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We demonstrate how the technique of ultrafast resonant x-ray scattering can be applied to imaging dynamics of electronic wave packets in crystals. We study scattering patterns from crystals with electron dynamics in valence bands taking…

Optics · Physics 2018-12-11 Daria Popova-Gorelova , Robin Santra

Interference terms between monopole and quadrupole Coulomb form factors that contribute to the cross-section of electron scattering from polarized nuclei are studied within the plane wave Born approximation. By experimentally exploring the…

Nuclear Theory · Physics 2024-02-14 Pedro Sarriguren

We report a joint experimental and theoretical study using a combination of polarization-controlled free-electron-laser (FEL) and near-infra\-red (NIR) pulses in a synchronized two-color photo\-ionization scheme. Excited He$^+$ ions,…

We present an approach for initiating and tracing ultra-fast electron dynamics in core-excited atoms, molecules and solids. The approach is based on stimulated resonant inelastic x-ray scattering induced by a single, chirped, broadband…

Atomic Physics · Physics 2019-01-23 Maximilian Hollstein , Nina Rohringer

Compton scattering is the nonresonant inelastic scattering of an x-ray photon by an electron and has been used to probe the electron momentum distribution in gas-phase and condensed-matter samples. In the low x-ray intensity regime, Compton…

Atomic Physics · Physics 2017-02-16 Sang-Kil Son , Otfried Geffert , Robin Santra

The laser-induced fragmentation dynamics of this most fundamental polar molecule HeH$^+$ are measured using an ion beam of helium hydride and an isotopologue at various wavelengths and intensities. In contrast to the prevailing…

Chemical Physics · Physics 2018-08-21 P. Wustelt , F. Oppermann , Lun Yue , M. Möller , T. Stöhlker , S. Gräfe , M. Lein , G. G. Paulus , A. M. Sayler

The development of intense high-energy radiation sources and the improvement of techniques for detecting charged fragments have made possible experiments on multiple ionization of a molecule with registration of the momentum and charge of…

We demonstrate an all-optical method for controlling the transverse motion of ionization injected electron beam, by utilizing the transversely asymmetrical wakefield via adjusting the shape of the laser focal spot. When the laser spot shape…

The radiative electron capture (REC) into the K shell of bare Xe ions colliding with a hydrogen gas target has been investigated. In this study, the degree of linear polarization of the K-REC radiation was measured and compared with…

We derive the photoionisation cross section in dipole approximation for many-electron atoms and ions for neutron star magnetic field strengths in the range of 10^7 to 10^9 T. Both bound and continuum states are treated in adiabatic…

Atomic Physics · Physics 2013-08-08 Thorsten Kersting , Damir Zajec , Peter Diemand , Günter Wunner

We use a Wigner distribution-like function based on the strong field approximation theory to obtain the time-energy distributions and the ionization time distributions of electrons ionized by an XUV pulse alone and in the presence of an…

Atomic Physics · Physics 2021-09-01 L. Guo , Y. Jia , M. Q. Liu , X. Y. Jia , S. L. Hu , R. H. Lu , S. S. Han , J. Chen

We investigate molecular dynamics of multiple ionization in N2 through multiple core-level photoabsorption and subsequent Auger decay processes induced by intense, short X-ray free electron laser pulses. The timing dynamics of the…

We report measurements of electron-impact excitation cross sections for the strong K-shell n=2-1 transitions in S XV using the LLNL EBIT-I electron beam ion trap, two crystal spectrometers, and the EBIT Calorimeter Spectrometer. The cross…

Intense X-ray photo-absorption from short and intense pulses by a molecule triggers complicated electron and subsequently ion dynamics leading to photo-electron spectra which are difficult to interpret. Illuminating fullerenes offers a way…

Atomic and Molecular Clusters · Physics 2014-08-20 Abraham Camacho Garibay , Ulf Saalmann , Jan M. Rost

A one parameter expression for the single ionization cross-section of atoms by electron impact is presented. Using this expression, the agreement obtained with available experimental data for 45 elements (from ionization threshold up to 200…

Atomic Physics · Physics 2007-05-23 B. Tsipinyuk , A. Bekkerman , E. Kolodney

The single ionization of noble gas atoms by the combined action of XUV attopulses and an infrared laser field is theoretically investigated by means of a non-perturbative model that under certain approximations gives closed-form expressions…

Atomic Physics · Physics 2015-12-21 D. I. R. Boll , O. A. Fojón

A theoretical study of the intense-field single ionization of molecular hydrogen or deuterium oriented either parallel or perpendicular to a linear polarized laser pulse (400 nm) is performed for different internuclear separations and pulse…

Quantum Physics · Physics 2015-05-14 Yulian V. Vanne , Alejandro Saenz

In many astrophysical objects an account for scattering of the X-ray fluorescent and resonance lines of iron ions by the electrons, bound in atomic and molecular hydrogen is important. Specific distortions of the scattered line profile…

Astrophysics · Physics 2007-05-23 R. Sunyaev , E. Churazov

We explore the laser-induced ionization dynamics of N2 and CO2 molecules subjected to a few-cycle, linearly polarized, 800\,nm laser pulse using effective two-dimensional single active electron time-dependent quantum simulations. We show…

Atomic Physics · Physics 2012-10-02 Michel Peters , Tung Nguyen-Dang , Eric Charron , Arne Keller , Osman Atabek

We theoretically study how time- and angle-resolved photoemission spectroscopy can be applied for imaging coherent electron dynamics in molecules. We consider a process in which a pump pulse triggers coherent electronic dynamics in a…

Optics · Physics 2018-12-11 Daria Popova-Gorelova , Jochen Küpper , Robin Santra