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We show that centrosymmetric natural hyperbolic media such as hexagonal boron nitride exhibit a bulk second-order nonlinear response, leading to second-harmonic and sum- and difference-frequency generation with efficiencies comparable to…

Optics · Physics 2026-05-26 Evgenii E. Narimanov

Here we employ the quasi-bound state in the continuum (quasi-BIC) resonance in all-dielectric metasurfaces for efficient nonlinear processes in consideration of the backward frequency conversion. We theoretically study the second-harmonic…

Optics · Physics 2024-06-28 Xu Tu , Siqi Feng , Jiajun Li , Yangguang Xing , Feng Wu , Tingting Liu , Shuyuan Xiao

In this work, we investigate the generation of second harmonic light by gold nanorods and demonstrate that the collected nonlinear intensity depends upon a phase interplay between different modes available in the nanostructure. By recording…

We conduct a theoretical and numerical study on the second-harmonic (SH) optical response of a nano-structured metamaterial composed of a periodic array of inclusions. Both the inclusions and their surrounding matrix are made of…

Mesoscale and Nanoscale Physics · Physics 2019-03-13 Ulises R. Meza , Bernardo S. Mendoza , W. Luis Mochán

Second-order nonlinear optical response allows to detect different properties of the system associated with the inversion symmetry breaking. Here, we use a second harmonic generation effect to investigate the alignment of a…

Mesoscale and Nanoscale Physics · Physics 2020-07-03 E. A. Stepanov , S. V. Semin , C. R. Woods , M. Vandelli , A. V. Kimel , K. S. Novoselov , M. I. Katsnelson

In nonlinear nanophotonics, cascaded second-harmonic generation (SHG) in pure plasmonic waveguides for sequential signal transformation and complex on-chip functionality remains a long-standing challenge. Precise phase matching becomes…

Optics · Physics 2025-08-22 Komal Gupta , Anand Hegde , Xiaofei Wu , Jer-Shing Huang , Chen-Bin Huang

We study the main nonlinear solutions of plasmonic slot waveguides made from an anisotropic metamaterial core with a positive Kerr-type nonlinearity surrounded by two semi-infinite metal regions. First, we demonstrate that for a highly…

Optics · Physics 2018-01-15 Mahmoud M. R. Elsawy , Gilles Renversez

In this work, we utilize thin dielectric meta-atoms placed on a silver substrate to efficiently enhance and manipulate the third harmonic generation. We theoretically and experimentally reveal that when the structural symmetry of the…

We demonstrate phase-matched second-harmonic generation (SHG) from three-dimensional metamaterials consisting of stacked metasurfaces. To achieve phase matching, we utilize a novel mechanism based on phase engineering of the metasurfaces at…

We experimentally and theoretically investigate the second order nonlinear optical response of metallo-dielectric multilayer structures composed of Ag and Ta2O5 layers, deposited by magnetron sputtering. Second harmonic generation…

We report the enhancement of the optical second harmonic signal in non-centrosymmetric semiconductor CdS quantum dots, when they are placed in close contact with isolated silver nanoparticles. The intensity enhancement is about 1000. We…

Mesoscale and Nanoscale Physics · Physics 2012-02-15 Pablo M. Jais , Catalina von Bilderling , Andrea V. Bragas

Plasmonic dimer antennas create strong field enhancement by squeezing light into a nanoscale gap. These optical hotspots are highly attractive for boosting nonlinear processes, such as harmonic generation, photoelectron emission, and…

The topological Weyl semimetals with peculiar band structure exhibit novel nonlinear optical enhancement phenomena even for light at optical wavelengths. While many intriguing nonlinear optical effects were constantly uncovered in type-I…

We show that the nonlinear optical response reflects sensitively the electronic structure of transition-metal surfaces and interfaces. $d$ and $s$ electrons may contribute rather differently to the second harmonic generation (SHG) signal.…

Condensed Matter · Physics 2007-05-23 W. H"ubner , K. H. Bennemann , K. Böhmer

The nonlinear processes of frequency conversion like second harmonic generation (SHG) usually obey certain selection rules, resulting from the preservation of different kind of physical quantities, e.g., the angular momentum. For SHG…

Optics · Physics 2020-04-09 Florian Spreyer , Ruizhe Zhao , Lingling Huang , Thomas Zentgraf

Plasmonic metamaterials and metasurfaces offer new opportunities in developing high performance terahertz emitters and detectors beyond the limitations of conventional nonlinear materials. However, simple meta-atoms for second-order…

Dielectric metasurfaces provide a unique platform for efficient harmonic generation and optical wavefront manipulation at the nanoscale. While several approaches are available for performing wavefront shaping, the one exploiting geometric…

We present a study of the second-order nonlinear optical properties of metal-based metamaterials. A hydrodynamic model for electronic response is used, in which nonlinear surface contributions are expressed in terms of the bulk…

The optical theorem relates the total scattering cross-section of a given structure with its forward scattering, but does not impose any restrictions on other directions. Strong backward-forward asymmetry in scattering could be achieved by…

Other Condensed Matter · Physics 2016-11-22 Vitali Kozlov , Dmitry Filonov , Alexander S. Shalin , Ben Z. Steinberg , Pavel Ginzburg

High-harmonic generation (HHG) in solids has rapidly emerged as a promising platform for creating compact attosecond sources and probing ultrafast electron dynamics. Resonant metasurfaces are essential for enhancement of the otherwise small…