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It is widely believed that the breakdown of the Stokes-Einstein (SE) relation between the translational diffusivity and the shear viscosity in supercooled liquids is due to the development of dynamic heterogeneity i.e. the presence of both…

Statistical Mechanics · Physics 2015-06-12 Shiladitya Sengupta , Smarajit Karmakar

Stokes-Einstein (SE) relation, which relates diffusion constant with the viscosity of a liquid at high temperatures in equilibrium, is violated in the supercooled temperature regime. Whether this relation is obeyed in nonequilibrium active…

Soft Condensed Matter · Physics 2023-06-21 Anoop Mutneja , Smarajit Karmakar

The Stokes-Einstein (SE) relation between the self-diffusion and shear viscosity coefficients operates in sufficiently dense liquids not too far from the liquid-solid phase transition. By considering four simple model systems with very…

Soft Condensed Matter · Physics 2021-10-27 Sergey Khrapak , Alexey Khrapak

The theories of Brownian motion, the Debye rotational diffusion model, and hydrodynamics together provide us with the Stokes--Einstein--Debye (SED) relation between the rotational relaxation time of the $\ell$-th degree Legendre polynomials…

Soft Condensed Matter · Physics 2019-06-03 Takeshi Kawasaki , Kang Kim

The description of molecular motion by macroscopic hydrodynamics has a long and continuing history. The Stokes-Einstein relation between the diffusion coefficient of a solute and the solvent viscosity predicted using macroscopic continuum…

Disordered Systems and Neural Networks · Physics 2007-05-23 Xiaoyu Xia , Peter G. Wolynes

Molecular Dynamics simulations of high density hard sphere fluids clearly show a breakdown of the Stokes-Einstein equation (SE). This result has been conjectured to be due to the presence of mobile particles, i.e., ones which have the…

Materials Science · Physics 2009-11-11 Sanat K. Kumar , Grzegorz Szamel , Jack F. Douglas

The Stokes-Einstein (SE) relation has been widely applied to quantitatively describe the Brownian motion. Notwithstanding, here we show that even for a simple fluid, the SE relation may not be completely applicable. Namely, although the SE…

Statistical Mechanics · Physics 2021-03-17 Hanqing Zhao , Hong Zhao

We investigate the origin of the breakdown of the Stokes-Einstein relation (SER) between diffusivity and viscosity in undercooled melts. A binary Lennard-Jones system, as a model for a metallic melt, is studied by molecular dynamics. A weak…

Disordered Systems and Neural Networks · Physics 2016-06-22 H. R. Schober , H. L. Peng

The Stokes-Einstein relation, relating the diffusion and viscosity coefficients D and eta, is tested in two dimensions. An equilibrium molecular-dynamics simulation was used with a Yukawa pair potential. Regimes are identified where motion…

Soft Condensed Matter · Physics 2009-11-11 Bin Liu , J. Goree

The Stokes-Einstein relation for the self-diffusion coefficient of a spherical particle suspended in an incompressible fluid is an asymptotic result in the limit of large Schmidt number, that is, when momentum diffuses much faster than the…

Soft Condensed Matter · Physics 2015-06-17 F. Balboa Usabiaga , X. Xie , R. Delgado-Buscalioni , A. Donev

We study the motion of a tracer particle injected in facilitated models which are used to model supercooled liquids in the vicinity of the glass transition. We consider the East model, FA1f model and a more general class of non-cooperative…

Statistical Mechanics · Physics 2015-06-16 Oriane Blondel , Cristina Toninelli

In this Research Note the Zwanzig's formulation of the Stokes-Einstein (SE) relation for simple atomistic fluids is re-examined. It is shown that the value of the coefficient in SE relation depends on the ratio of the transverse and…

Soft Condensed Matter · Physics 2020-04-22 Sergey Khrapak

We investigate the dynamical properties of liquid and supercooled liquid silicon, modeled using the Stillinger-Weber (SW) potential, to examine the validity of the Stokes-Einstein (SE) relation. Towards this end, we examine the relationship…

Materials Science · Physics 2025-03-25 Himani Rautela , Shiladitya Sengupta , Vishwas V. Vasisht

Molecular dynamics simulations have been performed on TIP4P/2005 supercooled water to investigate the molecular diffusion and shear viscosity at various timescales and assess the Stokes-Einstein (SE) and Stokes-Einstein-Debye (SED)…

Soft Condensed Matter · Physics 2019-08-12 Takeshi Kawasaki , Kang Kim

The celebrated Stokes Law (SL) of hydrodynamics predicts that the velocity of a particle pulled through a liquid by an external force, Fex, is directly proportional to the force and inversely proportional to the friction {\zeta} acted by…

Soft Condensed Matter · Physics 2024-02-27 Subhajit Acharya , Biman Bagchi

The violation of Stokes--Einstein (SE) relation $D\sim (\eta/T)^{-1}$ between the shear viscosity $\eta$ and the translational diffusion constant $D$ at temperature $T$ is of great importance for characterizing anomalous dynamics of…

Soft Condensed Matter · Physics 2017-08-22 Takeshi Kawasaki , Kang Kim

Diffusion coefficients are key thermophysical properties for modeling mass transport in liquids, but experimental data are scarce, making reliable prediction methods indispensable. In the present work, we introduce a new method for…

Molecular dynamics simulations are performed on a system of model linear polymers to look at the violations of Stokes-Einstein (SE) and Stokes-Einstein-Debye (SED) relations near the mode coupling theory transition temperature $T_c$ at…

Soft Condensed Matter · Physics 2020-11-10 Jalim Singh , Prasanth P. Jose

This work derives the Navier--Stokes hydrodynamic equations for a model of a confined, quasi-two-dimensional, $s$-component mixture of inelastic, smooth, hard spheres. Using the inelastic version of the revised Enskog theory, macroscopic…

Soft Condensed Matter · Physics 2026-03-27 David González Méndez , Vicente Garzó

The Stokes-Einstein relation (SER) is one of the most robust and widely employed results from the theory of liquids. Yet sizable deviations can be observed for self-solvation, which cannot be explained by the standard hydrodynamic…

Statistical Mechanics · Physics 2018-06-15 Benoit Charbonneau , Patrick Charbonneau , Grzegorz Szamel
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