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Boron-based clathrate materials, typically with three-dimensional networks of B atoms, have tunable properties through substitution of guest atoms, but the tuning of B cages themselves has not yet been developed. By combining crystal…

Materials Science · Physics 2021-12-08 Liang Ma , Xin Yang , Guangtao Liu , Hanyu Liu , Guochun Yang , Hui Wang , Jinqun Cai , Mi Zhou , Hongbo Wang

The two-dimensional polymer structure and lattice dynamics of the superionic conductor Li4 C60 are investigated by neutron diffraction and spectroscopy. The peculiar bonding architecture of this compound is definitely confirmed through the…

We apply the density functional theory for superconductors (SCDFT) based on the local-density approximation (LDA) to alkali-doped fullerides A3C60 with the face-centered cubic structure. We evaluate the superconducting transition…

Superconductivity · Physics 2013-08-23 Ryosuke Akashi , Ryotaro Arita

The compressed hydrogen-rich compounds have received extensive attention as promising candidates for room temperature superconductivity, however, the high pressure required to stabilize such materials hinders their wide practical…

Superconductivity · Physics 2023-11-14 Wendi Zhao , Defang Duan , Decheng An , Qiwen Jiang , Zhengtao Liu , Tiancheng Ma , Zihao Huo , Jianhui Du , Tian Cui

The alkali-doped fulleride Cs$_{3}$C$_{60}$, crystallized in the space group Fm$\overline 3$m or Pm$\overline 3$n, exhibits unconventional $s$-wave superconductivity under pressure with a maximum $T_c\sim 38$ K. Recently, a new…

Superconductivity · Physics 2024-03-08 Changming Yue , Yusuke Nomura , Kosmas Prassides , Philipp Werner

The structure of the material responsible for the room temperature and near ambient pressure superconductivity reported in an N-doped lutetium hydride [Nature, 615, 244 (2023)] has not been conclusively determined. Herein, density…

Superconductivity · Physics 2023-08-09 Katerina P. Hilleke , Xiaoyu Wang , Dongbao Luo , Nisha Geng , Busheng Wang , Eva Zurek

Recently, ternary clathrate hydrides are promising candidates for high-temperature superconductor. However, it is a formidable challenge to effectively hunt high-temperature superconductivity among multinary hydrides due to the expensive…

Superconductivity · Physics 2024-10-29 Bowen Jiang , Xiaoshan Luo , Toshiaki Iitaka , Ying Sun , Xin Zhong , Jian Lv , Yu Xie , Yanming Ma , Hanyu Liu

After three decades of enormous scientific inquiry, the emergence of superconductivity in the cuprates remains an unsolved puzzle. One major challenge has been to arrive at a satisfactory understanding of the unusual metallic normal state…

Strongly Correlated Electrons · Physics 2019-02-28 Yangmu Li , W. Tabis , Y. Tang , G. Yu , J. Jaroszynski , N. Barišić , M. Greven

The binary polyhydrides of heavy rare earth lutetium that shares a similar valence electron configuration to lanthanum have been experimentally discovered to be superconductive. The lutetium polyhydrides were successfully synthesized at…

Unconventional superconductivity in bilayer graphene has been reported for twist angles $\theta$ near the first magic angle and charged electrostatically with holes near half filling of the lower flat bands. A maximum superconducting…

Superconductivity · Physics 2019-08-06 Dale R. Harshman , Anthony T. Fiory

Recent theoretical and experimental studies of hydrogen-rich materials at megabar pressures (i.e., >100 GPa) have led to the discovery of very high-temperature superconductivity in these materials. Lanthanum superhydride LaH$_{10}$ has been…

Superconductivity · Physics 2022-01-05 Yanfeng Ge , Fan Zhang , Russell J. Hemley

Superconducting behavior even under harsh ambient conditions is expected to occur in La@C(60) if it could be isolated from the primary metallofullerene soot when functionalized by CF(3) radicals. We use ab initio density functional theory…

Materials Science · Physics 2017-08-02 Jie Guan , David Tomanek

Using first-principles calculations, we predict a lightweight room-temperature ferroelectric carbon-boron framework in a host/guest clathrate structure. This ferroelectric clathrate, with composition ScB$_3$C$_3$, exhibits high polarization…

Materials Science · Physics 2020-09-18 Li Zhu , Timothy A. Strobel , R. E. Cohen

The abundant chemical compositions in ternary hydrides bring much more possibility to explore high temperature superconductors under lower pressure. Here we constructed 115 ternary hydrides on the basis of the elements substitution using 16…

Superconductivity · Physics 2024-11-19 Bangshuai Zhu , Dexi Shao , Cuiying Pei , Qi Wang , Juefei Wu , Yanpeng Qi

Single molecule transistors (SMTs) are currently attracting enormous attention as possible quantum information processing devices. An intrinsic limitation to the prospects of these however is associated to the presence of a small number of…

Mesoscale and Nanoscale Physics · Physics 2015-05-14 C. B. Winkelmann , N. Roch , W. Wernsdorfer , V. Bouchiat , F. Balestro

Recent experimental reports on the realizations of two-dimensional (2D) networks of the C60-based fullerenes with anisotropic and nanoporous lattices represent a significant advance, and create exciting prospects for the development of a…

Materials Science · Physics 2023-07-13 Bohayra Mortazavi

Using density-functional-based methods, we show that the hole-doped Li_{x}BC and Na_{x}BC in P6_{3}/mmc crystal structure and C_{x} in graphite structure are capable of showing superconductivity, possibly with a T_{c} much higher than that…

Superconductivity · Physics 2016-08-31 Prabhakar P. Singh

The pursuit of room-temperature superconductors has recently advanced with the discovery of high-temperature superconductivity in compressed hydrides, although sustaining the superconductivity of hydrides at ambient pressure remains…

Superconductivity · Physics 2025-01-28 Ying Sun , Li Zhu

Alkali-fulleride superconductors with a maximum critical temperature Tc of 40 K exhibit similar electronic phase diagram with unconventional high-Tc superconductors where the superconductivity resides proximate to a magnetic Mott-insulating…

Superconductivity · Physics 2020-05-13 Ming-Qiang Ren , Sha Han , Shu-Ze Wang , Jia-Qi Fan , Can-Li Song , Xu-Cun Ma , Qi-Kun Xue

The superconducting parameters are the key for building or identifying the theory responsible for the mechanism of superconductivity. Such parameters for fulleride superconductors have not been well established despite the tremendous…

Superconductivity · Physics 2022-08-09 Ren-Shu Wang , Di Peng , Li-Na Zong , Zeng-Wei Zhu , Xiao-Jia Chen