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We study lithium systems over a range of number of atoms, e.g., atomic anion, dimer, metallic cluster, and body-centered cubic crystal by the diffusion Monte Carlo method. The calculations include both core and valence electrons in order to…

Computational Physics · Physics 2015-07-29 Kevin Rasch , Lubos Mitas

The sum-of-squares method can give rigorous lower bounds on the energy of quantum Hamiltonians. Unfortunately, typically using this method requires solving a semidefinite program, which can be computationally expensive. Further, the…

Quantum Physics · Physics 2024-12-05 M. B. Hastings

Quantum chemical methods dealing with challenging systems while retaining low computational costs have attracted attention. In particular, many efforts have been devoted to developing new methods based on the second-order perturbation that…

Chemical Physics · Physics 2023-10-30 Nhan Tri Tran , Hoang Thanh Nguyen , Lan Nguyen Tran

The Short-Time approximation is a method introduced to evaluate electroweak nuclear response for systems with $A\geq12$, extending the reach of first-principle many-body Quantum Monte Carlo calculations. Using realistic two- and three-body…

A comprehensive assessment of theoretical uncertainties defines an important frontier in nuclear structure research. Ideally, theory predictions include uncertainty estimates that take into account truncation effects from both the…

Nuclear Theory · Physics 2026-02-23 Isak Svensson , Alexander Tichai , Kai Hebeler , Achim Schwenk

We analyze the baryon mass differences up to second order in chiral perturbation theory, including the effects of decuplet intermediate states. We show that the Coleman--Glashow relation has computable corrections of order $(m_d - m_u)…

High Energy Physics - Phenomenology · Physics 2009-10-28 Richard F. Lebed , Markus A. Luty

We present the first nucleon-nucleon potential at next-to-next-to-next-to-leading order (fourth order) of chiral perturbation theory. Charge-dependence is included up to next-to-leading order of the isospin-violation scheme. The accuracy…

Nuclear Theory · Physics 2009-11-10 D. R. Entem , R. Machleidt

We present variational Monte Carlo calculations of the neutron matter equation of state using chiral nuclear forces. The ground-state wavefunction of neutron matter, containing non-perturbative many-body correlations, is obtained from…

Nuclear Theory · Physics 2014-11-06 G. Wlazłowski , J. W. Holt , S. Moroz , A. Bulgac , K. J. Roche

A new general approach is introduced for definining an optimum zero-order Hamiltonian for Rayleigh-Schr\"odinger perturbation theory. Instead of taking the operator directly from a model problem, it is constructed to be a best fit to the…

Quantum Physics · Physics 2021-12-09 Peter J. Knowles

We explore the possibility of calculating electronic excited states by using perturbation theory along a range-separated adiabatic connection. Starting from the energies of a partially interacting Hamiltonian, a first-order correction is…

Chemical Physics · Physics 2014-12-15 Elisa Rebolini , Julien Toulouse , Andrew M. Teale , Trygve Helgaker , Andreas Savin

Quantum Monte Carlo methods are powerful numerical tools to accurately solve the Schr\"odinger equation for nuclear systems, a necessary step to describe the structure and reactions of nuclei and nucleonic matter starting from realistic…

Nuclear Theory · Physics 2020-05-01 Stefano Gandolfi , Diego Lonardoni , Alessandro Lovato , Maria Piarulli

Auxiliary-field quantum Monte Carlo methods enable the calculation of thermal and ground state properties of correlated quantum many-body systems in model spaces that are many orders of magnitude larger than those that can be treated by…

Nuclear Theory · Physics 2019-07-29 Y. Alhassid

The diffusion quantum Monte Carlo method is extended to solve the old theoretical physics problem of many-electron atoms and ions in intense magnetic fields. The feature of our approach is the use of adiabatic approximation wave functions…

Quantum Physics · Physics 2009-11-13 S. Bucheler , D. Engel , J. Main , G. Wunner

In order to solve the A-body Schr\"odinger equation both accurately and efficiently for open-shell nuclei, a novel many-body method coined as Bogoliubov many-body perturbation theory (BMBPT) was recently formalized and applied at low…

Nuclear Theory · Physics 2020-12-10 Pepijn Demol , Mikael Frosini , Alexander Tichai , Vittorio Somà , Thomas Duguet

Effects of geometrical frustration and quantum fluctuation are theoretically investigated for the proton ordering in a quasi-two-dimensional hydrogen-bonded system, squaric acid crystal. We elucidate the phase diagram for an effective…

Strongly Correlated Electrons · Physics 2015-03-19 Hiroaki Ishizuka , Yukitoshi Motome , Nobuo Furukawa , Sei Suzuki

We present an algebraic, nondiagrammatic derivation of finite-temperature second-order many-body perturbation theory [FT-MBPT(2)], using techniques and concepts accessible to theoretical chemical physicists. We give explicit expressions not…

Chemical Physics · Physics 2016-09-05 Robin Santra , Jochen Schirmer

We report successful implementation of the time-dependent second-order many-body perturbation theory using optimized orthonormal orbital functions called time-dependent optimized second-order many-body perturbation theory [TD-OMP2] to reach…

Chemical Physics · Physics 2020-08-26 Himadri Pathak , Takeshi Sato , Kenichi L. Ishikawa

In this paper we present an evolution of our derivation of the shell-model effective Hamiltonian, namely introducing effects of three-body contributions. More precisely, we consider a three-body potential at next-to-next-to-leading order in…

Nuclear Theory · Physics 2018-10-10 T. Fukui , L. De Angelis , Y. Z. Ma , L. Coraggio , A. Gargano , N. Itaco , F. R. Xu

A strong effort will be dedicated in the coming years to extend the reach of ab initio nuclear-structure calculations to heavy doubly open-shell nuclei. In order to do so, the most efficient strategies to incorporate dominant many-body…

We predict neutron-proton scattering cross-sections and polarization observables up to next-to-next-to-next-to leading order in a renormalization-group invariant description of the strong nucleon-nucleon interaction. Low-energy constants…

Nuclear Theory · Physics 2024-06-12 Oliver Thim , Andreas Ekström , Christian Forssén
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