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Nonlinear optical phenomena in nanostructured materials have been challenging our perceptions of nonlinear optical processes that have been explored since the invention of lasers. For example, the ability to control optical field…

Optical second-harmonic generation (SHG) is a nonlinear parametric process that doubles the frequency of incoming light. Only allowed in non-centrosymmetric materials, it has been widely used in frequency modulation of lasers, surface…

Materials Science · Physics 2021-01-05 Wontaek Kim , Je Yhoung Ahn , Juseung Oh , Ji Hoon Shim , Sunmin Ryu

High-harmonic generation (HHG) provides short-wavelength light that is useful for precision spectroscopy and probing ultrafast dynamics. We report efficient, phase-coherent harmonic generation up to 9th-order (333 nm) in chirped…

By employing a pump-probe technique for enhanced spectral mapping of the dynamics in nonlinear frequency conversion, we demonstrate that photo-induced second-harmonic generation (SHG) in silicon nitride (Si3N4) microresonators can persist…

Topological photonics enables robust light manipulation with third-order optical nonlinearity, yet integrating second-order optical nonlinearity into a topological system faces fundamental challenges: frequency-dependent topological…

Optics · Physics 2025-06-30 Ruoyu Wang , Yiming Pan , Xiaoqin Shen

We report an integrated platform for efficient second-order nonlinear interactions based on linearly uncoupled resonators and angular phase matching. The proposed architecture confines phase control to a limited section of the device,…

Optics · Physics 2026-02-10 Alessia Stefano , Matteo Piccolini , Marco Liscidini

Due to their capacity for non-classical light generation, high-efficiency second-order nonlinear parametric processes play an important role in quantum photonic technology, and chip-scale realization of these processes is recognized as the…

We report a novel quasi-phase matching technique for high-order harmonic generation in low-density gases. Numerical simulations show that in few-optical cycle pulsed Bessel beams it is possible to control the pulse envelope and phase…

Mid-infrared nanophotonics can be realized using sub-diffractional light localization and field enhancement with surface phonon polaritons in polar dielectric materials. We experimentally demonstrate second harmonic generation due to the…

Quasi-phasematched interactions in waveguides with quadratic nonlinearities enable highly efficient nonlinear frequency conversion. In this article, we demonstrate the first generation of devices that combine the dispersion-engineering…

We report experimental results on second-harmonic generation in a z-cut quartz crystal under conditions of free-space quasi-phase matching in a multi-pass cell. In a 62-pass configuration, an efficiency of 0.027% or 1.4x10-4 %/MW/cm2 was…

Optics · Physics 2026-04-10 Nazar Kovalenko , Ankit Pai , Oleg Pronin

Chip-scale nonlinear optics enables strong light-matter interactions within compact devices, serving as a fundamental platform for multifunctional integrated photonics from classical optical signal processing to quantum information…

We propose a method for generating only even-order high harmonics. We formulate a condition for a shift in the relative-phase between bi-chromatic drivers that leads to a field sign-flip of only even-order harmonics. Induction of this…

Optics · Physics 2015-06-17 Tzvi Diskin , Oren Cohen

We describe an approach based on topology optimization that enables automatic discovery of wavelength-scale photonic structures for achieving high-efficiency second-harmonic generation (SHG). A key distinction from previous formulation and…

The 4-bar crystal symmetry in materials such as GaAs can enable quasi-phasematching for efficient frequency conversion without poling, twinning or other engineered domain inversions. 4-bar symmetry means that a 90 degree rotation is…

Mesoscale and Nanoscale Physics · Physics 2012-10-09 Paulina S. Kuo , Glenn S. Solomon

Bound states in the continuum (BICs) have been extensively studied in various systems since its first proposal in quantum mechanics. Photonic BICs can enable optical mode confinement and provide field enhancement for nonlinear optics, but…

Optics · Physics 2021-10-01 Fan Ye , Yue Yu , Xiang Xi , Xiankai Sun

We study surface second-harmonic generation (SHG) from a singular plasmonic structure consisting of touching metallic wires. We use the technique of transformation optics and relate the structure to a rather simpler geometry, a slab…

We investigate second-order nonlinear processes in a system of two coupled identical optical micro-resonators. The double resonance and phase-matching conditions are simultaneously obtained thanks to the frequency splitting induced by the…

Optics · Physics 2025-10-03 Yannick Dumeige , Yoan Léger

Domain-engineered quasi-phase-matching (QPM) devices are known for its versatility and ability to tune the nonlinear optical frequency conversion process. In this paper, a simple approach is presented to generate multiple…

In this paper we present a theoretical examination of second-harmonic generation (SHG) in a graphene monolayer integrated within an attenuated total internal reflection (ATR) configuration. By embedding graphene in this optical setup, we…