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We present a comprehensive study of single crystals of Na2Co2TeO6, a putative Kitaev honeycomb magnet, focusing on its low-temperature phase behaviors. A new thermal phase transition is identified at 31.0 K, below which the system develops…

Strongly Correlated Electrons · Physics 2021-05-26 Wenjie Chen , Xintong Li , Zhenhai Hu , Ze Hu , Li Yue , Ronny Sutarto , Feizhou He , Kazuki Iida , Kazuya Kamazawa , Weiqiang Yu , Xi Lin , Yuan Li

We have synthesized single crystals of Na$_3$Co$_2$SbO$_6$ and characterized the structure and magnetic order by measuring anisotropic magnetic properties, heat capacity, x-ray and neutron single crystal diffraction. Magnetic properties and…

Strongly Correlated Electrons · Physics 2019-07-17 J. -Q. Yan , S. Okamoto , Y. Wu , Q. Zheng , H. D. Zhou , H. B. Cao , M. A. McGuire

From magnetic susceptibility, dielectric permittivity, electric polarization and specific heat measurements, we discover spin-induced ferroelectricity and magnetoelectric coupling in Mn3TeO6 and observe two successive magnetic transitions…

Materials Science · Physics 2015-12-01 L. Zhao , Z. Hu , C. Y. Kuo , T. -W. Pi , M. -K. Wu , L. H. Tjeng , A. C. Komarek

We have performed a resonant x-ray scattering study at the Co pre-K edge on a single crystal of Ca3Co2O6. The measurements reveal an abrupt transition to a magnetically ordered state immediately below T_N = 25 K, with a magnetic correlation…

Other Condensed Matter · Physics 2008-05-10 S. Agrestini , C. Mazzoli , A. Bombardi , M. R. Lees

Low-dimensional magnetic systems based on honeycomb lattices provide a promising platform for exploring exotic quantum phenomena that emerge from the intricate interplay of competing spin, orbital, lattice, and dipolar degrees of freedom.…

To study the relationship between the properties of low-dimensional spin systems with weakly coupled Cu-triangles and their crystal structure, single crystals of $Cs_3Cu_3Cl_8OH$ (1) and the new $Cs_3Cu_3Cl_{7.6}Br_{0.4}OH$ (2) were grown.…

Li3Co2SbO6 is prepared by molten salt ion exchange and its structure refined by the Rietveld method confirming the honeycomb-type Co/Sb ordering of its Na precursor. Monoclinic rather than trigonal symmetry of Na3Co2SbO6 is directly…

The microscopic spin-spin correlations in the 2D layered spin-1 honeycomb lattice compound Na2Ni2TeO6 have been investigated by neutron diffraction and inelastic neutron scattering. The honeycomb lattice of spin-1 Ni2+ ions, within the…

Strongly Correlated Electrons · Physics 2022-02-17 A. K. Bera , S. M. Yusuf , L. Keller , F. Yokaichiya , J. R. Stewart

We report on the results of 23Na NMR in the honeycomb lattice magnet Na2Co2TeO6 which has been nominated as a Kitaev material. Measurements of magnetic shift and width of the NMR line as functions of temperature and magnetic field show that…

Strongly Correlated Electrons · Physics 2022-12-21 Jun Kikuchi , Takayuki Kamoda , Nobuyoshi Mera , Yodai Takahashi , Kouji Okumura , Yukio Yasui

Na4Ir3O8 is a unique case of a hyperkagome 3D corner sharing triangular lattice which can be decorated with quantum spins. It has spurred a lot of theoretical interest as a spin liquid candidate. We present a comprehensive set of NMR data…

Strongly Correlated Electrons · Physics 2015-07-29 A. C. Shockley , F. Bert , J-C Orain , Y. Okamoto , P. Mendels

The layered compound La2-2xSr1+2xMn2O7 (x=0.3) consists of bilayers of metallic MnO2 sheets separated by insulating material. The compound exhibits markedly anisotropic magnetoresistance at temperatures well below the three-dimensional…

Strongly Correlated Electrons · Physics 2009-10-31 T. G. Perring , G. Aeppli , T. Kimura , Y. Tokura , M. A. Adams

Multiple structure and symmetry types and their transformations are discovered in quasi-two-dimensional (quasi-2D) Cr2Ge2Te6 crystal in surprisingly very narrow temperature range of 2 K and magnetic field range of 0.07 T using a homebuilt…

Materials Science · Physics 2018-03-22 Tengfei Guo , Zongwei Ma , Gaoting Lin , Xuan Luo , Yubin Hou , Yuping Sun , Zhigao Sheng , Qingyou Lu

Magnetic order and the underlying magnetic model of the multiferroic pyroxene NaFeGe2O6 are systematically investigated by neutron powder diffraction, thermodynamic measurements, density-functional bandstructure calculations, and…

Strongly Correlated Electrons · Physics 2018-09-19 Lei Ding , Pascal Manuel , Dmitry D. Khalyavin , Fabio Orlandi , Alexander A. Tsirlin

As a candidate Kitaev material, Na$_2$Co$_2$TeO$_6$ exhibits intriguing magnetism on a honeycomb lattice that is believed to be $C_3$-symmetric. Here we report a neutron diffraction study of high quality single crystals under $a$-axis…

Strongly Correlated Electrons · Physics 2023-06-06 Weiliang Yao , Yang Zhao , Yiming Qiu , Christian Balz , J. Ross Stewart , Jeffrey W. Lynn , Yuan Li

This paper presents structural, detailed magnetic, and exchange bias studies in polycrystalline Ba$_{2}$ScRuO$_{6}$ synthesized at ambient pressure. In contrast to its strontium analogue, this material crystallizes in a 6L hexagonal…

Materials Science · Physics 2023-04-28 Prachi Mohanty , Sourav Marik , R. P. Singh

We report that the major features in the temperature dependence of dc and ac magnetization of a well-known spin-chain compound, Ca3Co2O6, which has been known to exhibit two complex magnetic transitions due to geometrical frustration (one…

Strongly Correlated Electrons · Physics 2015-05-13 Niharika Mohapatra , Kartik K Iyer , Sitikantha D Das , B. A. Chalke , S. C. Purandare , E. V. Sampathkumaran

Ion-exchange treatment of Na2SnTeO6 in molten salt mixtures resulted in rosiaite (PbSb2O6)-related MnSnTeO6. Its crystal structure was refined by the Rietveld method. Of the three possible models of Sn/Te distribution, the disordered model…

We present new experimental results of low temperature x-ray synchrotron diffraction, neutron scattering and very low temperature (mK-range) bulk measurements on the nanotube system ${\tube}$. The crystal structure determined from our data…

We investigated the crystal and magnetic structures of the spin-1/2 frustrated antiferromagnet Cu3Mo2O9 in which the spin system consists of antiferromagnetic chains and dimers. The space group at room temperature has been reported to be…

The dimensionality of the electronic and magnetic structure of a given material is generally predetermined by its crystal structure. Here, using elastic and inelastic neutron scattering combined with magnetization measurements, we find…

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