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We present time-resolved X-ray diffraction measurements using advanced timing schemes that provide high temporal resolution while also maintaining a high flux in the X-ray probe beam. The method employs patterned probe pulse sequences that…

Accurate characterization of radiation pulse profiles is crucial for optimizing beam quality and enhancing experimental outcomes in Free Electron Laser (FEL) research. In this paper, we present a novel approach that employs machine learning…

Accelerator Physics · Physics 2024-11-27 Till Korten , Vladimir Rybnikov , Peter Steinbach , Najmeh Mirian

We examine time-resolved X-ray diffraction from molecules in the gas phase which undergo nonadiabatic avoided-crossing dynamics involving strongly coupled electrons and nuclei. Several contributions to the signal are identified,…

Chemical Physics · Physics 2017-05-30 Markus Kowalewski , Kochise Bennett , Shaul Mukamel

Plane-wave electrons undergo momentum transfer as they scatter off a target in overlapping spherical waves. The transferred momentum leads to target structural information to be encoded in angle and energy differential scattering. For…

Atomic and Molecular Clusters · Physics 2024-02-14 Aiswarya R. , Rasheed Shaik , Jobin Jose , Hari R. Varma , Himadri S. Chakraborty

In materials science and particularly electron microscopy, Electron Back-scatter Diffraction (EBSD) is a common and powerful mapping technique for collecting local crystallographic data at the sub-micron scale. The quality of the…

Computer Vision and Pattern Recognition · Computer Science 2019-03-08 Florian Strub , Marie-Agathe Charpagne , Tresa M. Pollock

Probing signal injection is a well-established technique to extract additional information from a weakly (or non) observable dynamical system. Using averaging theory, a framework to analyse such schemes for general nonlinear systems has…

Systems and Control · Computer Science 2019-11-20 Bowen Yi , Romeo Ortega , Houria Siguerdidjane , Juan E. Machado , Weidong Zhang

Streaking of photoelectrons has long been used for the temporal characterization of attosecond extreme ultraviolet pulses. When the time-resolved photoelectrons originate from a coherent superposition of electronic states, they carry an…

Chemical Physics · Physics 2016-07-27 Markus Kowalewski , Kochise Bennett , Jérémy R. Rouxel , Shaul Mukamel

We propose a novel way to image dynamical properties of nonstationary electron systems using ultrafast resonant x-ray scattering. Employing a rigorous theoretical analysis within the framework of quantum electrodynamics, we demonstrate that…

Atomic Physics · Physics 2017-11-03 Daria Popova-Gorelova , Robin Santra

It has been shown that with the use of ultra-wideband (UWB) electromagnetic signal and time of arrival (ToA) principle, it is possible to locate medical implants given the permittivity distribution of the body. We propose a new imaging…

Image and Video Processing · Electrical Eng. & Systems 2020-03-03 Tao Feng

Laser-induced electron diffraction is an evolving tabletop method, which aims to image ultrafast structural changes in gas-phase polyatomic molecules with sub-{\AA}ngstr\"om spatial and femtosecond temporal resolution. Here, we provide the…

Real-time simulations of laser-driven electron dynamics contain information about molecular optical properties through all orders in response theory. These properties can be extracted by assuming convergence of the power series expansion of…

Ultra-fast transmission electron microscopy (UTEM) combines sub-picosecond time-resolution with the versatility of TEM spectroscopies. It allows one to study the dynamics of materials properties combining complementary techniques. However,…

Materials Science · Physics 2021-08-25 S. Meuret , L. H. G. Tizei , F. Houdellier , S. Weber , Y. Auad , M. Tencé , H. -C. Chang , M. Kociak , A. Arbouet

Megaelectronvolt ultrafast electron diffraction (UED) is a promising detection tool for ultrafast processes. The quality of diffraction image is determined by the transverse evolution of the probe bunch. In this paper, we study the…

Accelerator Physics · Physics 2015-06-18 Xianhai Lu , Yingchao Du , Wenhui Huang , Chuanxiang Tang

Ultrafast diffraction imaging is a powerful tool to retrieve the geometric structure of gas-phase molecules with combined picometre spatial and attosecond temporal resolution. However, structural retrieval becomes progressively difficult…

Chemical Physics · Physics 2021-10-13 Xinyao Liu , Kasra Amini , Aurelien Sanchez , Blanca Belsa , Tobias Steinle , Jens Biegert

Using a new technique to directly detect current induced on a nearby electrode, we measure plasma oscillations in ultracold plasmas, which are influenced by the inhomogeneous and time-varying density and changing neutrality. Electronic…

Plasma Physics · Physics 2012-02-10 K. A. Twedt , S. L. Rolston

Advancements in fast electron detectors have enabled the statistically significant sampling of crystal structures on the nanometre scale by means of Scanning Electron Nanobeam Diffraction (SEND). Characterisation of structural similarity…

Materials Science · Physics 2022-07-28 Andy Bridger , William I. F. David , Thomas J. Wood , Mohsen Danaie , Keith T. Butler

A time-dependent potential barrier has been used to probe the arrival-time distribution of the wave packet of a hot electron by raising the barrier to block the packet upon arrival of the packet at the barrier. To see whether the barrier…

Mesoscale and Nanoscale Physics · Physics 2023-12-07 Wanki Park , H. -S. Sim , Sungguen Ryu

Ion-assisted surface processes are the basis of modern plasma processing. Ion energy distribution (IED) control is critical for precise material modification, especially in atomic-level technologies such as atomic layer etching. Since this…

Plasma Physics · Physics 2021-08-11 M. Bogdanova , D. Lopaev , T. Rakhimova , D. Voloshin , A. Zotovich , S. Zyryanov

Ultrasound shear wave elasticity imaging is a valuable tool for quantifying the elastic properties of tissue. Typically, the shear wave velocity is derived and mapped to an elasticity value, which neglects information such as the shape of…

Image and Video Processing · Electrical Eng. & Systems 2022-04-29 Maximilian Neidhardt , Marcel Bengs , Sarah Latus , Stefan Gerlach , Christian J. Cyron , Johanna Sprenger , Alexander Schlaefer

Electron backscatter diffraction (EBSD) in the scanning electron microscope is routinely used for microstructural characterisation of polycrystalline materials. Maps of EBSD data are typically acquired at high stage tilt and slow scan…

Materials Science · Physics 2020-09-01 Vivian Tong , Thomas Benjamin Britton
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