations of radiation-induced collision cascades is crucial for reliable predictions of primary radiation damage. In this work, we explore the performance of a recently…

Materials Science · Physics 2024-01-10 Andrea E. Sand , Glen P. Kiely , Artur Tamm , Alfredo A. Correa

We study the transient photoluminescence (PL) of photoexcited metals by solving the Boltzmann equation considering the effects of electron-electron (e-e) and electron-phonon (e-ph) collisions, where the e-ph coupling function is calculated…

Materials Science · Physics 2020-07-29 Shota Ono , Tohru Suemoto

Photoexcited hot carriers in solids can drive processes, such as photocatalytic reactions on the surface, beyond those available in thermal equilibrium. Hot-electron-mediated reaction pathways are limited by the thermalization of the…

Materials Science · Physics 2026-04-13 Christopher Seibel , Tobias Held , Markus Uehlein , Baerbel Rethfeld

We study the electron-acoustic instabilities in plasmas with two kappa-distributed electrons and stationary ions. The instabilities are driven by the relative drift between two electron components. The suprathermal effects of different…

Plasma Physics · Physics 2023-12-08 Ran Guo

In this work we study the effects of nonadiabatic external driving on the thermodynamics of an electronic system coupled to two electronic leads and to a phonon mode, with and without damping. In the limit of slow driving, we establish…

Statistical Mechanics · Physics 2022-06-03 Jakob Bätge , Amikam Levy , Wenjie Dou , Michael Thoss

We investigate an exact nonequilibrium solution of a two-site electron-phonon model, where an infrared-active phonon that is nonlinearly coupled to the electrons is driven by a laser field. The time-resolved electronic spectrum shows…

Strongly Correlated Electrons · Physics 2017-05-10 M. A. Sentef

X-ray laser-induced structural changes in silicon undergoing femtosecond melting have been investigated by using an x-ray pump-x-ray probe technique. The experimental results for different initial sample temperatures reveal that the onset…

Ultrafast light-matter interaction is a powerful tool for the study of solids. Upon laser excitation, carrier multiplication and lattice acceleration beyond thermal velocity can occur, as a result of far-from-equilibrium carrier relaxation.…

Materials Science · Physics 2019-01-04 Chao Lian , S. B. Zhang , Sheng Meng
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